421 research outputs found
Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project Final Technical Report
This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects')
Impacts from ice-nucleating bacteria on deep convection: implications for the biosphere-atmosphere interaction in climate change
International audienceA cloud modeling framework is described to simulate ice nucleation by biogenic aerosol particles, as represented by airborne ice-nucleation active (INA) bacteria. It includes the empirical parameterization of heterogeneous ice nucleation. The formation of cloud liquid by soluble material coated on such insoluble aerosols is represented and determines their partial removal from deep convective clouds by accretion onto precipitation. Preliminary simulations are performed for a case of deep convection over Oklahoma. If present at high enough concentrations, as might occur in proximity to land sources, INA bacteria are found to influence significantly: â (1) the average numbers and sizes of crystals in the clouds; (2) the horizontal cloud coverage in the free troposphere; and (3) precipitation and incident solar insolation at the surface, which influence rates of bacterial growth. At lower concentrations, the corresponding responses of cloud fields appear much lower or are ambiguous. In nature, the growth rates of INA bacteria on leaves prior to emission into the atmosphere are known to be highly dependent on temperature, precipitation and plant species. Consequently, the open question emerges of whether emissions of such ice-nucleating biogenic particles can then be modified by their own effects on clouds and atmospheric conditions, forming a weak feedback in climate or microclimate systems
Description and evaluation of a secondary organic aerosol and new particle formation scheme within TM5-MP v1.2
We have implemented and evaluated a secondary organic aerosol scheme within the chemistry transport model TM5-MP in this work. In earlier versions of TM5-MP the secondary organic aerosol (SOA) was emitted as Aitken-sized particle mass emulating the condensation. In the current scheme we simulate the formation of secondary organic aerosol from oxidation of isoprene and monoterpenes by ozone and hydroxyl radicals, which produce semi-volatile organic compounds (SVOCs) and extremely low-volatility compounds (EVOCs). Subsequently, SVOCs and ELVOCs can condense on particles. Furthermore, we have introduced a new particle formation mechanism depending on the concentration of ELVOCs. For evaluation purposes, we have simulated the year 2010 with the old and new scheme; we see an increase in simulated production of SOA from 39.9 Tg yr(-1) with the old scheme to 52.5 Tg yr(-1) with the new scheme. For more detailed analysis, the particle mass and number concentrations and their influence on the simulated aerosol optical depth are compared to observations. Phenomenologically, the new particle formation scheme implemented here is able to reproduce the occurrence of observed particle formation events. However, the modelled concentrations of formed particles are clearly lower than in observations, as is the subsequent growth to larger sizes. Com - pared to the old scheme, the new scheme increases the number concentrations across the observation stations while still underestimating the observations. The organic aerosol mass concentrations in the US show a much better seasonal cycle and no clear overestimation of mass concentrations anymore. In Europe the mass concentrations are lowered, leading to a larger underestimation of observations. Aerosol optical depth (AOD) is generally slightly increased except in the northern high latitudes. This brings the simulated annual global mean AOD closer to the observational estimate. However, as the increase is rather uniform, biases tend to be reduced only in regions where the model underestimates the AOD. Furthermore, the correlations with satellite retrievals and ground-based sun-photometer observations of AOD are improved. Although the process-based approach to SOA formation causes a reduction in model performance in some areas, overall the new scheme improves the simulated aerosol fields.Peer reviewe
Basic concepts for convection parameterization in weather forecast and climate models: COST Action ES0905 final report
The research network âBasic Concepts for Convection Parameterization in Weather Forecast and Climate Modelsâ was organized with European funding (COST Action ES0905) for the period of 2010â2014. Its extensive brainstorming suggests how the
subgrid-scale parameterization problem in atmospheric modeling, especially for convection, can be examined and developed from the point of view of a robust theoretical basis. Our main cautions are current emphasis on massive observational data analyses and process studies. The closure and the entrainmentâdetrainment problems are identified as the two highest priorities for convection parameterization under the massâflux formulation. The need for
a drastic change of the current European research culture as concerns policies and funding in order not to further deplete the visions of the European researchers focusing on those basic issues is emphasized
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Improvements to an Empirical Parameterization of Heterogeneous Ice Nucleation and Its Comparison with Observations
A framework for an empirical parameterization (EP) of heterogeneous nucleation of ice crystals by multiple species of aerosol material in clouds was proposed in a 2008 paper by the authors. The present paper reports improvements to specification of a few of its empirical parameters. These include temperatures for onset of freezing, baseline surface areas of aerosol observed in field campaigns over Colorado, and new parameters for properties of black carbon, such as surface hydrophilicity and organic coatings. The EP's third group of ice nucleus (IN) aerosols is redefined as that of primary biological aerosol particles (PBAPs), replacing insoluble organic aerosols. A fourth group of IN is introduced-namely, soluble organic aerosols.
