165 research outputs found
Kink far below the Fermi level reveals new electron-magnon scattering channel in Fe
Many properties of real materials can be modeled using ab initio methods
within a single-particle picture. However, for an accurate theoretical
treatment of excited states, it is necessary to describe electron-electron
correlations including interactions with bosons: phonons, plasmons, or magnons.
In this work, by comparing spin- and momentum-resolved photoemission
spectroscopy measurements to many-body calculations carried out with a newly
developed first-principles method, we show that a kink in the electronic band
dispersion of a ferromagnetic material can occur at much deeper binding
energies than expected (E_b=1.5 eV). We demonstrate that the observed spectral
signature reflects the formation of a many-body state that includes a photohole
bound to a coherent superposition of renormalized spin-flip excitations. The
existence of such a many-body state sheds new light on the physics of the
electron-magnon interaction which is essential in fields such as spintronics
and Fe-based superconductivity.Comment: 6 pages, 2 figure
Classifying the wandering mind : Revealing the affective content of thoughts during task-free rest periods
Many powerful human emotional thoughts are generated in the absence of a precipitating event in the environment. Here, we tested whether we can decode the valence of internally driven, self-generated thoughts during task-free rest based on neural similarities with task-related affective mental states. We acquired functional magnetic resonance imaging (fMRI) data while participants generated positive and negative thoughts as part of an attribution task (Session A) and while they reported the occurrence of comparable mental states during task-free rest periods (Session B). With the use of multivariate pattern analyses (MVPA), we identified response patterns in the medial orbitofrontal cortex (mOFC) that encode the affective content of thoughts that are generated in response to an external experimental cue. Importantly, these task driven response patterns reliably predicted the occurrence of affective thoughts generated during unconstrained rest periods recorded one week apart. This demonstrates that at least certain elements of task-cued and task-free affective experiences rely on a common neural code. Furthermore, our findings reveal the role that the mOFC plays in determining the affective tone of unconstrained thoughts. More generally, our results suggest that MVPA is an important methodological tool for attempts to understand unguided subject driven mental states such as mind-wandering and daydreaming based on neural similarities with task-based experiences
Time- and momentum-resolved photoemission studies using time-of-ïŹight momentum microscopy at a free-electron laser
Time-resolved photoemission with ultrafast pump and probe pulses is an emerging technique with wide application potential. Real-time recording of nonequilibrium electronic processes, transient states in chemical reactions, or the interplay of electronic and structural dynamics offers fascinating opportunities for future research. Combining valence-band and core-level spectroscopy with photoelectron diffraction for electronic, chemical, and structural analyses requires few 10 fs soft X-ray pulses with some 10 meV spectral resolution, which are currently available at high repetition rate free-electron lasers. We have constructed and optimized a versatile setup commissioned at FLASH/PG2 that combines free-electron laser capabilities together with a multidimensional recording scheme for photoemission studies. We use a full-field imaging momentum microscope with time-of-flight energy recording as the detector for mapping of 3D band structures in (kx, ky, E) parameter space with unprecedented efficiency. Our instrument can image full surface Brillouin zones with up to 7 Ă
â1 diameter in a binding-energy range of several eV, resolving about 2.5 Ă 105 data voxels simultaneously. Using the ultrafast excited state dynamics in the van der Waals semiconductor WSe2 measured at photon energies of 36.5 eV and 109.5 eV, we demonstrate an experimental energy resolution of 130 meV, a momentum resolution of 0.06 Ă
â1, and a system response function of 150 fs
Quasicrystals and their approximants in 2D ternary oxides
2D oxide quasicrystals (OQCs) are recently discovered aperiodic, but well-ordered oxide interfaces. In this topical review, an introduction to these new thin-film systems is given. The concept of quasicrystals and their approximants is explained for BaTiO3 - and SrTiO3 - derived OQCs and related periodic structures in these 2D oxides. In situ microscopy unravels the high-temperature formation process of OQCs on Pt(111). The dodecagonal structure is discussed regarding tiling statistics and tiling decoration based on the results of atomically resolved scanning tunneling microscopy and various diffraction techniques. In addition, angle-resolved ultraviolet photoemission spectroscopy and X-ray photoelectron spectroscopy results prove a metallic character of the 2D oxide
Atomic structure and properties of magnetic adsorbates on the topological insulator Bi2Se
Resumen del trabajo presentado al Moscow International Symposium on Magnetism (MISM), celebrado en MoscĂș (Rusia) del 29 de junio al 3 de julio de 2014.Support by DFG through SPP1666 is acknowledged.Peer reviewe
Spin texture of time reversal symmetry invariant surface states on W 110
We find in the case of W 110 previously overlooked anomalous surface states having their spin locked at right angle to their momentum using spin resolved momentum microscopy. In addition to the well known Dirac like surface state with Rashba spin texture near the point, we observe a tilted Dirac cone with circularly shaped cross section and a Dirac crossing at 0.28 amp; 8201; amp; 8201; amp; 8201; within the projected bulk band gap of tungsten. This state has eye catching similarities to the spin locked surface state of a topological insulator. The experiments are fortified by a one step photoemission calculation in its density matrix formulatio
Selective C-Rel Activation via Malt1 Controls Anti-Fungal TH-17 Immunity by Dectin-1 and Dectin-2
C-type lectins dectin-1 and dectin-2 on dendritic cells elicit protective immunity against fungal infections through induction of TH1 and TH-17 cellular responses. Fungal recognition by dectin-1 on human dendritic cells engages the CARD9-Bcl10-Malt1 module to activate NF-ÎșB. Here we demonstrate that Malt1 recruitment is pivotal to TH-17 immunity by selective activation of NF-ÎșB subunit c-Rel, which induces expression of TH-17-polarizing cytokines IL-1ÎČ and IL-23p19. Malt1 inhibition abrogates c-Rel activation and TH-17 immunity to Candida species. We found that Malt1-mediated activation of c-Rel is similarly essential to induction of TH-17-polarizing cytokines by dectin-2. Whereas dectin-1 activates all NF-ÎșB subunits, dectin-2 selectively activates c-Rel, signifying a specialized TH-17-enhancing function for dectin-2 in anti-fungal immunity by human dendritic cells. Thus, dectin-1 and dectin-2 control adaptive TH-17 immunity to fungi via Malt1-dependent activation of c-Rel
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