7,134 research outputs found
Magnetic properties of a metal-organic antiferromagnet on a distorted honeycomb lattice
For temperatures T well above the ordering temperature T*=3.0+-0.2K the
magnetic properties of the metal-organic material Mn[C10H6(OH)(COO)]2x2H20
built from Mn^2+ ions and 3-hydroxy-2-naphthoic anions can be described by a
S=5/2 quantum antiferromagnet on a distorted honeycomb lattice with two
different nearest neighbor exchange couplings J2 \approx 2J1 \approx 1.8K.
Measurements of the magnetization M(H,T) as a function of a uniform external
field H and of the uniform zero field susceptibility \chi(T) are explained
within the framework of a modified spin-wave approach which takes into account
the absence of a spontaneous staggered magnetization at finite temperatures.Comment: 11 pages, 11 figures; more thorough discussion of the dependence of
the correlation length on the uniform magnetic field adde
Magneto-structural properties of the layered quasi-2D triangular-lattice antiferromagnets CsCuClBr for = 0,1,2 and 4
We present a study of the magnetic susceptibility under variable
hydrostatic pressure on single crystals of CsCuClBr. This
includes the border compounds \textit{x} = 0 and 4, known as good realizations
of the distorted triangular-lattice spin-1/2 Heisenberg antiferromagnet, as
well as the isostructural stoichiometric systems CsCuClBr and
CsCuClBr. For the determination of the exchange coupling
constants and , data were fitted by a
model \cite{Schmidt2015}. Its application, validated for the
border compounds, yields a degree of frustration / = 0.47 for
CsCuClBr and / 0.63 - 0.78 for
CsCuClBr, making these systems particular interesting
representatives of this family. From the evolution of the magnetic
susceptibility under pressure up to about 0.4\,GPa, the maximum pressure
applied, two observations were made for all the compounds investigated here.
First, we find that the overall energy scale, given by +
), increases under pressure, whereas the ratio
/ remains unchanged in this pressure range. These experimental
observations are in accordance with the results of DFT calculations performed
for these materials. Secondly, for the magnetoelastic coupling constants,
extraordinarily small values are obtained. We assign these observations to a
structural peculiarity of this class of materials
Photoabsorption on nuclei
We calculate the total photoabsorption cross section on nuclei in the energy
range from 300 MeV to 1 GeV within the framework of a semi-classical phase
space model. Besides medium modifications like Fermi motion and Pauli blocking
we focus on the collision broadening of the involved resonances. The resonance
contributions to the elementary cross section are fixed by fits to partial wave
amplitudes of pion photoproduction. The cross sections for ,
needed for the calculation of collision broadening, are obtained by detailed
balance from a fit to cross sections. We show that a
reasonable collision broadening is not able to explain the experimentally
observed disappearance of the -resonance in the photoabsorption
cross section on nuclei.Comment: 26 pages Latex including 9 postscript figure
Exclusive measurement of coherent eta photoproduction from the deuteron
Coherent photoproduction of eta mesons from the deuteron has been measured
from threshold up to incident photon energies of 750 MeV using the photon
spectrometer TAPS at the tagged photon facility at the Mainz microtron MAMI.
For the first time, differential coherent cross sections have been deduced from
the coincident detection of the eta meson and the recoil deuteron. A missing
energy analysis was used for the suppression of background events so that a
very clean identification of coherent eta-photoproduction was achieved. The
resulting cross sections agree with previous experimental results except for
angles around 90 deg in the photon-deuteron cm-system where they are smaller.
They are compared to various model calculations.Comment: 4 pages, 4 figure
Isotope shift in the dielectronic recombination of three-electron ^{A}Nd^{57+}
Isotope shifts in dielectronic recombination spectra were studied for Li-like
^{A}Nd^{57+} ions with A=142 and A=150. From the displacement of resonance
positions energy shifts \delta E^{142,150}(2s-2p_1/2)= 40.2(3)(6) meV
(stat)(sys)) and \delta E^{142,150}(2s-2p_3/2) = 42.3(12)(20) meV of 2s-2p_j
transitions were deduced. An evaluation of these values within a full QED
treatment yields a change in the mean-square charge radius of ^{142,150}\delta
= -1.36(1)(3) fm^2. The approach is conceptually new and combines the
advantage of a simple atomic structure with high sensitivity to nuclear size.Comment: 10 pages, 3 figures, accepted for publication in Physical Review
Letter
Specific Heat Study of 1D and 2D Excitations in the Layered Frustrated Quantum Antiferromagnets CsCuClBr
We report an experimental and theoretical study of the low-temperature
specific heat and magnetic susceptibility of the layered anisotropic
triangular-lattice spin-1/2 Heisenberg antiferromagnets
CsCuClBr with = 0, 1, 2, and 4. We find that the ratio
of the exchange couplings ranges from 0.32 to , implying a
change (crossover or quantum phase transition) in the materials' magnetic
properties from one-dimensional (1D) behavior for to
two-dimensional (2D) behavior for behavior. For , realized for = 0, 1, and 4, we find a magnetic contribution to the
low-temperature specific heat, , consistent with spinon
excitations in 1D spin-1/2 Heisenberg antiferromagnets. Remarkably, for =
2, where implies a 2D magnatic character, we also observe
. This finding, which contrasts the prediction of made by standard spin-wave theories, shows that Fermi-like
statistics also plays a significant role for the magnetic excitations in
frustrated spin-1/2 2D antiferromagnets
Scaling Behavior of Cyclical Surface Growth
The scaling behavior of cyclical surface growth (e.g. deposition/desorption),
with the number of cycles n, is investigated. The roughness of surfaces grown
by two linear primary processes follows a scaling behavior with asymptotic
exponents inherited from the dominant process while the effective amplitudes
are determined by both. Relevant non-linear effects in the primary processes
may remain so or be rendered irrelevant. Numerical simulations for several
pairs of generic primary processes confirm these conclusions. Experimental
results for the surface roughness during cyclical electrodeposition/dissolution
of silver show a power-law dependence on n, consistent with the scaling
description.Comment: 2 figures adde
High Magnetic Field ESR in the Haldane Spin Chains NENP and NINO
We present electron spin resonance experiments in the one-dimensional
antiferromagnetic S=1 spin chains NENP and NINO in pulsed magnetic fields up to
50T. The measured field dependence of the quantum energy gap for B||b is
analyzed using the exact diagonalization method and the density matrix
renormalization group method (DMRG). A staggered anisotropy term (-1)^i d(S_i^x
S_i^z + S_i^z S_i^x) was considered for the first time in addition to a
staggered field term (-1)^i S_i^x B_st. We show that the spin dynamics in high
magnetic fields strongly depends on the orthorhombic anisotropy E.Comment: 4 pages, RevTeX, 4 figure
Spin-drift transport and its applications
We study the generation of non-equilibrium spin currents in systems with
spatially-inhomogeneous magnetic potentials. For sufficiently high current
densities, the spin polarization can be transported over distances
significantly exceeding the intrinsic spin-diffusion length. This enables
applications that are impossible within the conventional spin-diffusion regime.
Specifically, we propose dc measurement schemes for the carrier spin relaxation
times, and , as well as demonstrate the possibility of spin species
separation by driving current through a region with an inhomogeneous magnetic
potential.Comment: 4 pages, 2 eps figure
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