49 research outputs found
Spins, Electromagnetic Moments, and Isomers of 107-129Cd
The neutron-rich isotopes of cadmium up to the N=82 shell closure have been
investigated by high-resolution laser spectroscopy. Deep-UV excitation at 214.5
nm and radioactive-beam bunching provided the required experimental
sensitivity. Long-lived isomers are observed in 127Cd and 129Cd for the first
time. One essential feature of the spherical shell model is unambiguously
confirmed by a linear increase of the 11/2- quadrupole moments. Remarkably,
this mechanism is found to act well beyond the h11/2 shell
Calculation of energy levels and transition amplitudes for barium and radium
The radium atom is a promising system for studying parity and time invariance
violating weak interactions. However, available experimental spectroscopic data
for radium is insufficient for designing an optimal experimental setup. We
calculate the energy levels and transition amplitudes for radium states of
significant interest. Forty states corresponding to all possible configurations
consisting of the , and single-electron states as well as the
states of the , and configurations have been calculated.
The energies of ten of these states corresponding to the , ,
, and configurations are not known from experiment. Calculations
for barium are used to control the accuracy.Comment: 12 pages, 4 table
Charge radii and electromagnetic moments of 195-211At
Hyperfine-structure parameters and isotope shifts of At195-211 have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantly α-decaying nuclei. The electromagnetic moments and changes in the mean-square charge radii of the astatine nuclei have been extracted from the measured hyperfine-structure constants and isotope shifts. This was only made possible by dedicated state-of-the-art large-scale atomic computations of the electronic factors and the specific mass shift of atomic transitions in astatine that are needed for these extractions. By comparison with systematics, it was possible to assess the reliability of the results of these calculations and their ascribed uncertainties. A strong deviation in the ground-state mean-square charge radii of the lightest astatine isotopes, from the trend of the (spherical) lead isotopes, is interpreted as the result of an onset of deformation. This behavior bears a resemblance to the deviation observed in the isotonic polonium isotopes. Cases for shape coexistence have been identified in At197,199, for which a significant difference in the charge radii for ground (9/2-) and isomeric (1/2+) states has been observed
Characterization of the shape-staggering effect in mercury nuclei
In rare cases, the removal of a single proton (Z) or neutron (N) from an atomic nucleus leads to a dramatic shape change. These instances are crucial for understanding the components of the nuclear interactions that drive deformation. The mercury isotopes (Z = 80) are a striking example1,2: their close neighbours, the lead isotopes (Z = 82), are spherical and steadily shrink with decreasing N. The even-mass (A = N + Z) mercury isotopes follow this trend. The odd-mass mercury isotopes 181,183,185Hg, however, exhibit noticeably larger charge radii. Due to the experimental difficulties of probing extremely neutron-deficient systems, and the computational complexity of modelling such heavy nuclides, the microscopic origin of this unique shape staggering has remained unclear. Here, by applying resonance ionization spectroscopy, mass spectrometry and nuclear spectroscopy as far as 177Hg, we determine 181Hg as the shape-staggering endpoint. By combining our experimental measurements with Monte Carlo shell model calculations, we conclude that this phenomenon results from the interplay between monopole and quadrupole interactions driving a quantum phase transition, for which we identify the participating orbitals. Although shape staggering in the mercury isotopes is a unique and localized feature in the nuclear chart, it nicely illustrates the concurrence of single-particle and collective degrees of freedom at play in atomic nuclei
Relativistic lifetimes of the levels belonging to the configuration in As I, Sb I and Bi I spectra
Relativistic multiconfiguration Dirac-Fock study of transition in aluminium isoelectronic sequence
Optical excitation of ultra-relativistic partially stripped ions
The Gamma Factory (GF) initiative aims at the construction of a unique
experimental tool exploiting resonant interaction of light with
ultra-relativistic partially stripped ions (PSI) stored in circular
accelerators at CERN. Resonant excitation of high-energy electronic transitions
in the ions is achieved through Doppler-boosting (by twice the Lorentz factor;
from hundred to several thousand times) of light energy. In order to
efficiently excite the ions, and hence generate intense beams of
scattered/fluorescent photons, a detailed knowledge of the ions' electronic
energy structure and the dynamics of optical excitation is required.
Spectroscopic properties of PSI selected for the GF operation, as well as their
optical excitation schemes, are investigated. Two regimes of the ion--light
interaction are identified, leading to different dynamics of the excitation.
The efficiency of the ion--light interaction, as well as the number of photons
emitted from a single ion bunch, are estimated, both analytically and
numerically, for three ions considered for the GF, i.e.~Li-like
Pb, Li-like Ca, and
H-like Pb.Comment: Ann. Phys. 534, 2100250 (2022