880 research outputs found
Probing the phase diagram of CeRu_2Ge_2 by thermopower at high pressure
The temperature dependence of the thermoelectric power, S(T), and the
electrical resistivity of the magnetically ordered CeRu_2Ge_2 (T_N=8.55 K and
T_C=7.40 K) were measured for pressures p < 16 GPa in the temperature range 1.2
K < T < 300 K. Long-range magnetic order is suppressed at a p_c of
approximately 6.4 GPa. Pressure drives S(T) through a sequence of temperature
dependences, ranging from a behaviour characteristic for magnetically ordered
heavy fermion compounds to a typical behaviour of intermediate-valent systems.
At intermediate pressures a large positive maximum develops above 10 K in S(T).
Its origin is attributed to the Kondo effect and its position is assumed to
reflect the Kondo temperature T_K. The pressure dependence of T_K is discussed
in a revised and extended (T,p) phase diagram of CeRu_2Ge_2.Comment: 7 pages, 6 figure
Probing the extended non-Fermi liquid regimes of MnSi and Fe
Recent studies show that the non-Fermi liquid (NFL) behavior of MnSi and Fe
spans over an unexpectedly broad pressure range, between the critical pressure
p_c and around 2p_c. In order to determine the extension of their NFL regions,
we analyze the evolution of the resistivity rho(T) A(p)T^n at higher pressures.
We find that in MnSi the n=3/2 exponent holds below 4.8 GPa=3 p_c, but it
increases above that pressure. At 7.2 GPa we observe the low temperature Fermi
liquid exponent n=2 whereas for T>1.5 K, n=5/3. Our measurements in Fe show
that the NFL behavior rho T^{5/3} extends at least up to 30.5 GPa, above the
entire superconducting (SC) region. In the studied pressure range, the onset of
the SC transition reduces by a factor 10 down to T_c^onset(30.5 GPa)=0.23 K,
while the A-coefficient diminishes monotonically by around 50%.Comment: 2 pages, 2 figures, Proceedings SCES 200
Calorimetric Investigation of CeRu2Ge2 up to 8 GPa
We have developed a calorimeter able to give a qualitative picture of the
specific heat of a sample under high pressure up to approximately 10 GPa. The
principle of ac-calorimetry was adapted to the conditions in a high pressure
clamp. The performance of this technique was successfully tested with the
measurement of the specific heat of CeRu2Ge2 in the temperature range 1.5
K<T<12 K. The phase diagram of its magnetic phases is consistent with previous
transport measurements.Comment: 5 pages, 4 figure
EPR optical detection of F centre pairs in alkali halides. - I : Pumping cycle kinetics and characteristics of the resonances
The EPR of F centres in the ground and excited states was optically detected in the following alkali halide crystals: NaCl, KF, KCl, KBr, KI, RbBr, and RbI. A decrease of the radiative quantum efficiency of the F centre luminescence was observed when microwave transitions were induced between the spin levels. The mechanism responsible for this effect was an electronic tunnelling through the crystal field potential; the electron in the relaxed excited state of an F centre (F~*) is transferred nonradiatively to another nearby F centre in its ground state (F0), and leads to the momentary formation of an ¿ and an F\u27 centre. Such a process is a function of the total spin of the F~*-F0 pair. The role played by the paired centres was confirmed by measurements at different F centre concentration. Moreover, at high optical excitation pumping rates, the population of the intermediate complexes (F\u27-¿) is large enough to allow an estimation of the rate of the reverse process F\u27 + ¿ \u27¨ F0 + F0
Optical and ESR studies on an IR absorption band in CsI:Na after x-ray irradiation
The nature of the defect giving rise to a near IR absorption band (717 nm)in x-irradiated CaI:Na by measuring its linear dichroism, its magnetic CD and its change due to the resonance microwave was studied. The defect (g|| = 1.96, g\u27Û = 2.23 with axis near 100\u27r) involves a Na+ ion and an excess electron
Signatures of valence fluctuations in CeCu2Si2 under high pressure
Simultaneous resistivity and a.c.-specific heat measurements have been
performed under pressure on single crystalline CeCu2Si2 to over 6 GPa in a
hydrostatic helium pressure medium. A series of anomalies were observed around
the pressure coinciding with a maximum in the superconducting critical
temperature, . These anomalies can be linked with an abrupt change
of the Ce valence, and suggest a second quantum critical point at a pressure
GPa, where critical valence fluctuations provide the
superconducting pairing mechanism, as opposed to spin fluctuations at ambient
pressure. Such a valence instability, and associated superconductivity, is
predicted by an extended Anderson lattice model with Coulomb repulsion between
the conduction and f-electrons. We explain the T-linear resistivity found at
in this picture, while other anomalies found around can be
qualitatively understood using the same model.Comment: Submitted to Phys. Rev.
Exotic superconductivity in the coexistent phase of antiferromagnetism and superconductivity in CeCu2(Si0.98Ge0.02)2: A Cu-NQR study under hydrostatic pressure
We report a pressure () effect on CeCu(SiGe)
where an antiferromagnetic (AFM) order at 0.75 K coexists with
superconductivity below 0.4 K\@. At pressures exceeding
GPa, the AFM order is suppressed, which demonstrates that the sudden emergence
of AFM order due to the Ge doping is ascribed to the intrinsic lattice
expansion. The exotic superconductivity at GPa is found to evolve into
a typical heavy-fermion one with a line-node gap above GPa\@. We
highlight that the anomalous enhancement in nuclear spin-lattice relaxation
rate that follows a = const. behavior well below at =
0 GPa is characterized by the persistence of low-lying magnetic excitations,
which may be inherent to the coexistent state of antiferromagnetism and
superconductivity.Comment: 5 pages with 4 figures embedded in the text. To be published in J.
Phys. Soc. Jp
Superconductivity of epsilon-Fe: complete resistive transition
Last year, iron was reported to become superconducting at temperatures below
2K and pressures between 15 and 30 GPa. The evidence presented was a weak
resistivity drop, suppressed by a magnetic field above 0.2 T, and a small
Meissner signal. However, a compelling demonstration, such as the occurrence of
zero resistance, was lacking. Here we report the measurement of a complete
resistive transition at 22.2 GPa with an onset slightly above 2 K in two very
pure samples of iron, of different origins. The superconductivity appears
unusually sensitive to disorder, developing only when the electronic mean free
path is above a threshold value, while the normal state resistivity is
characteristic of a nearly ferromagnetic metal.Comment: 4 pages, 4 figures. To be published in Physics Letters
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