15 research outputs found
Ground-State Candidate for the Dipolar Kagome Ising Antiferromagnet
We have investigated the low-temperature thermodynamic properties of the
dipolar kagome Ising antiferromagnet using at-equilibrium Monte Carlo
simulations, in the quest for the ground-state manifold. In spite of the
limitations of a single spin-flip approach, we managed to identify certain
ordering patterns in the low-temperature regime and we propose a candidate for
this unknown state. This novel configuration presents some intriguing features
and passes several test-criteria, making it a very likely choice for the
dipolar long-range order of this kagome Ising antiferromagnet.Comment: 8 pages, 5 figure
Non-universality of artificial frustrated spin systems
Magnetic frustration effects in artificial kagome arrays of nanomagnets with
out-of-plane magnetization are investigated using Magnetic Force Microscopy and
Monte Carlo simulations. Experimental and theoretical results are compared to
those found for the artificial kagome spin ice, in which the nanomagnets have
in-plane magnetization. In contrast with what has been recently reported, we
demonstrate that long range (i.e. beyond nearest-neighbors) dipolar
interactions between the nanomagnets cannot be neglected when describing the
magnetic configurations observed after demagnetizing the arrays using a field
protocol. As a consequence, there are clear limits to any universality in the
behavior of these two artificial frustrated spin systems. We provide arguments
to explain why these two systems show striking similarities at first sight in
the development of pairwise spin correlations.Comment: 7 pages, 6 figure
Extensive degeneracy, Coulomb phase and magnetic monopoles in an artificial realization of the square ice model
Artificial spin ice systems have been introduced as a possible mean to
investigate frustration effects in a well-controlled manner by fabricating
lithographically-patterned two-dimensional arrangements of interacting magnetic
nanostructures. This approach offers the opportunity to visualize
unconventional states of matter, directly in real space, and triggered a wealth
of studies at the frontier between nanomagnetism, statistical thermodynamics
and condensed matter physics. Despite the strong efforts made these last ten
years to provide an artificial realization of the celebrated square ice model,
no simple geometry based on arrays of nanomagnets succeeded to capture the
macroscopically degenerate ground state manifold of the corresponding model.
Instead, in all works reported so far, square lattices of nanomagnets are
characterized by a magnetically ordered ground state consisting of local
flux-closure configurations with alternating chirality. Here, we show
experimentally and theoretically, that all the characteristics of the square
ice model can be observed if the artificial square lattice is properly
designed. The spin configurations we image after demagnetizing our arrays
reveal unambiguous signatures of an algebraic spin liquid state characterized
by the presence of pinch points in the associated magnetic structure factor.
Local excitations, i.e. classical analogues of magnetic monopoles, are found to
be free to evolve in a massively degenerated, divergence-free vacuum. We thus
provide the first lab-on-chip platform allowing the investigation of collective
phenomena, including Coulomb phases and ice-like physics.Comment: 26 pages, 10 figure
The importance of the weak: Interaction modifiers in artificial spin ices
The modification of geometry and interactions in two-dimensional magnetic
nanosystems has enabled a range of studies addressing the magnetic order,
collective low-energy dynamics, and emergent magnetic properties, in e.g.
artificial spin ice structures. The common denominator of all these
investigations is the use of Ising-like mesospins as building blocks, in the
form of elongated magnetic islands. Here we introduce a new approach: single
interaction modifiers, using slave-mesospins in the form of discs, within which
the mesospin is free to rotate in the disc plane. We show that by placing these
on the vertices of square artificial spin ice arrays and varying their
diameter, it is possible to tailor the strength and the ratio of the
interaction energies. We demonstrate the existence of degenerate ice-rule
obeying states in square artificial spin ice structures, enabling the
exploration of thermal dynamics in a spin liquid manifold. Furthermore, we even
observe the emergence of flux lattices on larger length-scales, when the energy
landscape of the vertices is reversed. The work highlights the potential of a
design strategy for two-dimensional magnetic nano-architectures, through which
mixed dimensionality of mesospins can be used to promote thermally emergent
mesoscale magnetic states.Comment: 17 pages, including methods, 4 figures. Supplementary information
contains 16 pages and 15 figure
Direction‐sensitive magnetophotonic surface crystals
Nanometer-thin rare-earth–transition-metal (RE–TM) alloys with precisely controlled compositions and out-of-plane magnetic anisotropy are currently in the focus for ultrafast magnetophotonic applications. However, achieving lateral nanoscale dimensions, crucial for potential device downscaling, while maintaining designable optomagnetic functionality and out-of-plane magnetic anisotropy is extremely challenging. Herein, nanosized Tb18Co82 ferrimagnetic alloys, having strong out-of-plane magnetic anisotropy, within a gold plasmonic nanoantenna array to design a micrometer-scale magnetophotonic crystal that exhibits abrupt and narrow magneto-optical (MO) spectral features that are both magnetic field and light incidence direction controlled are integrated. The narrow Fano-type resonance arises through the interference of the individual nanoantenna's surface plasmons and a Rayleigh anomaly of the whole nanoantenna array, in both optical and MO spectra, which are demonstrated and explained using Maxwell theory simulations. This robust magnetophotonic crystal opens the way for conceptually new high-resolution light incidence direction sensors, as well as for building blocks for plasmon-assisted all-optical magnetization switching in ferrimagnetic RE–TM alloys
Nanoscale magnetophotonics
This Perspective surveys the state-of-the-art and future prospects of science and technology employing the nanoconfined light (nanophotonics and nanoplasmonics) in combination with magnetism. We denote this field broadly as nanoscale magnetophotonics. We include a general introduction to the field and describe the emerging magneto-optical effects in magnetoplasmonic and magnetophotonic nanostructures as well as their applications in biological and chemical sensing, and in light polarization and phase control. Special attention is given to magnetoplasmonic crystals with transverse magnetization and the associated nanophotonic non-reciprocal effects, and to magneto-optical effects in nanostructures periodic arrays. We further review the area of nonlinear magnetophotonics, the semiconductor spin-plasmonics, and the general principles and applications of opto-magnetism and nano-optical ultrafast control of magnetism and spintronics
Observation of the nonlinear Wood's anomaly on periodic arrays of nickel nanodimers
Linear and nonlinear magnetophotonic properties of periodic arrays of nickel nanodimers are governed by the interplay of the (local) optical response of individual nanoparticles and (nonlocal) diffraction phenomena. The redistribution of light intensity between diffracted beams when a diffraction order onsets or disappears is known as Wood's anomaly. Here, angular and magnetic-field-dependent near-infrared spectroscopic measurements, performed for different optical wavelengths and grating constants, discriminate between the linear and nonlinear excitation mechanisms of Wood's anomalies. In the nonlinear regime, evidenced by the magnetic second-harmonic generation, Wood's anomaly is characterized by an order-of-magnitude larger effect in intensity redistribution between the diffracted beams as compared to the linear case. The nonlinear Wood's anomaly manifests itself also in the nonlinear magnetic contrast highlighting the prospects of nonlinear magnetophotonics
Magnetic and all-optical switching properties of amorphous TbxCo100-x alloys
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