240 research outputs found

    Atmospheric processes in a young biomass burning plume - radiation and chemistry

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    Trends and Variability of Surface Solar Radiation in Europe Based On Surface- and Satellite-Based Data Records

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    The incoming solar radiation is the essential climate variable that determines the Earth's energy cycle and climate. As long-term high-quality surface measurements of solar radiation are rare, satellite data are used to derive more information on its spatial pattern and its temporal variability. Recently, the EUMETSAT Satellite Application on Climate Monitoring (CM SAF) has published two satellite-based climate data records: Surface Solar Radiation Data Set-Heliosat, Edition 2 (SARAH-2), and Clouds and Radiation Data Set based on AVHRR (advanced very high resolution radiometer) Satellite Measurements, Edition 2 (CLARA-A2). Both data records provide estimates of surface solar radiation. In this study, these new climate data records are compared to surface measurements in Europe during the period 1983\u20132015. SARAH-2 and CLARA-A2 show a high accuracy compared to ground-based observations (mean absolute deviations of 6.9 and 7.3 W/m2, respectively) highlighting a good agreement considering the temporal behavior and the spatial distribution. The results show an overall brightening period since the 1980s onward (comprised between 1.9 and 2.4 W/m2/decade), with substantial decadal and spatial variability. The strongest brightening is found in eastern Europe in spring. An exception is found for northern and southern Europe, where the trends shown by the station data are not completely reproduced by satellite data, especially in summer in southern Europe. We conclude that the major part of the observed trends in surface solar radiation in Europe is caused by changes in clouds and that remaining differences between the satellite- and the station-based data might be connected to changes in the direct aerosol effect and in snow cover

    The Chisholm firestorm: observed microstructure, precipitation and lightning activity of a pyro-Cb

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    International audienceA fire storm that occured on 28 May 2001 devastated the town of Chisholm, ~150 km north of Edmonton, Alberta, induced a violent fire-invigorated cumulonimbus cloud. This pyro-cumulonimbus (pyro-Cb) had overshooting tops of 2.5?3 km above the tropopause, and injected massive amounts of smoke into the lower stratosphere. Fortunately, this event occurred under good coverage of radar, rain gauge, lightning and satellite measurements, which allowed in-depth documentation of the event. The combination of heat and smoke created a cloud with extremely small drops, which ascended rapidly in violent updrafts. There appeared to be little freezing up to the homogeneous freezing isotherm level of ?38°C. A cloud with such small and short-lived highly supercooled drops is incapable of producing precipitation except for few large graupel and hail, which produced the observed radar echoes and charged the cloud with positive lightning. The small cloud drops froze homogeneously to equally small ice particles, for which there is no mechanism to aggregate into precipitation particles that hence remain in the anvil. The small precipitation efficiency implies that only a small fraction of the smoke is scavenged, so that most of it is exhausted through the anvil to the upper troposphere and lower stratosphere. Comparisons with other cases suggest that a pyro-Cb does not have to be as violent as the Chisholm case to have strongly suppressed precipitation. However, this level of convective vigor is necessary to create the overshooting updraft that injects the smoke into the lower stratosphere

    The Chisholm firestorm: observed microstructure, precipitation and lightning activity of a pyro-cumulonimbus

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    International audienceA fire storm that occurred on 28 May 2001 and devastated the town of Chisholm, ~150 km north of Edmonton, Alberta, induced a violent fire-invigorated cumulonimbus cloud. This pyro-cumulonimbus (pyro-Cb) had overshooting tops of 2.5?3 km above the tropopause, and injected massive amounts of smoke into the lower stratosphere. Fortunately, this event occurred under good coverage of radar, rain gauge, lightning and satellite measurements, which allowed in-depth documentation of the event, and gave us an opportunity to study the cloud top morphology and microstructure, precipitation and cloud electrification of the pyro-Cb. The combination of heat and smoke created a cloud with extremely small drops, which ascended rapidly in violent updrafts. There appeared to be little freezing up to the homogeneous freezing isotherm level of ?38°C. A cloud with such small and short-lived highly supercooled drops is incapable of producing precipitation except for few large graupel and hail, which produced the observed radar echoes and charged the cloud with positive lightning. The small cloud drops froze homogeneously to equally small ice particles, for which there is no mechanism to aggregate into precipitation particles, and which hence remain in the anvil. The lack of significant precipitation implies that only a small fraction of the smoke is scavenged, so that most of it is exhausted through the anvil to the upper troposphere and lower stratosphere. Comparisons with other cases suggest that a pyro-Cb does not have to be as violent as the Chisholm case for precipitation to be strongly suppressed. However, this level of convective vigor is necessary to create the overshooting updraft that injects the smoke into the lower stratosphere

    Evaluating satellite-based diurnal cycles of precipitation in the African tropics

