Nonlinear Decay of Quantum Confined Magnons in Itinerant Ferromagnets

Quantum confinement leads to the emergence of several magnon modes in ultrathin layered magnetic structures. We probe the lifetime of these quantum confined modes in a model system composed of three atomic layers of Co grown on different surfaces. We demonstrate that the quantum confined magnons exhibit nonlinear decay rates, which strongly depend on the mode number, in sharp contrast to what is assumed in the classical dynamics. Combining the experimental results with those of linear-response density functional calculations we provide a quantitative explanation for this nonlinear damping effect. The results provide new insights into the decay mechanism of spin excitations in ultrathin films and multilayers and pave the way for tuning the dynamical properties of such structures

Detailed Studies of Pixelated CZT Detectors Grown with the Modified Horizontal Bridgman Method

The detector material Cadmium Zinc Telluride (CZT), known for its high resolution over a broad energy range, is produced mainly by two methods: the Modified High-Pressure Bridgman (MHB) and the High-Pressure Bridgman (HPB) process. This study is based on MHB CZT substrates from the company Orbotech Medical Solutions Ltd. with a detector size of 2.0x2.0x0.5 cm^3, 8x8 pixels and a pitch of 2.46 mm. Former studies have emphasized only on the cathode material showing that high-work-function improve the energy resolution at lower energies. Therfore, we studied the influence of the anode material while keeping the cathode material constant. We used four different materials: Indium, Titanium, Chromium and Gold with work-functions between 4.1 eV and 5.1 eV. The low work-function materials Indium and Titanium achieved the best performance with energy resolutions: 2.0 keV (at 59 keV) and 1.9 keV (at 122 keV) for Titanium; 2.1 keV (at 59 keV) and 2.9 keV (at 122 keV) for Indium. These detectors are very competitive compared with the more expensive ones based on HPB material if one takes the large pixel pitch of 2.46 mm into account. We present a detailed comparison of our detector response with 3-D simulations, from which we determined the mobility-lifetime-products for electrons and holes. Finally, we evaluated the temperature dependency of the detector performance and mobility-lifetime-products, which is important for many applications. With decreasing temperature down to -30C the breakdown voltage increases and the electron mobility-lifetime-product decreases by about 30% over a range from 20C to -30C. This causes the energy resolution to deteriorate, but the concomitantly increasing breakdown voltage makes it possible to increase the applied bias voltage and restore the full performance.Comment: Accepted for publication in Astroparticle Physics, 25 pages, 13 figure

Diffusive Spreading of Chainlike Molecules on Surfaces

We study the diffusion and submonolayer spreading of chainlike molecules on surfaces. Using the fluctuating bond model we extract the collective and tracer diffusion coefficients D_c and D_t with a variety of methods. We show that D_c(theta) has unusual behavior as a function of the coverage theta. It first increases but after a maximum goes to zero as theta go to one. We show that the increase is due to entropic repulsion that leads to steep density profiles for spreading droplets seen in experiments. We also develop an analytic model for D_c(theta) which agrees well with the simulations.Comment: 3 pages, RevTeX, 4 postscript figures, to appear in Phys. Rev. Letters (1996

Non-Arrhenius Behavior of Surface Diffusion Near a Phase Transition Boundary

We study the non-Arrhenius behavior of surface diffusion near the second-order phase transition boundary of an adsorbate layer. In contrast to expectations based on macroscopic thermodynamic effects, we show that this behavior can be related to the average microscopic jump rate which in turn is determined by the waiting-time distribution W(t) of single-particle jumps at short times. At long times, W(t) yields a barrier that corresponds to the rate-limiting step in diffusion. The microscopic information in W(t) should be accessible by STM measurements.Comment: 4 pages, Latex with RevTeX macro

Dynamics and Scaling of 2D Polymers in a Dilute Solution

The breakdown of dynamical scaling for a dilute polymer solution in 2D has been suggested by Shannon and Choy [Phys. Rev. Lett. {\bf 79}, 1455 (1997)]. However, we show here both numerically and analytically that dynamical scaling holds when the finite-size dependence of the relevant dynamical quantities is properly taken into account. We carry out large-scale simulations in 2D for a polymer chain in a good solvent with full hydrodynamic interactions to verify dynamical scaling. This is achieved by novel mesoscopic simulation techniques

Diffusion of gold nanoclusters on graphite

We present a detailed molecular-dynamics study of the diffusion and coalescence of large (249-atom) gold clusters on graphite surfaces. The diffusivity of monoclusters is found to be comparable to that for single adatoms. Likewise, and even more important, cluster dimers are also found to diffuse at a rate which is comparable to that for adatoms and monoclusters. As a consequence, large islands formed by cluster aggregation are also expected to be mobile. Using kinetic Monte Carlo simulations, and assuming a proper scaling law for the dependence on size of the diffusivity of large clusters, we find that islands consisting of as many as 100 monoclusters should exhibit significant mobility. This result has profound implications for the morphology of cluster-assembled materials

Visual pattern recognition as a means to optimising building performance?

Visual pattern recognition as a means to optimising building performance