3,607 research outputs found
Exciton fine structure and spin decoherence in monolayers of transition metal dichalcogenides
We study the neutral exciton energy spectrum fine structure and its spin
dephasing in transition metal dichalcogenides such as MoS. The interaction
of the mechanical exciton with its macroscopic longitudinal electric field is
taken into account. The splitting between the longitudinal and transverse
excitons is calculated by means of the both electrodynamical approach and
perturbation theory. This long-range exciton
exchange interaction can induce valley polarization decay. The estimated
exciton spin dephasing time is in the picosecond range, in agreement with
available experimental data.Comment: 5 pages, 3 figure
Carrier and polarization dynamics in monolayer MoS2
In monolayer MoS2 optical transitions across the direct bandgap are governed
by chiral selection rules, allowing optical valley initialization. In time
resolved photoluminescence (PL) experiments we find that both the polarization
and emission dynamics do not change from 4K to 300K within our time resolution.
We measure a high polarization and show that under pulsed excitation the
emission polarization significantly decreases with increasing laser power. We
find a fast exciton emission decay time on the order of 4ps. The absence of a
clear PL polarization decay within our time resolution suggests that the
initially injected polarization dominates the steady state PL polarization. The
observed decrease of the initial polarization with increasing pump photon
energy hints at a possible ultrafast intervalley relaxation beyond the
experimental ps time resolution. By compensating the temperature induced change
in bandgap energy with the excitation laser energy an emission polarization of
40% is recovered at 300K, close to the maximum emission polarization for this
sample at 4K.Comment: 7 pages, 7 figures including supplementary materia
Exciton dynamics in WSe2 bilayers
We investigate exciton dynamics in 2H-WSe2 bilayers in time-resolved
photoluminescence (PL) spectroscopy. Fast PL emission times are recorded for
both the direct exciton with ~ 3 ps and the indirect optical
transition with ~ 25 ps. For temperatures between 4 to 150 K
remains constant. Following polarized laser excitation, we observe
for the direct exciton transition at the K point of the Brillouin zone
efficient optical orientation and alignment during the short emission time
. The evolution of the direct exciton polarization and intensity as a
function of excitation laser energy is monitored in PL excitation (PLE)
experiments.Comment: 4 pages, 3 figure
Exciton states in monolayer MoSe2: impact on interband transitions
We combine linear and non-linear optical spectroscopy at 4K with ab initio
calculations to study the electronic bandstructure of MoSe2 monolayers. In
1-photon photoluminescence excitation (PLE) and reflectivity we measure a
separation between the A- and B-exciton emission of 220 meV. In 2-photon PLE we
detect for the A- and B-exciton the 2p state 180meV above the respective 1s
state. In second harmonic generation (SHG) spectroscopy we record an
enhancement by more than 2 orders of magnitude of the SHG signal at resonances
of the charged exciton and the 1s and 2p neutral A- and B-exciton. Our
post-Density Functional Theory calculations show in the conduction band along
the direction a local minimum that is energetically and in k-space
close to the global minimum at the K-point. This has a potentially strong
impact on the polarization and energy of the excitonic states that govern the
interband transitions and marks an important difference to MoS2 and WSe2
monolayers.Comment: 8 pages, 3 figure
Perception and prediction of simple object interactions
For humans, it is useful to be able to visually detect an object's physical properties. One potentially important source of information is the way the object moves and interacts with other objects in the environment. Here, we use computer simulations of a virtual ball bouncing on a horizontal plane to study the correspondence between our ability to estimate the ball's elasticity and to predict its future path. Three experiments were conducted to address (1) perception of the ball's elasticity, (2) interaction with the ball, and (3) prediction of its trajectory. The results suggest that different strategies and information sources are used for passive perception versus actively predicting future behavior
Delay and distortion of slow light pulses by excitons in ZnO
Light pulses propagating through ZnO undergo distortions caused by both bound
and free excitons. Numerous lines of bound excitons dissect the pulse and
induce slowing of light around them, to the extend dependent on their nature.
Exciton-polariton resonances determine the overall pulse delay and attenuation.
The delay time of the higher-energy edge of a strongly curved light stripe
approaches 1.6 ns at 3.374 eV with a 0.3 mm propagation length. Modelling the
data of cw and time-of-flight spectroscopies has enabled us to determine the
excitonic parameters, inherent for bulk ZnO. We reveal the restrictions on
these parameters induced by the light attenuation, as well as a discrepancy
between the parameters characterizing the surface and internal regions of the
crystal.Comment: 4 pages, 4 figure
Atmospheric parameters and chemical properties of red giants in the CoRoT asteroseismology fields
A precise characterisation of the red giants in the seismology fields of the
CoRoT satellite is a prerequisite for further in-depth seismic modelling.
High-resolution FEROS and HARPS spectra were obtained as part of the
ground-based follow-up campaigns for 19 targets holding great asteroseismic
potential. These data are used to accurately estimate their fundamental
parameters and the abundances of 16 chemical species in a self-consistent
manner. Some powerful probes of mixing are investigated (the Li and CNO
abundances, as well as the carbon isotopic ratio in a few cases). The
information provided by the spectroscopic and seismic data is combined to
provide more accurate physical parameters and abundances. The stars in our
sample follow the general abundance trends as a function of the metallicity
observed in stars of the Galactic disk. After an allowance is made for the
chemical evolution of the interstellar medium, the observational signature of
internal mixing phenomena is revealed through the detection at the stellar
surface of the products of the CN cycle. A contamination by NeNa-cycled
material in the most massive stars is also discussed. With the asteroseismic
constraints, these data will pave the way for a detailed theoretical
investigation of the physical processes responsible for the transport of
chemical elements in evolved, low- and intermediate-mass stars.Comment: Accepted for publication in A&A, 25 pages, 13 colour figures (revised
version after language editing
Dark-bright mixing of interband transitions in symmetric semiconductor quantum dots
In photoluminescence spectra of symmetric [111] grown GaAs/AlGaAs quantum
dots in longitudinal magnetic fields applied along the growth axis we observe
in addition to the expected bright states also nominally dark transitions for
both charged and neutral excitons. We uncover a strongly non-monotonous, sign
changing field dependence of the bright neutral exciton splitting resulting
from the interplay between exchange and Zeeman effects. Our theory shows
quantitatively that these surprising experimental results are due to
magnetic-field-induced \pm 3/2 heavy-hole mixing, an inherent property of
systems with C_3v point-group symmetry.Comment: 5 pages, 3 figure
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