209 research outputs found
Quasi one dimensional He inside carbon nanotubes
We report results of diffusion Monte Carlo calculations for both He
absorbed in a narrow single walled carbon nanotube (R = 3.42 \AA) and strictly
one dimensional He. Inside the tube, the binding energy of liquid He is
approximately three times larger than on planar graphite. At low linear
densities, He in a nanotube is an experimental realization of a
one-dimensional quantum fluid. However, when the density increases the
structural and energetic properties of both systems differ. At high density, a
quasi-continuous liquid-solid phase transition is observed in both cases.Comment: 11 pages, 3ps figures, to appear in Phys. Rev. B (RC
Electronic response of aligned multishell carbon nanotubes
We report calculations of the effective electronic response of aligned
multishell carbon nanotubes. A local graphite-like dielectric tensor is
assigned to every point of the multishell tubules, and the effective transverse
dielectric function of the composite is computed by solving Maxwell's
equations. Calculations of both real and imaginary parts of the effective
dielectric function are presented, for various values of the filling fraction
and the ratio of the internal and external radii of hollow tubules. Our full
calculations indicate that the experimentally measured macroscopic dielectric
function of carbon nanotube materials is the result of a strong electromagnetic
coupling between the tubes, which cannot be accounted for with the use of
simplified effective medium theories. The presence of surface plasmons is
investigated, and both optical absorption cross sections and energy-loss
spectra of aligned tubules are calculated.Comment: 4 pages, 4 figures, to appear in Phys. Rev.
The evaluation of shear deformation for contact analysis with large displacement
A common problem encountered in the study of contact problem is the failure to obtain stable and accurate convergence result when the contact node is close to the element edge, which is referred as "critical area". In previous studies, the modification of the element force equation to apply it to a node-element contact problem using the Euler-Bernoulli beam theory [1]. A simple single-element consists two edges and a contact point was used to simulate contact phenomenon of a plane frame. The modification was proven to be effective by the convergeability of the unbalanced force at the tip of element edge, which enabled the contact node to "pass-through", resulting in precise results. However, in another recent study, we discover that, if shear deformation based on Timoshenko beam theory is taken into consideration, a basic simply supported beam coordinate afforded a much simpler and more efficient technique for avoiding the divergence of the unbalanced force in the "critical area". Using our unique and robust Tangent Stiffness Method, the improved equation can be used to overcome any geometrically nonlinear analyses, including those involving extremely large displacements
Electronic and Magnetic Properties of Partially-Open Carbon Nanotubes
On the basis of the spin-polarized density functional theory calculations, we
demonstrate that partially-open carbon nanotubes (CNTs) observed in recent
experiments have rich electronic and magnetic properties which depend on the
degree of the opening. A partially-open armchair CNT is converted from a metal
to a semiconductor, and then to a spin-polarized semiconductor by increasing
the length of the opening on the wall. Spin-polarized states become
increasingly more stable than nonmagnetic states as the length of the opening
is further increased. In addition, external electric fields or chemical
modifications are usable to control the electronic and magnetic properties of
the system. We show that half-metallicity may be achieved and the spin current
may be controlled by external electric fields or by asymmetric
functionalization of the edges of the opening. Our findings suggest that
partially-open CNTs may offer unique opportunities for the future development
of nanoscale electronics and spintronics.Comment: 6 figures, to appear in J. Am. Chem. So
Chirality effects in carbon nanotubes
We consider chirality related effects in optical, photogalvanic and
electron-transport properties of carbon nanotubes. We show that these
properties of chiral nanotubes are determined by terms in the electron
effective Hamiltonian describing the coupling between the electron wavevector
along the tube principal axis and the orbital momentum around the tube
circumference. We develop a theory of photogalvanic effects and a theory of
d.c. electric current, which is linear in the magnetic field and quadratic in
the bias voltage. Moreover, we present analytic estimations for the natural
circular dichroism and magneto-spatial effect in the light absorption.Comment: 23 pages, 3 figure
Realistic description of electron-energy loss spectroscopy for One-Dimensional SrCuO
We investigate the electron-energy loss spectrum of one-dimensional undoped
CuO chains within an extended multi-band Hubbard model and an extended
one-band Hubbard model, using the standard Lanczos algorithm. Short-range
intersite Coulomb interactions are explicitly included in these models, and
long-range interactions are treated in random-phase approximation. The results
for the multi-band model with standard parameter values agree very well with
experimental spectra of SrCuO. In particular, the width of the main
structure is correctly reproduced for all values of momentum transfer. It is
shown for both models that intersite Coulomb interactions mainly lead to an
energy shift of the spectra. We find no evidence for enhanced intersite
interactions in SrCuO.Comment: 4 pages, 4 figure
Results from the Fourth WMO Filter Radiometer Comparison for aerosol optical depth measurements
This study presents the results of the Fourth Filter Radiometer Comparison that was held in Davos, Switzerland, between 28 September and 16 October 2015. Thirty filter radiometers and spectroradiometers from 12 countries participated including reference instruments from global aerosol networks. The absolute differences of all instruments compared to the reference have been based on the World Meteorological Organization (WMO) criterion defined as follows: 95% of the measured data has to be within 0.005±0.001∕m (where m is the air mass). At least 24 out of 29 instruments achieved this goal at both 500 and 865nm, while 12 out of 17 and 13 out of 21 achieved this at 368 and 412nm, respectively. While searching for sources of differences among different instruments, it was found that all individual differences linked to Rayleigh, NO2, ozone, water vapor calculations and related optical depths and air mass calculations were smaller than 0.01 in aerosol optical depth (AOD) at 500 and 865nm. Different cloud-detecting algorithms used have been compared. Ångström exponent calculations showed relatively large differences among different instruments, partly because of the high calculation uncertainty of this parameter in low AOD conditions. The overall low deviations of these AOD results and the high accuracy of reference aerosol network instruments demonstrated a promising framework to achieve homogeneity, compatibility and harmonization among the different spectral AOD networks in the near future
Hypoxic preconditioning potentiates the trophic effects of mesenchymal stem cells on co-cultured human primary hepatocytes
Improved non-covalent biofunctionalization of multi-walled carbon nanotubes using carbohydrate amphiphiles with a butterfly-like polyaromatic tail
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