593 research outputs found
Measurement of the 187Re({\alpha},n)190Ir reaction cross section at sub-Coulomb energies using the Cologne Clover Counting Setup
Uncertainties in adopted models of particle+nucleus optical-model potentials
directly influence the accuracy in the theoretical predictions of reaction
rates as they are needed for reaction-network calculations in, for instance,
{\gamma}-process nucleosynthesis. The improvement of the {\alpha}+nucleus
optical-model potential is hampered by the lack of experimental data at
astrophysically relevant energies especially for heavier nuclei. Measuring the
Re187({\alpha},n)Ir190 reaction cross section at sub-Coulomb energies extends
the scarce experimental data available in this mass region and helps
understanding the energy dependence of the imaginary part of the
{\alpha}+nucleus optical-model potential at low energies. Applying the
activation method, after the irradiation of natural rhenium targets with
{\alpha}-particle energies of 12.4 to 14.1 MeV, the reaction yield and thus the
reaction cross section were determined via {\gamma}-ray spectroscopy by using
the Cologne Clover Counting Setup and the method of {\gamma}{\gamma}
coincidences. Cross-section values at five energies close to the
astrophysically relevant energy region were measured. Statistical model
calculations revealed discrepancies between the experimental values and
predictions based on widely used {\alpha}+nucleus optical-model potentials.
However, an excellent reproduction of the measured cross-section values could
be achieved from calculations based on the so-called Sauerwein-Rauscher
{\alpha}+nucleus optical-model potential. The results obtained indicate that
the energy dependence of the imaginary part of the {\alpha}+nucleus
optical-model potential can be described by an exponential decrease. Successful
reproductions of measured cross sections at low energies for {\alpha}-induced
reactions in the mass range 141{\leq}A{\leq}187 confirm the global character of
the Sauerwein-Rauscher potential
Principle of Maximum Entropy Applied to Rayleigh-B\'enard Convection
A statistical-mechanical investigation is performed on Rayleigh-B\'enard
convection of a dilute classical gas starting from the Boltzmann equation. We
first present a microscopic derivation of basic hydrodynamic equations and an
expression of entropy appropriate for the convection. This includes an
alternative justification for the Oberbeck-Boussinesq approximation. We then
calculate entropy change through the convective transition choosing mechanical
quantities as independent variables. Above the critical Rayleigh number, the
system is found to evolve from the heat-conducting uniform state towards the
convective roll state with monotonic increase of entropy on the average. Thus,
the principle of maximum entropy proposed for nonequilibrium steady states in a
preceding paper is indeed obeyed in this prototype example. The principle also
provides a natural explanation for the enhancement of the Nusselt number in
convection.Comment: 13 pages, 4 figures; typos corrected; Eq. (66a) corrected to remove a
double counting for ; Figs. 1-4 replace
Electron-phonon interaction in C70
The matrix elements of the deformation potential of C are calculated
by means of a simple, yet accurate solution of the electron-phonon coupling
problem in fullerenes, based on a parametrization of the ground state
electronic density of the system in terms of hybridized orbitals.
The value of the calculated dimensionless total electron-phonon coupling
constant is , an order of magnitude smaller than in
C, consistent with the lack of a superconducting phase transition in
CA fullerite, and in overall agreement with measurements of the
broadening of Raman peaks in CK. We also calculate the photoemission
cross section of C, which is found to display less structure than that
associated with C, in overall agreement with the experimental
findings.Comment: To be published in Phys. Rev.
Renormalization Group Approach to the Coulomb Pseudopotential for C_{60}
A numerical renormalization group technique recently developed by one of us
is used to analyse the Coulomb pseudopotential () in
for a variety of bare potentials. We find a large reduction in due to
intraball screening alone, leading to an interesting non-monotonic dependence
of on the bare interaction strength.