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    Precipitation plays a major role in the energy and water cycles of the earth. Because of its variable nature, consistent observations of global precipitation are challenging. Satellite-based precipitation datasets present an alternative to in situ–based datasets in areas sparsely covered by ground stations. These datasets are a unique tool for model evaluations, but the value of satellite-based precipitation datasets depends on their application and scale. Numerous validation studies considered monthly or daily time scales, while less attention is given to subdaily scales. In this study subdaily satellite-based rainfall data are analyzed in West Africa, a region with strong diurnal variability. Several satellite-based precipitation datasets are validated, including Tropical Rainfall Measuring Mission (TRMM) Multisatellite Precipitation Analysis (TMPA), TRMM 3G68 products, Precipitation Estimation from Remotely Sensed Information Using Artificial Neural Networks (PERSIANN), and Climate Prediction Center (CPC) morphing technique (CMORPH) data. As a reference, highly resolved in situ data from the African Monsoon Multidisciplinary Analysis–Couplage de l’Atmosphere Tropical et du Cycle Hydrologique (AMMA-CATCH) are used. As a result, overall the satellite products capture the diurnal cycles of precipitation and its variability as observed on the ground reasonably well. CMORPH and TMPA data show overall good results. For locally induced convective rainfall in the evening most satellite data show slight delays in peak precipitation of up to 2 h

    An Analysis of the Chemical Processes in the Smoke Plume from a Savanna Fire

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    [1] Photochemistry in young plumes from vegetation fires significantly transforms the initial fire emissions within the first hour after the emissions are injected into the atmosphere. Here we present an investigation of field measurements obtained in a smoke plume from a prescribed savanna fire during the SAFARI 2000 field experiment using a detailed photochemical box-dilution model. The dilution used in the model simulations was constrained by measurements of chemically passive tracers (e.g., CO) near and downwind of the fire. The emissions of the dominant carbonaceous compounds, including oxygenated ones, were taken into account. The field measurements revealed significant production of ozone and acetic acid in the gas phase. The photochemical model simulations also predict ozone production, but significantly less than the measurements. The underestimation of the ozone production in the model simulations is likely caused by shortcomings of our current understanding of ozone photochemistry under the polluted conditions in this young smoke plume. Several potential reasons for this discrepancy are discussed. One possible cause could be the neglect of unmeasured emissions or surface reactions of NO2 with methanol or other hydrocarbons. In contrast to the field measurements, no significant production of acetic acid was simulated by the model. We know of no gas-phase reactions that cause the production of acetic acid on the timescale considered here. Though many processes were well-simulated by the model, there is a need for further research on some key photochemical processes within young plumes from biomass burning and the potential interactions between gas and the particulate phases. These fundamental photochemical processes may also be of importance in other polluted environments

    Satellite-based trends of solar radiation and cloud parameters in Europe

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    Solar radiation is the main driver of the Earth\u2019s climate. Measuring solar radiation and analysing its interaction with clouds are essential for the understanding of the climate system. The EUMETSAT Satellite Application Facility on Climate Monitoring (CM SAF) generates satellite-based, high-quality climate data records, with a focus on the energy balance and water cycle. Here, multiple of these data records are analyzed in a common framework to assess the consistency in trends and spatio-temporal variability of surface solar radiation, top-of-atmosphere reflected solar radiation and cloud fraction. This multi-parameter analysis focuses on Europe and covers the time period from 1992 to 2015. A high correlation between these three variables has been found over Europe. An overall consistency of the climate data records reveals an increase of surface solar radiation and a decrease in top-of-atmosphere reflected radiation. In addition, those trends are confirmed by negative trends in cloud cover. This consistency documents the high quality and stability of the CM SAF climate data records, which are mostly derived independently from each other. The results of this study indicate that one of the main reasons for the positive trend in surface solar radiation since the 1990\u2019s is a decrease in cloud coverage even if an aerosol contribution cannot be completely ruled out

    Modeling of biomass smoke injection into the lower stratosphere by a large forest fire (Part I): reference simulation

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    Wildland fires in boreal regions have the potential to initiate deep convection, so-called pyro-convection, due to their release of sensible heat. Under favorable atmospheric conditions, large fires can result in pyro-convection that transports the emissions into the upper troposphere and the lower stratosphere. Here, we present three-dimensional model simulations of the injection of fire emissions into the lower stratosphere by pyro-convection. These model simulations are constrained and evaluated with observations obtained from the Chisholm fire in Alberta, Canada, in 2001. The active tracer high resolution atmospheric model (ATHAM) is initialized with observations obtained by radiosonde. Information on the fire forcing is obtained from ground-based observations of the mass and moisture of the burned fuel. Based on radar observations, the pyro-convection reached an altitude of about 13 km, well above the tropopause, which was located at about 11.2 km. The model simulation yields a similarly strong convection with an overshoot of the convection above the tropopause. The main outflow from the pyro-convection occurs at about 10.6 km, but a significant fraction (about 8%) of the emitted mass of the smoke aerosol is transported above the tropopause. In contrast to regular convection, the region with maximum updraft velocity in the pyro-convection is located close to the surface above the fire. This results in high updraft velocities &gt;10 m s<sup>&minus;1</sup> at cloud base. The temperature anomaly in the plume decreases rapidly with height from values above 50 K at the fire to about 5 K at about 3000 m above the fire. While the sensible heat released from the fire is responsible for the initiation of convection in the model, the release of latent heat from condensation and freezing dominates the overall energy budget. Emissions of water vapor from the fire do not significantly contribute to the energy budget of the convection
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