Neutron capture cross sections of 69Ga and 71Ga at 25 keV and e peak = 90 keV

This project was supported by EFNUDAT, ERINDA, the EuroGENESIS project MASCHE, HIC for FAIR and BMBF (05P15RFFN1).We measured the neutron capture cross sections of 69Ga and 71Ga for a quasi-stellar spectrum at kBT = 25 keV and a spectrum with a peak energy at 90 keV by the activation technique at the Joint Research Centre (JRC) in Geel, Belgium. Protons were provided by an electrostatic Van de Graaff accelerator to produce neutrons via the reaction 7Li(p,n). The produced activity was measured via the γ emission of the product nuclei by high-purity germanium detectors. We present preliminary results.publishersversionpublishe

Measurement of the 244^{244}Cm and 246^{246}Cm Neutron-Induced Cross Sections at the n_TOF Facility

The neutron capture reactions of the $^{244}$Cm and $^{246}$Cm isotopes open the path for the formation of heavier Cm isotopes and of heavier elements such as Bk and Cf in a nuclear reactor. In addition, both isotopes belong to the minor actinides with a large contribution to the decay heat and to the neutron emission in irradiated fuels proposed for the transmutation of nuclear waste and fast critical reactors. The available experimental data for both isotopes are very scarce. We measured the neutron capture cross section with isotopically enriched samples of $^{244}$Cm and $^{246}$Cm provided by JAEA. The measurement covers the range from 1 eV to 250 eV in the n_TOF Experimental Area 2 (EAR-2). In addition, a normalization measurement with the $^{244}$Cm sample was performed at Experimental Area 1 (EAR-1) with the Total Absorption Calorimeter (TAC)

Reactor neutrons in nuclear astrophysics

The huge neutron fluxes offer the possibility to use research reactors to produce isotopes of interest, which can be investigated afterwards. An example is the half-lives of long-lived isotopes like 129I. A direct usage of reactor neutrons in the astrophysical energy regime is only possible, if the corresponding ions are not at rest in the laboratory frame. The combination of an ion storage ring with a reactor and a neutron guide could open the path to direct measurements of neutron-induced cross sections on short-lived radioactive isotopes in the astrophysically interesting energy regime

Reactor neutrons in nuclear astrophysics

The huge neutron fluxes offer the possibility to use research reactors to produce isotopes of interest, which can be investigated afterwards. An example is the half-lives of long-lived isotopes like 129I. A direct usage of reactor neutrons in the astrophysical energy regime is only possible, if the corresponding ions are not at rest in the laboratory frame. The combination of an ion storage ring with a reactor and a neutron guide could open the path to direct measurements of neutron-induced cross sections on short-lived radioactive isotopes in the astrophysically interesting energy regime

Neutron capture cross sections of 69Ga and 71Ga at 25 keV and Epeak = 90 keV

We measured the neutron capture cross sections of 69Ga and 71Ga for a quasi-stellar spectrum at kBT = 25 keV and a spectrum with a peak energy at 90 keV by the activation technique at the Joint Research Centre (JRC) in Geel, Belgium. Protons were provided by an electrostatic Van de Graaff accelerator to produce neutrons via the reaction 7Li(p,n). The produced activity was measured via the γ emission of the product nuclei by high-purity germanium detectors. We present preliminary results

Neutron-induced cross sections

Neutron capture cross sections are one of the most important nuclear inputs to models of stellar nucleosynthesis of the elements heavier than iron. The activation technique and the time-of-flight method are mostly used to determine the required data experimentally. Recent developments of experimental techniques allow for new experiments on radioactive isotopes. Monte-Carlo based analysis methods give new insights into the systematic uncertainties of previous measurements. We present an overview over the state-of-the-art experimental techniques, a detailed new evaluation of the $^{197}$Au(n,$\gamma$) cross section in the keV-regime and the corresponding re-evaluation of 63 more isotopes, which have been measured in the past relative to the gold cross section.Comment: 34 pages, 83 fig

Neutron activation of Ga 69 and Ga 71 at kBT≈25 keV

Funding Information: This project was supported by EFNUDAT, ERINDA, the EuroGENESIS project MASCHE, HIC for FAIR, BMBF (05P15RFFN1) and DFG (RE 3461/4-1).Background: About 50% of heavy elements are produced by the slow neutron capture process (s process) in stars. The element gallium is mostly produced during the weak s process in massive stars. Purpose: Our activation at kBT≈25 keV is the first experiment in a series of activation and time-of-flight measurements on Ga69 and Ga71 relevant for astrophysics. Methods: We activated Ga69 and Ga71 with a neutron distribution that corresponds to a quasistellar distribution with kBT=25keV at the Joint Research Centre (JRC), Geel, Belgium. Protons were provided by an electrostatic Van de Graaff accelerator to produce neutrons via the reaction Li7(p,n). The produced activity was measured via the γ emission by the decaying product nuclei by high-purity germanium detectors. Results: We provide spectrum-averaged cross sections (SACS) and ratios of the cross sections σGa/σAu for the neutron spectrum of the activation. We obtain values of σ69Ga,SACS=(186±12)mb and σ71Ga,SACS=(112±7)mb, and cross-section ratios of σ69Ga/σAu=0.29±0.02 and σ71Ga/σAu=0.17±0.01. Conclusions: Our data disagree with the available evaluated data provided by KADoNiS v0.3, our cross-section ratio is about 20% higher for Ga69 and about 20% lower for Ga71.publishersversionpublishe

63Ni(n,γ) cross sections measured with DANCE

The neutron capture cross section of the s-process branch nucleus 63Ni affects the abundances of other nuclei in its region, especially 63Cu and 64Zn. In order to determine the energy-dependent neutron capture cross section in the astrophysical energy region, an experiment at the Los Alamos National Laboratory has been performed using the calorimetric 4πBaF2 array DANCE. The (n,γ) cross section of 63Ni has been determined relative to the well-known 197Au standard with uncertainties below 15%. Various 63Ni resonances have been identified based on the Q value. Furthermore, the s-process sensitivity of the new values was analyzed with the new network calculation tool NETZ