243 research outputs found
Magnetocaloritronic nanomachines
We introduce and study a magnetocaloritronic circuit element based on a
domain wall that can move under applied voltage, magnetic field and temperature
gradient. We draw analogies between the Carnot machines and possible devices
employing such circuit element. We further point out the parallels between the
operational principles of thermoelectric and magnetocaloritronic cooling and
power generation and also introduce a magnetocaloritronic figure of merit. Even
though the magnetocaloritronic figure of merit turns out to be very small for
transition-metal based magnets, we speculate that larger numbers may be
expected in ferromagnetic insulators.Comment: Submitted to "Special issue: Caloritronics" in Solid State
Communication
Measuring Temperature Gradients over Nanometer Length Scales
When a quantum dot is subjected to a thermal gradient, the temperature of
electrons entering the dot can be determined from the dot's thermocurrent if
the conductance spectrum and background temperature are known. We demonstrate
this technique by measuring the temperature difference across a 15 nm quantum
dot embedded in a nanowire. This technique can be used when the dot's energy
states are separated by many kT and will enable future quantitative
investigations of electron-phonon interaction, nonlinear thermoelectric
effects, and the effciency of thermoelectric energy conversion in quantum dots.Comment: 6 pages, 5 figure
Direct Observation of Propagating Gigahertz Coherent Guided Acoustic Phonons in Free Standing Single Copper Nanowires
We report on gigahertz acoustic phonon waveguiding in free-standing single
copper nanowires studied by femtosecond transient reflectivity measurements.
The results are discussed on the basis of the semianalytical resolution of the
Pochhammer and Chree equation. The spreading of the generated Gaussian wave
packet of two different modes is derived analytically and compared with the
observed oscillations of the sample reflectivity. These experiments provide a
unique way to independently obtain geometrical and material characterization.
This direct observation of coherent guided acoustic phonons in a single
nano-object is also the first step toward nanolateral size acoustic transducer
and comprehensive studies of the thermal properties of nanowires
Determining the electronic performance limitations in top-down fabricated Si nanowires with mean widths down to 4 nm
Silicon nanowires have been patterned with mean widths down to 4 nm using top-down lithography and dry etching. Performance-limiting scattering processes have been measured directly which provide new insight into the electronic conduction mechanisms within the nanowires. Results demonstrate a transition from 3-dimensional (3D) to 2D and then 1D as the nanowire mean widths are reduced from 12 to 4 nm. The importance of high quality surface passivation is demonstrated by a lack of significant donor deactivation, resulting in neutral impurity scattering ultimately limiting the electronic performance. The results indicate the important parameters requiring optimization when fabricating nanowires with atomic dimensions
Study of Thermal Properties of Graphene-Based Structures Using the Force Constant Method
The thermal properties of graphene-based materials are theoretically
investigated. The fourth-nearest neighbor force constant method for phonon
properties is used in conjunction with both the Landauer ballistic and the
non-equilibrium Green's function techniques for transport. Ballistic phonon
transport is investigated for different structures including graphene, graphene
antidot lattices, and graphene nanoribbons. We demonstrate that this particular
methodology is suitable for robust and efficient investigation of phonon
transport in graphene-based devices. This methodology is especially useful for
investigations of thermoelectric and heat transport applications.Comment: 23 pages, 9 figures, 1 tabl
Obvious Temperature Difference Along a Pb Cluster-Decorated Carbon Nanowire
Pb nanoclusters were deposited onto a suspended carbon nanowire (CNW), where in situ temperature variable observation was carried out by a transmission electron microscope. The heating temperature was up to 450 °C. Both the melting and evaporation of the Pb nanoparticles on the CNW were retarded when compared to the particles on the support frame. The obvious temperature difference of up to 10 K along the CNW of less than 1 μm was demonstrated. It was attributed to the irradiating dissipation-dependent on the surface area of the decorating Pb particle by calculation