The new EP predicts IN concentrations that agree well with aircraft data from selected traverses of shallow wave clouds observed in five flights (1, 3, 4, 6, and 12) of the 2007 Ice in Clouds Experiment Layer Clouds (ICE-L). Selected traverses were confined to temperatures between about -25 degrees and -29 degrees C in layer cloud without homogeneously nucleated ice from aloft. Some of the wave clouds were affected by carbonaceous aerosols from biomass burning and by dust from dry lakebeds and elsewhere. The EP predicts a trend between number concentrations of heterogeneously nucleated ice crystals and apparent black carbon among the five wave clouds, observed by aircraft in ICE-L. It is predicted in terms of IN activity of black carbon.
The EP's predictions are consistent with laboratory and field observations not used in its construction, for black carbon, dust, primary biological aerosols, and soluble organics. The EP's prediction of biological ice nucleation is validated using coincident field observations of PBAP IN and PBAPs in Colorado.Keywords: Ice particles, Ice crystals, Aerosol
The dependence of aerosol effects on clouds and precipitation on cloudâsystem organization, shear and stability
Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/95546/1/jgrd14296.pd
What drives the 'August effect'?: an observational study of the effect of junior doctor changeover on out of hours work
Objective: To investigate whether measurements of junior doctor on-call workload and performance can clarify the mechanisms underlying the increase in morbidity and mortality seen after junior doctor changeover: the âAugust effectâ.
Design: Quantitative retrospective observational study of routinely collected data on junior doctor workload.
Setting: Two large teaching hospitals in England.
Participants: Task level data from a wireless out of hours system (nâ=â29,885 requests) used by medical staff, nurses, and allied health professionals.
Main outcome measures: Number and type of tasks requested by nurses, time to completion of tasks by junior doctors.
Results: There was no overall change in the number of tasks requested by nurses out of hours around the August changeover (median requests per hour 15 before and 14 after, pâ=â0.46). However, the number of tasks classified as urgent was greater (pâ=â0.016) equating to five more urgent tasks per day. After changeover, doctors took less time to complete tasks overall due to a reduction in time taken for routine tasks (median 74 vs. 66âmin; pâ=â3.9âĂâ10â9).
Conclusion: This study suggests that the âAugust effectâ is not due to new junior doctors completing tasks more slowly or having a greater workload. Further studies are required to investigate the causes of the increased number of urgent tasks seen, but likely factors are errors, omissions, and poor prioritization. Thus, improved training and quality control has the potential to address this increased duration of unresolved patient risk. The study also highlights the potential of newer technologies to facilitate quantitative study of clinical activity
Understanding perceptions on 'Buruli' in northwestern Uganda: A biosocial investigation.
