33 research outputs found
Strong coupling of excitons in 2D MoSe2/hBN heterostructure with optical bound states in the continuum
We experimentally demonstrate strong exciton-photon coupling in a MoSe2/hBN heterostructure interfaced with an all-dielectric metasurface supporting high-Q bound states in the continuum. The resulting exciton-polaritons are probed by means of temperature- and angle-resolved reflectivity and photoluminescence. Our findings pave the way towards new-generation nonlinear planar polaritonic devices
Negative local resistance caused by viscous electron backflow in graphene
Graphene hosts a unique electron system in which electron-phonon scattering
is extremely weak but electron-electron collisions are sufficiently frequent to
provide local equilibrium above liquid nitrogen temperature. Under these
conditions, electrons can behave as a viscous liquid and exhibit hydrodynamic
phenomena similar to classical liquids. Here we report strong evidence for this
transport regime. We find that doped graphene exhibits an anomalous (negative)
voltage drop near current injection contacts, which is attributed to the
formation of submicrometer-size whirlpools in the electron flow. The viscosity
of graphene's electron liquid is found to be ~0.1 m /s, an order of
magnitude larger than that of honey, in agreement with many-body theory. Our
work shows a possibility to study electron hydrodynamics using high quality
graphene
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Large magnetoelectric coupling in multiferroic oxide heterostructures assembled via epitaxial lift-off.
Epitaxial films may be released from growth substrates and transferred to structurally and chemically incompatible substrates, but epitaxial films of transition metal perovskite oxides have not been transferred to electroactive substrates for voltage control of their myriad functional properties. Here we demonstrate good strain transmission at the incoherent interface between a strain-released film of epitaxially grown ferromagnetic La0.7Sr0.3MnO3 and an electroactive substrate of ferroelectric 0.68Pb(Mg1/3Nb2/3)O3-0.32PbTiO3 in a different crystallographic orientation. Our strain mediated magnetoelectric coupling compares well with respect to epitaxial heterostructures, where the epitaxy responsible for strong coupling can degrade film magnetization via strain and dislocations. Moreover, the electrical switching of magnetic anisotropy is repeatable and non volatile. High resolution magnetic vector maps reveal that micromagnetic behaviour is governed by electrically controlled strain and film microstructure. Our demonstration should permit the physical/chemical properties in strain-released epitaxial oxide films to be controlled using electroactive substrates to impart strain via non epitaxial interfaces.Beatriu de Pinós postdoctoral fellowship (2014 BP-A 00079) from the Catalan government via the Agència de Gestió d’Ajuts Universitaris i de Recerca (AGAUR); Ministry of Science and Higher Education of Russian Federation, goszadanie no. 2019-1246; the Royal Society; EPSRC (Grant EP/P009050/1, EP/M010619/1 and the NoWNano DTC); European Research Council (ERC) (ERC-2016-STG-EvoluTEM-715502 and ERC Synergy HETERO2D); “la Caixa” Foundation (ID 100010434)
Strained bubbles in van der Waals heterostructures as local emitters of photoluminescence with adjustable wavelength
The
possibility to tailor photoluminescence (PL) of monolayer transition
metal dichalcogenides (TMDCs) using external factors such as strain,
doping, and external environment is of significant interest for optoelectronic
applications. Strain in particular can be exploited as a means to
continuously vary the band gap. Micrometer-scale strain gradients
were proposed for creating “artificial atoms” that can
utilize the so-called exciton funneling effect and work, for example,
as exciton condensers. Here we describe room-temperature PL emitters
that naturally occur whenever monolayer TMDC is deposited on an atomically
flat substrate. These are hydrocarbon-filled bubbles, which provide
predictable, localized PL from well-separated sub-micrometer areas.
Their emission energy is determined by the built-in strain controlled
only by the substrate material, such that both the maximum strain
and the strain profile are universal for all bubbles on a given substrate,
i.e., independent of the bubble size. We show that for bubbles formed
by monolayer MoS<sub>2</sub>, PL can be tuned between 1.72 and 1.81
eV by choosing bulk PtSe<sub>2</sub>, WS<sub>2</sub>, MoS<sub>2</sub>, or graphite as a substrate, and its intensity is strongly enhanced
by the funneling effect. Strong substrate-dependent quenching of the
PL in areas of good contact between MoS<sub>2</sub> and the substrate
ensures localization of the luminescence to bubbles only; by employing
optical reflectivity measurements we identify the mechanisms responsible
for the quenching. Given the variety of available monolayer TMDCs
and atomically flat substrates and the ease of creating such bubbles,
our findings open a venue for making and studying the discussed light-emitting
“artificial atoms” that could be used in applications
High-temperature quantum oscillations caused by recurring Bloch states in graphene superlattices
Cyclotron motion of charge carriers in metals and semiconductors leads to Landau quantization and magneto-oscillatory behavior in their properties. Cryogenic temperatures are usually required to observe these oscillations. We show that graphene superlattices support a different type of quantum oscillations that do not rely on Landau quantization. The oscillations are extremely robust and persist well above room temperature in magnetic fields of only a few T. We attribute this phenomenon to repetitive changes in the electronic structure of superlattices such that charge carriers experience effectively no magnetic field at simple fractions of the flux quantum per superlattice unit cell. Our work points at unexplored physics in Hofstadter butterfly systems at high temperatures
Strained graphene structures: from valleytronics to pressure sensing
Due to its strong bonds graphene can stretch up to 25% of its original size
without breaking. Furthermore, mechanical deformations lead to the generation
of pseudo-magnetic fields (PMF) that can exceed 300 T. The generated PMF has
opposite direction for electrons originating from different valleys. We show
that valley-polarized currents can be generated by local straining of
multi-terminal graphene devices. The pseudo-magnetic field created by a
Gaussian-like deformation allows electrons from only one valley to transmit and
a current of electrons from a single valley is generated at the opposite side
of the locally strained region. Furthermore, applying a pressure difference
between the two sides of a graphene membrane causes it to bend/bulge resulting
in a resistance change. We find that the resistance changes linearly with
pressure for bubbles of small radius while the response becomes non-linear for
bubbles that stretch almost to the edges of the sample. This is explained as
due to the strong interference of propagating electronic modes inside the
bubble. Our calculations show that high gauge factors can be obtained in this
way which makes graphene a good candidate for pressure sensing.Comment: to appear in proceedings of the NATO Advanced Research Worksho