999 research outputs found
Wither the sliding Luttinger liquid phase in the planar pyrochlore
Using series expansion based on the flow equation method we study the zero
temperature properties of the spin-1/2 planar pyrochlore antiferromagnet in the
limit of strong diagonal coupling. Starting from the limit of decoupled crossed
dimers we analyze the evolution of the ground state energy and the elementary
triplet excitations in terms of two coupling constants describing the inter
dimer exchange. In the limit of weakly coupled spin-1/2 chains we find that the
fully frustrated inter chain coupling is critical, forcing a dimer phase which
adiabatically connects to the state of isolated dimers. This result is
consistent with findings by O. Starykh, A. Furusaki and L. Balents (Phys. Rev.
B 72, 094416 (2005)) which is inconsistent with a two-dimensional sliding
Luttinger liquid phase at finite inter chain coupling.Comment: 6 pages, 4 Postscript figures, 1 tabl
Molecular double core-hole electron spectroscopy for chemical analysis
We explore the potential of double core hole electron spectroscopy for
chemical analysis in terms of x-ray two-photon photoelectron spectroscopy
(XTPPS). The creation of deep single and double core vacancies induces
significant reorganization of valence electrons. The corresponding relaxation
energies and the interatomic relaxation energies are evaluated by CASSCF
calculations. We propose a method how to experimentally extract these
quantities by the measurement of single and double core-hole ionization
potentials (IPs and DIPs). The influence of the chemical environment on these
DIPs is also discussed for states with two holes at the same atomic site and
states with two holes at two different atomic sites. Electron density
difference between the ground and double core-hole states clearly shows the
relaxations accompanying the double core-hole ionization. The effect is also
compared with the sensitivity of single core hole ionization potentials (IPs)
arising in single core hole electron spectroscopy. We have demonstrated the
method for a representative set of small molecules LiF, BeO, BF, CO, N2, C2H2,
C2H4, C2H6, CO2 and N2O. The scalar relativistic effect on IPs and on DIPs are
briefly addressed.Comment: 35 pages, 6 figures. To appear in J. Chem. Phys
Polariton Bose-Einstein condensate at room temperature in a Al(Ga)N nanowire-dielectric microcavity with a spatial potential trap
A spatial potential trap is formed in a 6.0 {\mu}m Al(Ga)N nanowire by
varying the Al composition along its length during epitaxial growth. The
polariton emission characteristics of a dielectric microcavity with the single
nanowire embedded in-plane has been studied at room temperature. Excitation is
provided at the Al(Ga)N end of the nanowire and polariton emission is observed
from the lowest bandgap GaN region of the nanowire. Comparison of the results
with those measured in an identical microcavity with an uniform GaN nanowire
and having an identical exciton-photon detuning suggests evaporative cooling of
the polaritons as they are transported across the trap in the Al(Ga)N nanowire.
Measurement of the spectral characteristics of the polariton emission, their
momentum distribution, first-order spatial coherence and time-resolved
measurements of polariton cooling provide strong evidence of the formation of
an equilibrium Bose-Einstein condensate, a unique state of matter in solid
state systems, in the GaN region of the nanowire, at room temperature. An
equilibrium condensate is not formed in the GaN nanowire dielectric microcavity
without the spatial potential trap.Comment: 28 pages, 6 figures, Submitted to the Proceedings of the National
Academy of Sciences of the United States of Americ
Composition profiling InAs quantum dots and wetting layers by atom probe tomography and cross-sectional scanning tunnelling microscopy
This study compares cross-sectional scanning tunnelling microscopy (XSTM) and
atom probe tomography (APT). We use epitaxially grown self-assembled InAs
quantum dots (QDs) in GaAs as an exemplary material with which to compare these
two nanostructural analysis techniques. We studied the composition of the
wetting layer and the QDs, and performed quantitative comparisons of the indium
concentration profiles measured by each method. We show that computational
models of the wetting layer and the QDs, based on experimental data, are
consistent with both analytical approaches. This establishes a link between the
two techniques and shows their complimentary behaviour, an advantage which we
exploit in order to highlight unique features of the examined QD material.Comment: Main article: 8 pages, 6 figures. Appendix: 3 pages, 5 figure
Breakdown of the Two-Step Model in K-Shell Photoemission and Subsequent Decay Probed by the Molecular-Frame Photoelectron Angular Distributions of CO_2