Efficient thermoelectric energy conversion on quasi-localized electron states in diameter modulated nanowires
It is known that the thermoelectric efficiency of nanowires increases when their diameter decreases. Recently, we proposed that increase of the thermoelectric efficiency could be achieved by modulating the diameter of the nanowires. We showed that the electron thermoelectric properties depend strongly on the geometry of the diameter modulation. Moreover, it has been shown by another group that the phonon conductivity decreases in nanowires when they are modulated by dots. Here, the thermoelectric efficiency of diameter modulated nanowires is estimated, in the ballistic regime, by taking into account the electron and phonon transmission properties. It is demonstrated that quasi-localized states can be formed that are prosperous for efficient thermoelectric energy conversion
Numerical study of the thermoelectric power factor in ultra-thin Si nanowires
Low dimensional structures have demonstrated improved thermoelectric (TE)
performance because of a drastic reduction in their thermal conductivity,
{\kappa}l. This has been observed for a variety of materials, even for
traditionally poor thermoelectrics such as silicon. Other than the reduction in
{\kappa}l, further improvements in the TE figure of merit ZT could potentially
originate from the thermoelectric power factor. In this work, we couple the
ballistic (Landauer) and diffusive linearized Boltzmann electron transport
theory to the atomistic sp3d5s*-spin-orbit-coupled tight-binding (TB)
electronic structure model. We calculate the room temperature electrical
conductivity, Seebeck coefficient, and power factor of narrow 1D Si nanowires
(NWs). We describe the numerical formulation of coupling TB to those transport
formalisms, the approximations involved, and explain the differences in the
conclusions obtained from each model. We investigate the effects of cross
section size, transport orientation and confinement orientation, and the
influence of the different scattering mechanisms. We show that such methodology
can provide robust results for structures including thousands of atoms in the
simulation domain and extending to length scales beyond 10nm, and point towards
insightful design directions using the length scale and geometry as a design
degree of freedom. We find that the effect of low dimensionality on the
thermoelectric power factor of Si NWs can be observed at diameters below ~7nm,
and that quantum confinement and different transport orientations offer the
possibility for power factor optimization.Comment: 42 pages, 14 figures; Journal of Computational Electronics, 201
Anomalous Heat Conduction and Anomalous Diffusion in Low Dimensional Nanoscale Systems
Thermal transport is an important energy transfer process in nature. Phonon
is the major energy carrier for heat in semiconductor and dielectric materials.
In analogy to Ohm's law for electrical conductivity, Fourier's law is a
fundamental rule of heat transfer in solids. It states that the thermal
conductivity is independent of sample scale and geometry. Although Fourier's
law has received great success in describing macroscopic thermal transport in
the past two hundreds years, its validity in low dimensional systems is still
an open question. Here we give a brief review of the recent developments in
experimental, theoretical and numerical studies of heat transport in low
dimensional systems, include lattice models, nanowires, nanotubes and
graphenes. We will demonstrate that the phonon transports in low dimensional
systems super-diffusively, which leads to a size dependent thermal
conductivity. In other words, Fourier's law is breakdown in low dimensional
structures
Heat conductance is strongly anisotropic for pristine silicon nanowires
We compute atomistically the heat conductance for ultra-thin pristine silicon
nanowires (SiNWs) with diameters ranging from 1 to 5 nm. The room temperature
thermal conductance is found to be highly anisotropic: wires oriented along the
direction have 50-75% larger conductance than wires oriented along the
and directions. We show that the anisotropies can be qualitatively
understood and reproduced from the bulk phonon band structure. Ab initio
density functional theory (DFT) is used to study the thinnest wires, but
becomes computationally prohibitive for larger diameters, where we instead use
the Tersoff empirical potential model (TEP). For the smallest wires, the
thermal conductances obtained from DFT- and TEP calculations agree within 10%.
The presented results could be relevant for future phonon-engineering of
nanowire devices.Comment: 7 pages, 5 figure
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