BACKGROUND: An understudied disease, little research thus far has explored responses to Buruli ulcer and quests for therapy from biosocial perspective, despite reports that people seek biomedical treatment too late. METHODS AND FINDINGS: Taking an inductive approach and drawing on long-term ethnographic fieldwork in 2013-14, this article presents perspectives on this affliction of people living and working along the River Nile in northwest Uganda. Little is known biomedically about its presence, yet 'Buruli', as it is known locally, was and is a significant affliction in this region. Establishing a biosocial history of 'Buruli', largely obscured from biomedical perspectives, offers explanations for contemporary understandings, perceptions and practices. CONCLUSIONS/SIGNIFICANCE: We must move beyond over-simplifying and problematising 'late presentation for treatment' in public health, rather, develop biosocial approaches to understanding quests for therapy that take into account historical and contemporary contexts of health, healing and illness. Seeking to understand the context in which healthcare decisions are made, a biosocial approach enables greater depth and breadth of insight into the complexities of global and local public health priorities such as Buruli ulcer
Type Ia Supernovae and Cosmology
I discuss the use of Type Ia supernovae (SNe Ia) for cosmological distance
determinations. Low-redshift SNe Ia (z < 0.1) demonstrate that the Hubble
expansion is linear with H_0 = 72 +/- 8 km/s/Mpc, and that the properties of
dust in other galaxies are generally similar to those of dust in the Milky Way.
The measured luminosity distances of SNe Ia as a function of redshift have
shown that the expansion of the Universe is currently accelerating, probably
due to the presence of repulsive dark energy such as Einstein's cosmological
constant (Lambda). From about 200 SNe Ia, we find that Omega_Lambda - 1.4
Omega_M = 0.35 +/- 0.14. Combining our data with other results, we find a best
fit for Omega_M and Omega_Lambda of 0.28 and 0.72, respectively. A number of
possible systematic effects (dust, supernova evolution) thus far do not seem to
eliminate the need for Omega_Lambda > 0. Recently, analyses of SNe Ia at z =
1.0-1.7 provide further support for current acceleration, and give tentative
evidence for an early epoch of deceleration. The dynamical age of the Universe
is estimated to be 13.1 +/- 1.5 Gyr. According to the most recent data sets,
the SN Ia rate at z > 1 is several times greater than that at low redshifts,
presumably because of higher star formation rates long ago. Moreover, the
typical delay time from progenitor star formation to SNIa explosion appears to
be substantial, ~3 Gyr. Current projects include the measurement of a few
hundred SNe Ia at z = 0.2-0.8 to more accurately determine the
equation-of-state parameter of the dark energy, w = P/(\rho c^2), whose value
is now constrained by SNe Ia to be in the range -1.48 < w < -0.72 at 95%
confidence.Comment: 39 pages, 17 figures, to be published in "White Dwarfs: Probes of
Galactic Structure and Cosmology" ed. E. M. Sion, H. L. Shipman, and S.
Vennes (Kluwer: Dordrecht). Part of the Astrophysics and Space Science
Library Serie
Magnetism, FeS colloids, and Origins of Life
A number of features of living systems: reversible interactions and weak
bonds underlying motor-dynamics; gel-sol transitions; cellular connected
fractal organization; asymmetry in interactions and organization; quantum
coherent phenomena; to name some, can have a natural accounting via
interactions, which we therefore seek to incorporate by expanding the horizons
of `chemistry-only' approaches to the origins of life. It is suggested that the
magnetic 'face' of the minerals from the inorganic world, recognized to have
played a pivotal role in initiating Life, may throw light on some of these
issues. A magnetic environment in the form of rocks in the Hadean Ocean could
have enabled the accretion and therefore an ordered confinement of
super-paramagnetic colloids within a structured phase. A moderate H-field can
help magnetic nano-particles to not only overcome thermal fluctuations but also
harness them. Such controlled dynamics brings in the possibility of accessing
quantum effects, which together with frustrations in magnetic ordering and
hysteresis (a natural mechanism for a primitive memory) could throw light on
the birth of biological information which, as Abel argues, requires a
combination of order and complexity. This scenario gains strength from
observations of scale-free framboidal forms of the greigite mineral, with a
magnetic basis of assembly. And greigite's metabolic potential plays a key role
in the mound scenario of Russell and coworkers-an expansion of which is
suggested for including magnetism.Comment: 42 pages, 5 figures, to be published in A.R. Memorial volume, Ed
Krishnaswami Alladi, Springer 201
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