We find that is positive for physically reasonable bare parameters,
but small enough to make the electron-phonon coupling a viable mechanism for
superconductivity in alkali-doped fullerides. We end with some open problems.Comment: 12 pages, latex, 7 figures available from [email protected]
Electron--Vibron Interactions and Berry Phases in Charged Buckminsterfullerene: Part I
A simple model for electron-vibron interactions on charged
buckminsterfullerene C, , is solved both at weak and
strong couplings. We consider a single vibrational multiplet interacting
with electrons. At strong coupling the semiclassical dynamical
Jahn-Teller theory is valid. The Jahn-Teller distortions are unimodal for
=1,2,4,5 electrons, and bimodal for 3 electrons. The distortions are
quantized as rigid body pseudo--rotators which are subject to geometrical Berry
phases. These impose ground state degeneracies and dramatically change zero
point energies. Exact diagonalization shows that the semiclassical level
degeneracies and ordering survive well into the weak coupling regime. At weak
coupling, we discover an enhancement factor of for the pair binding
energies over their classical values. This has potentially important
implications for superconductivity in fullerides, and demonstrates the
shortcoming of Migdal--Eliashberg theory for molecular crystals.Comment: 29 pages (+7 figures, 3 available upon request), LATEX,
report-number: BM515
Raman Scattering Study of Ba-doped C60 with t1g States
Raman spectra are reported for Ba doped fullerides, BaxC60(x=3,4,and 6). The
lowest frequency Hg modes split into five components for Ba4C60 and Ba6C60 even
at room temperature, allowing us a quantitative analysis based on the
electron-phonon couping theory. For the superconducting Ba4C60, the density of
states at the Fermi energy was derived as 7 eV-1, while the total value of
electron-phonon coupling \lambda was found to be 1.0, which is comparable to
that of K3C60. The tangential Ag(2) mode, which is known as a sensitive probe
for the degree of charge transfer on C60 molecule, shows a remarkable shift
depending on the Ba concentration, being roughly consistent with the full
charge transfer from Ba to C60. An effect of hybridization between Ba and C60
\pi orbitals is also discussed.Comment: 15 pages, 6 figures submitted to Phys. Rev. B (December 1,1998
Statistical quality assessment and outlier detection for liquid chromatography-mass spectrometry experiments
<p>Abstract</p> <p>Background</p> <p>Quality assessment methods, that are common place in engineering and industrial production, are not widely spread in large-scale proteomics experiments. But modern technologies such as Multi-Dimensional Liquid Chromatography coupled to Mass Spectrometry (LC-MS) produce large quantities of proteomic data. These data are prone to measurement errors and reproducibility problems such that an automatic quality assessment and control become increasingly important.</p> <p>Results</p> <p>We propose a methodology to assess the quality and reproducibility of data generated in quantitative LC-MS experiments. We introduce quality descriptors that capture different aspects of the quality and reproducibility of LC-MS data sets. Our method is based on the Mahalanobis distance and a robust Principal Component Analysis.</p> <p>Conclusion</p> <p>We evaluate our approach on several data sets of different complexities and show that we are able to precisely detect LC-MS runs of poor signal quality in large-scale studies.</p
Resonance Production and S-wave in at 190 GeV/c
The COMPASS collaboration has collected the currently largest data set on
diffractively produced final states using a negative pion
beam of 190 GeV/c momentum impinging on a stationary proton target. This data
set allows for a systematic partial-wave analysis in 100 bins of three-pion
mass, GeV/c , and in 11 bins of the reduced
four-momentum transfer squared, (GeV/c) . This
two-dimensional analysis offers sensitivity to genuine one-step resonance
production, i.e. the production of a state followed by its decay, as well as to
more complex dynamical effects in nonresonant production. In this paper,
we present detailed studies on selected partial waves with , , , , and . In these waves, we observe
the well-known ground-state mesons as well as a new narrow axial-vector meson
decaying into . In addition, we present the results
of a novel method to extract the amplitude of the subsystem with
in various partial waves from the
data. Evidence is found for correlation of the and
appearing as intermediate isobars in the decay of the known
and .Comment: 96 page
Measurement of the charged-pion polarisability
The COMPASS collaboration at CERN has investigated pion Compton scattering,
, at centre-of-mass energy below 3.5 pion
masses. The process is embedded in the reaction
, which is initiated by
190\,GeV pions impinging on a nickel target. The exchange of quasi-real photons
is selected by isolating the sharp Coulomb peak observed at smallest momentum
transfers, \,(GeV/). From a sample of 63\,000 events the
pion electric polarisability is determined to be $\alpha_\pi\ =\ (\,2.0\ \pm\
0.6_{\mbox{\scriptsize stat}}\ \pm\ 0.7_{\mbox{\scriptsize syst}}\,) \times
10^{-4}\,\mbox{fm}^3\alpha_\pi=-\beta_\pi$, which
relates the electric and magnetic dipole polarisabilities. It is the most
precise measurement of this fundamental low-energy parameter of strong
interaction, that has been addressed since long by various methods with
conflicting outcomes. While this result is in tension with previous dedicated
measurements, it is found in agreement with the expectation from chiral
perturbation theory. An additional measurement replacing pions by muons, for
which the cross-section behavior is unambigiously known, was performed for an
independent estimate of the systematic uncertainty.Comment: Published version: 9 pages, 3 figures, 1 tabl
First Measurement of Chiral Dynamics in \pi^- \gamma -> \pi^- \pi^- \pi^+
The COMPASS collaboration at CERN has investigated the \pi^- \gamma -> \pi^-
\pi^- \pi^+ reaction at center-of-momentum energy below five pion masses,
sqrt(s) < 5 m(\pi), embedded in the Primakoff reaction of 190 GeV pions
impinging on a lead target. Exchange of quasi-real photons is selected by
isolating the sharp Coulomb peak observed at smallest momentum transfers, t' <
0.001 (GeV/c)^2. Using partial-wave analysis techniques, the scattering
intensity of Coulomb production described in terms of chiral dynamics and its
dependence on the 3\pi-invariant mass m(3\pi) = sqrt(s) were extracted. The
absolute cross section was determined in seven bins of with an
overall precision of 20%. At leading order, the result is found to be in good
agreement with the prediction of chiral perturbation theory over the whole
energy range investigated.Comment: 10 pages, 5 figure
- …