We report results of measurements and of Hartree-Fock level calculations of molecular-frame photoelectron angular distributions (MFPADs) for C 1s photoemission from CO2. The agreement between the measured and calculated MFPADs is on average reasonable. The measured MFPADs display a weak but definite asymmetry with respect to the O+ and CO+ fragment ions at certain energies, providing evidence for an overlap of gerade and ungerade final ionic states giving rise to a partial breakdown of the two-step model of core-level photoionization and its subsequent Auger decay
Unusual development of light-reflecting pigment cells in intact and regenerating tail in the periodic albino mutant of Xenopus laevis
Unusual light-reflecting pigment cells, âwhite pigment cellsâ, specifically appear in the periodic albino mutant (ap/ap) of Xenopus laevis and localize in the same place where melanophores normally differentiate in the wild-type. The mechanism responsible for the development of unusual pigment cells is unclear. In this study, white pigment cells in the periodic albino were compared with melanophores in the wild-type, using a cell culture system and a tail-regenerating system. Observations of both intact and cultured cells demonstrate that white pigment cells are unique in (1) showing characteristics of melanophore precursors at various stages of development, (2) accumulating reflecting platelets characteristic of iridophores, and (3) exhibiting pigment dispersion in response to α-melanocyte stimulating hormone (α-MSH) in the same way that melanophores do. When a tadpole tail is amputated, a functionally competent new tail is regenerated. White pigment cells appear in the mutant regenerating tail, whereas melanophores differentiate in the wild-type regenerating tail. White pigment cells in the mutant regenerating tail are essentially similar to melanophores in the wild-type regenerating tail with respect to their localization, number, and response to α-MSH. In addition to white pigment cells, iridophores which are never present in the intact tadpole tail appear specifically in the somites near the amputation level in the mutant regenerating tail. Iridophores are distinct from white pigment cells in size, shape, blue light-induced fluorescence, and response to α-MSH. These findings strongly suggest that white pigment cells in the mutant arise from melanophore precursors and accumulate reflecting platelets characteristic of iridophores
Excitonic instability and electric-field-induced phase transition towards a two dimensional exciton condensate
We present an InAs-GaSb-based system in which the electric-field tunability
of its 2D energy gap implies a transition towards a thermodynamically stable
excitonic condensed phase. Detailed calculations show a 3 meV BCS-like gap
appearing in a second-order phase transition with electric field. We find this
transition to be very sharp, solely due to exchange interaction, and so, the
exciton binding energy is greatly renormalized even at small condensate
densities. This density gradually increases with external field, thus enabling
the direct probe of the Bose-Einstein to BCS crossover.Comment: LaTex, 11 pages, 3 ps figures, To appear in PR
Drag in paired electron-hole layers
We investigate transresistance effects in electron-hole double layer systems
with an excitonic condensate. Our theory is based on the use of a minimum
dissipation premise to fix the current carried by the condensate. We find that
the drag resistance jumps discontinuously at the condensation temperature and
diverges as the temperature approaches zero.Comment: 12 pages, 1 Figure, .eps file attache
Dissociative photoionization of the NO molecule studied by photoelectron-photon coincidence technique
Low-energy photoelectronâvacuum ultraviolet (VUV) photon coincidences have been measured using synchrotron radiation excitation in the inner-valence region of the nitric oxide molecule. The capabilities of the coincidence set-up were demonstrated by detecting the 2sâ1 â 2pâ1 radiative transitions in coincidence with the 2s photoelectron emission in Ne. In NO, the observed coincidence events are attributed to dissociative photoionization with excitation, whereby photoelectron emission is followed by fragmentation of excited NO+ ions into O+ + N* or N+ + O* and VUV emission from an excited neutral fragment. The highest coincidence rate occurs with the opening of ionization channels which are due to correlation satellites of the 3Ï photoionization. The decay time of VUV photon emission was also measured, implying that specific excited states of N atoms contribute significantly to observed VUV emission
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