312 research outputs found

    Multiobjective Sparse Ensemble Learning by Means of Evolutionary Algorithms

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    The file attached to this record is the author's final peer reviewed version. The Publisher's final version can be found by following the DOI link.Ensemble learning can improve the performance of individual classifiers by combining their decisions. The sparseness of ensemble learning has attracted much attention in recent years. In this paper, a novel multiobjective sparse ensemble learning (MOSEL) model is proposed. Firstly, to describe the ensemble classifiers more precisely the detection error trade-off (DET) curve is taken into consideration. The sparsity ratio (sr) is treated as the third objective to be minimized, in addition to false positive rate (fpr) and false negative rate (fnr) minimization. The MOSEL turns out to be augmented DET (ADET) convex hull maximization problem. Secondly, several evolutionary multiobjective algorithms are exploited to find sparse ensemble classifiers with strong performance. The relationship between the sparsity and the performance of ensemble classifiers on the ADET space is explained. Thirdly, an adaptive MOSEL classifiers selection method is designed to select the most suitable ensemble classifiers for a given dataset. The proposed MOSEL method is applied to well-known MNIST datasets and a real-world remote sensing image change detection problem, and several datasets are used to test the performance of the method on this problem. Experimental results based on both MNIST datasets and remote sensing image change detection show that MOSEL performs significantly better than conventional ensemble learning methods

    Effects of Selfâ Assembled Monolayer Modification of Nickel Oxide Nanoparticles Layer on the Performance and Application of Inverted Perovskite Solar Cells

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    Entirely lowâ temperature solutionâ processed (â ¤100â °C) planar pâ iâ n perovskite solar cells (PSCs) offer great potential for commercialization of rollâ toâ roll fabricated photovoltaic devices. However, the stable inorganic holeâ transporting layer (HTL) in PSCs is usually processed at high temperature (200â 500â °C), which is far beyond the tolerant temperature (â ¤150â °C) of rollâ toâ roll fabrication. In this context, inorganic NiOx nanoparticles (NPs) are an excellent candidate to serve as the HTL in PSCs, owing to their excellent solution processability at room temperature. However, the lowâ temperature processing condition is usually accompanied with defect formation, which deteriorates the film quality and device efficiency to a large extent. To suppress this setback, we used a series of benzoic acid selfassembled monolayers (SAMs) to passivate the surface defects of the NiOx NPs and found that 4â bromobenzoic acid could effectively play the role of the surface passivation. This SAM layer reduces the trapâ assisted recombination, minimizes the energy offset between the NiOx NPs and perovskite, and changes the HTL surface wettability, thus enhancing the perovskite crystallization, resulting in more stable PSCs with enhanced power conversion efficiency (PCE) of 18.4â %, exceeding the control device PCE (15.5â %). Also, we incorporated the aboveâ mentioned SAMs into flexible PSCs (Fâ PSCs) and achieved one of the highest PCE of 16.2â % on a polyethylene terephthalate (PET) substrate with a remarkable powerâ perâ weight of 26.9â Wâ gâ 1. This facile interfacial engineering method offers great potential for the largeâ scale manufacturing and commercialization of PSCs.Engineered layers: Lowâ temperature solutionâ processed NiOx nanoparticle film is usually accompanied with defect formation. Here, we find that 4â bromobenzoic acid can form a selfâ assembled monolayer (SAM) on the NiOx film and effectively tune the interfacial properties, resulting in high perovskite solar cells (PSCs) efficiency. Also, we incorporate the aboveâ mentioned SAM into flexible PSCsPeer Reviewedhttps://deepblue.lib.umich.edu/bitstream/2027.42/138886/1/cssc201701262_am.pdfhttps://deepblue.lib.umich.edu/bitstream/2027.42/138886/2/cssc201701262.pdfhttps://deepblue.lib.umich.edu/bitstream/2027.42/138886/3/cssc201701262-sup-0001-misc_information.pd

    China's post-coal growth

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    Slowing GDP growth, a structural shift away from heavy industry, and more proactive policies on air pollution and clean energy have caused China's coal use to peak. It seems that economic growth has decoupled from growth in coal consumption

    Experimental investigation of kinetic instabilities driven by runaway electrons in the EXL-50 spherical torus

