1,990 research outputs found
Studies for a Photon Collider at the ILC
One option at the International Linear Collider is to convert the electron
beams into high energy photon beams by Compton scattering a few millimetres in
front of the interaction region. Selected physics channels for this option have
been analysed and technical issues have been studied. So far no showstoppers
for this option have been found.Comment: V2: Minor changes, accepted by NI
Probing three-dimensional surface force fields with atomic resolution: Measurement strategies, limitations, and artifact reduction
Noncontact atomic force microscopy (NC-AFM) is being increasingly used to measure the interaction force between an atomically sharp probe tip and surfaces of interest, as a function of the three spatial dimensions, with picometer and piconewton accuracy. Since the results of such measurements may be affected by piezo nonlinearities, thermal and electronic drift, tip asymmetries, and elastic deformation of the tip apex, these effects need to be considered during image interpretation. In this paper, we analyze their impact on the acquired data, compare different methods to record atomic-resolution surface force fields, and determine the approaches that suffer the least from the associated artifacts. The related discussion underscores the idea that since force fields recorded by using NC-AFM always reflect the properties of both the sample and the probe tip, efforts to reduce unwanted effects of the tip on recorded data are indispensable for the extraction of detailed information about the atomicscale properties of the surface. © 2012 Baykara et al
LiCaFeF6 A zero strain cathode material for use in Li ion batteries
A new zero strain LiCaFeF6 cathode material for reversible insertion and extraction of lithium ions is presented. LiCaFeF6 is synthesized by a solid state reaction and processed to a conductive electrode composite via high energy ball milling. In the first cycle, a discharge capacity of 112 mAh g amp; 8315; is achieved in the voltage range from 2.0 V to 4.5 V. The electrochemically active redox couple is Fe3 amp; 8314; Fe2 amp; 8314; as confirmed by Mössbauer spectroscopy and X ray absorption spectroscopy. The compound has a trigonal colquiriite type crystal structure space group . By means of in situ and ex situ XRD as well as X ray absorption fine structure spectroscopy a reversible response to Li uptake release is found. For an uptake of 0.8 mol Li per formula unit only minimal changes occur in the lattice parameters causing a total change in unit cell volume of less than 0.5 . The spatial distribution of cations in the crystal structure as well as the linkage between their corresponding fluorine octahedra is responsible for this very small structural response. With its zero strain behaviour this material is expected to exhibit only negligible mechanical degradation. It may be used as a cathode material in future lithium ion batteries with strongly improved safety and cycle lif
Depth profile analyses of films grown at different temperatures
Cu(In,Ga)Se2films are used as absorber layers in chalcopyrite thin filmsolar
cells. As the gallium concentration in the absorber can be used to control the
band gap, there have been many efforts to vary the gallium concentration in
depth to gain an optimum balance of light absorption, carrier collection, and
recombination at different depths of the absorber film, leading to improved
quantum efficiency. In this study, we investigate the effect of the maximum
substrate temperature during film growth on the depth dependent gallium
concentration. For the in-depth gallium concentration analyses, we use two
techniques, covering complementary depth ranges. Angle dependent soft x-ray
emission spectroscopy provides access to information depths between 20 and 470
nm, which covers the depth range of the space charge region, where most of the
photoexcited carriers are generated. Therefore, this depth range is of
particular interest. To complement this investigation we use secondary neutral
mass spectrometry, which destructively probes the whole thickness of the
absorber (â2âÎŒm). The two methods show increasingly pronounced gallium and
indium gradients with decreasing maximum substrate temperature. The probing of
the complementary depth ranges of the absorbers gives a consistent picture of
the in-depth gallium distribution, which provides a solid basis for a
comprehensive discussion about the effect of a reduced substrate temperature
on the formation of gallium gradients in Cu(In,Ga)Se2 and the device
performance of the corresponding reference solar cells
Electroweak Physics, Experimental Aspects
Collider measurements on electroweak physics are summarised. Although the
precision on some observables is very high, no deviation from the Standard
Model of electroweak interactions is observed. The data allow to set stringent
limits on some models for new physics.Comment: Plenary Talk at the UK Phenomenology Workshop on Collider Physics,
Durham, 199
SUSY Parameter Analysis at TeV and Planck Scales
Coherent analyses at future LHC and LC experiments can be used to explore the
breaking mechanism of supersymmetry and to reconstruct the fundamental theory
at high energies, in particular at the grand unification scale. This will be
exemplified for minimal supergravity.Comment: 7 pages, 3 figures, uses espcrc2.sty (included), Proceedings, Loops
and Legs 2004, Zinnowitz on Usedo
Gallium gradients in chalcopyrite thin films: Depth profile analyses of films grown at different temperatures