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    In this study, the first observation of high-frequency instabilities driven by runaway electrons has been reported in the EXL-50 spherical torus using a high-frequency magnetic pickup coil. The central frequency of these instabilities is found to be exponentially dependent on the plasma density, similar to the dispersion relation of the whistler wave. The instability frequency displays chirping characteristics consistent with the Berk-Breizman model of beam instability. Theoretically, the excitation threshold of the instability driven by runaway electrons is related to the ratio of the runaway electron density to the background plasma density, and such a relationship is first demonstrated experimentally in this study. The instability can be stabilized by increasing the plasma density, consistent with the wave-particle resonance mechanism. This investigation demonstrates the controlled excitation of chirping instabilities in a tokamak plasma and reveals new features of these instabilities, thereby advancing the understanding of the mechanisms for controlling and mitigating runaway electrons

    Rapid Screening of Complex DNA Samples by Single-Molecule Amplification and Sequencing

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    Microbial cloning makes Sanger sequencing of complex DNA samples possible but is labor intensive. We present a simple, rapid and robust method that enables laboratories without special equipment to perform single-molecule amplicon sequencing, although in a low-throughput manner, from sub-picogram quantities of DNA. The method can also be used for quick quality control of next-generation sequencing libraries, as was demonstrated for a metagenomic sample

    A molecular movie of ultrafast singlet fission

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    Abstract: The complex dynamics of ultrafast photoinduced reactions are governed by their evolution along vibronically coupled potential energy surfaces. It is now often possible to identify such processes, but a detailed depiction of the crucial nuclear degrees of freedom involved typically remains elusive. Here, combining excited-state time-domain Raman spectroscopy and tree-tensor network state simulations, we construct the full 108-atom molecular movie of ultrafast singlet fission in a pentacene dimer, explicitly treating 252 vibrational modes on 5 electronic states. We assign the tuning and coupling modes, quantifying their relative intensities and contributions, and demonstrate how these modes coherently synchronise to drive the reaction. Our combined experimental and theoretical approach reveals the atomic-scale singlet fission mechanism and can be generalized to other ultrafast photoinduced reactions in complex systems. This will enable mechanistic insight on a detailed structural level, with the ultimate aim to rationally design molecules to maximise the efficiency of photoinduced reactions

    Observation of whistler wave instability driven by temperature anisotropy of energetic electrons on EXL-50 spherical torus

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    Electromagnetic modes in the frequency range of 30-120MHz were observed in electron cyclotron wave (ECW) steady state plasmas on the ENN XuanLong-50 (EXL-50) spherical torus. These modes were found to have multiple bands of frequencies proportional to the Alfv\'en velocity. This indicates that the observed mode frequencies satisfy the dispersion relation of whistler waves. In addition, suppression of the whistler waves by the synergistic effect of Lower Hybrid Wave (LHW) and ECW was also observed. This suggests that the whistler waves were driven by temperature anisotropy of energetic electrons. These are the first such observations (not runaway discharge) made in magnetically confined toroidal plasmas and may have important implications for studying wave-particle interactions, RF wave current driver, and runaway electron control in future fusion devices

    The Diploid Genome Sequence of an Individual Human

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    Presented here is a genome sequence of an individual human. It was produced from ∼32 million random DNA fragments, sequenced by Sanger dideoxy technology and assembled into 4,528 scaffolds, comprising 2,810 million bases (Mb) of contiguous sequence with approximately 7.5-fold coverage for any given region. We developed a modified version of the Celera assembler to facilitate the identification and comparison of alternate alleles within this individual diploid genome. Comparison of this genome and the National Center for Biotechnology Information human reference assembly revealed more than 4.1 million DNA variants, encompassing 12.3 Mb. These variants (of which 1,288,319 were novel) included 3,213,401 single nucleotide polymorphisms (SNPs), 53,823 block substitutions (2–206 bp), 292,102 heterozygous insertion/deletion events (indels)(1–571 bp), 559,473 homozygous indels (1–82,711 bp), 90 inversions, as well as numerous segmental duplications and copy number variation regions. Non-SNP DNA variation accounts for 22% of all events identified in the donor, however they involve 74% of all variant bases. This suggests an important role for non-SNP genetic alterations in defining the diploid genome structure. Moreover, 44% of genes were heterozygous for one or more variants. Using a novel haplotype assembly strategy, we were able to span 1.5 Gb of genome sequence in segments >200 kb, providing further precision to the diploid nature of the genome. These data depict a definitive molecular portrait of a diploid human genome that provides a starting point for future genome comparisons and enables an era of individualized genomic information
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