The following article appeared in Journal of Applied Physics 110.9 (2011): 093509 and may be found at http://scitation.aip.org/content/aip/journal/jap/110/9/10.1063/1.3656986Cu(In,Ga)Se2 films are used as absorber layers in chalcopyrite thin film solar cells. As the gallium concentration in the absorber can be used to control the band gap, there have been many efforts to vary the gallium concentration in depth to gain an optimum balance of light absorption, carrier collection, and recombination at different depths of the absorber film, leading to improved quantum efficiency. In this study, we investigate the effect of the maximum substrate temperature during film growth on the depth dependent gallium concentration. For the in-depth gallium concentration analyses, we use two techniques, covering complementary depth ranges. Angle dependent soft x-ray emission spectroscopy provides access to information depths between 20 and 470 nm, which covers the depth range of the space charge region, where most of the photoexcited carriers are generated. Therefore, this depth range is of particular interest. To complement this investigation we use secondary neutral mass spectrometry, which destructively probes the whole thickness of the absorber (â2 ”m). The two methods show increasingly pronounced gallium and indium gradients with decreasing maximum substrate temperature. The probing of the complementary depth ranges of the absorbers gives a consistent picture of the in-depth gallium distribution, which provides a solid basis for a comprehensive discussion about the effect of a reduced substrate temperature on the formation of gallium gradients in Cu(In,Ga)Se2 and the device performance of the corresponding reference solar cells.The authors acknowledge the support of the European Commission in the framework of the ATHLET-project (Project No. 019670)
Three-dimensional interaction force and tunneling current spectroscopy of point defects on rutile TiO2(110)
The extent to which point defects affect the local chemical reactivity and electronic properties of an oxide surface was evaluated with picometer resolution in all three spatial dimensions using simultaneous atomic force/scanning tunneling microscopy measurements performed on the (110) face of rutile TiO2. Oxygen atoms were imaged as protrusions in both data channels, corresponding to a rarely observed imaging mode for this prototypical metal oxide surface. Three-dimensional spectroscopy of interaction forces and tunneling currents was performed on individual surface and subsurface defects as a function of tip-sample distance. An interstitial defect assigned to a subsurface hydrogen atom is found to have a distinct effect on the local density of electronic states on the surface, but no detectable influence on the tip-sample interaction force. Meanwhile, spectroscopic data acquired on an oxygen vacancy highlight the role of the probe tip in chemical reactivity measurements. © 2016 AIP Publishing LLC
High-precision measurements from LHC to FCC-ee
This document provides a writeup of all contributions to the workshop on
"High precision measurements of : From LHC to FCC-ee" held at CERN,
Oct. 12--13, 2015. The workshop explored in depth the latest developments on
the determination of the QCD coupling from 15 methods where high
precision measurements are (or will be) available. Those include low-energy
observables: (i) lattice QCD, (ii) pion decay factor, (iii) quarkonia and (iv)
decays, (v) soft parton-to-hadron fragmentation functions, as well as
high-energy observables: (vi) global fits of parton distribution functions,
(vii) hard parton-to-hadron fragmentation functions, (viii) jets in p
DIS and -p photoproduction, (ix) photon structure function in
-, (x) event shapes and (xi) jet cross sections in
collisions, (xii) W boson and (xiii) Z boson decays, and (xiv) jets and (xv)
top-quark cross sections in proton-(anti)proton collisions. The current status
of the theoretical and experimental uncertainties associated to each extraction
method, the improvements expected from LHC data in the coming years, and future
perspectives achievable in collisions at the Future Circular Collider
(FCC-ee) with (1--100 ab) integrated luminosities yielding
10 Z bosons and jets, and 10 W bosons and leptons, are
thoroughly reviewed. The current uncertainty of the (preliminary) 2015 strong
coupling world-average value, = 0.1177 0.0013, is about
1\%. Some participants believed this may be reduced by a factor of three in the
near future by including novel high-precision observables, although this
opinion was not universally shared. At the FCC-ee facility, a factor of ten
reduction in the uncertainty should be possible, mostly thanks to
the huge Z and W data samples available.Comment: 135 pages, 56 figures. CERN-PH-TH-2015-299, CoEPP-MN-15-13. This
document is dedicated to the memory of Guido Altarell
Simultaneous measurement of multiple independent atomic-scale interactions using scanning probe microscopy: Data interpretation and the effect of cross-talk
In high-resolution scanning probe microscopy, it is becoming increasingly common to simultaneously record multiple channels representing different tip-sample interactions to collect complementary information about the sample surface. A popular choice involves simultaneous scanning tunneling microscopy (STM) and noncontact atomic force microscopy (NC-AFM) measurements, which are thought to reflect the chemical and electronic properties of the sample surface. With surface-oxidized Cu(100) as an example, we investigate whether atomic-scale information on chemical interactions can be reliably extracted from frequency shift maps obtained while using the tunneling current as the feedback parameter. Ab initio calculations of interaction forces between specific tip apexes and the surface are utilized to compare experiments with theoretical expectations. The examination reveals that constant-current operation may induce a noticeable influence of topography-feedback-induced cross-talk on the frequency shift data, resulting in misleading interpretations of local chemical interactions on the surface. Consequently, the need to apply methods such as 3D-AFM is emphasized when accurate conclusions about both the local charge density near the Fermi level, as provided by the STM channel, and the site-specific strength of tip-sample interactions (NC-AFM channel) are desired. We conclude by generalizing to the case where multiple atomic-scale interactions are being probed while only one of them is kept constant. © 2015 American Chemical Society
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