Parametric frequency mixing in the magneto-elastically driven FMR-oscillator

We demonstrate the nonlinear frequency conversion of ferromagnetic resonance (FMR) frequency by optically excited elastic waves in a thin metallic film on dielectric substrates. Time-resolved probing of the magnetization directly witnesses magneto-elastically driven second harmonic generation, sum- and difference frequency mixing from two distinct frequencies, as well as parametric downconversion of each individual drive frequency. Starting from the Landau-Lifshitz-Gilbert equations, we derive an analytical equation of an elastically driven nonlinear parametric oscillator and show that frequency mixing is dominated by the parametric modulation of FMR frequency

Magneto-optical properties of Au upon the injection of hot spin-polarized electrons across Fe/Au(001) interfaces

We demonstrate a novel method for the excitation of sizable magneto-optical effects in Au by means of the laser-induced injection of hot spin-polarized electrons in Au/Fe/MgO(001) heterostructures. It is based on the energy- and spin-dependent electron transmittance of Fe/Au interface which acts as a spin filter for non-thermalized electrons optically excited in Fe. We show that after crossing the interface, majority electrons propagate through the Au layer with the velocity on the order of 1 nm/fs (close to the Fermi velocity) and the decay length on the order of 100 nm. Featuring ultrafast functionality and requiring no strong external magnetic fields, spin injection results in a distinct magneto-optical response of Au. We develop a formalism based on the phase of the transient complex MOKE response and demonstrate its robustness in a plethora of experimental and theoretical MOKE studies on Au, including our ab initio calculations. Our work introduces a flexible tool to manipulate magneto-optical properties of metals on the femtosecond timescale that holds high potential for active magneto-photonics, plasmonics, and spintronics

The effect of the complex processing of Microalgae Chlorella vulgaris on the intensification of the lipid extraction process

Microalgae are considered a promising source of lipids. However, the existing technologies of their extraction necessitate a massive improvement. In the course of the study optimal parameters of microwave radiation and of enzyme mixture "Cellolux A" and "Protosubtilin G3x" were experimentally selected and theoretically proved so as to allow increasing the yield of lipids 5.75 times to 23 % in comparison with the control sample (5 %). Moreover, the ratio and type of polar and non-polar solvents in the extraction stage for the maximum extraction of lipids was determined taking into account the necessity to process protein-lipid complexes

Femtosecond nonlinear ultrasonics in gold probed with ultrashort surface plasmons

Fundamental interactions induced by lattice vibrations on ultrafast time scales become increasingly important for modern nanoscience and technology. Experimental access to the physical properties of acoustic phonons in the THz frequency range and over the entire Brillouin zone is crucial for understanding electric and thermal transport in solids and their compounds. Here, we report on the generation and nonlinear propagation of giant (1 percent) acoustic strain pulses in hybrid gold/cobalt bilayer structures probed with ultrafast surface plasmon interferometry. This new technique allows for unambiguous characterization of arbitrary ultrafast acoustic transients. The giant acoustic pulses experience substantial nonlinear reshaping already after a propagation distance of 100 nm in a crystalline gold layer. Excellent agreement with the Korteveg-de Vries model points to future quantitative nonlinear femtosecond THz-ultrasonics at the nano-scale in metals at room temperature

Anatomy of ultrafast quantitative magneto-acoustics in freestanding nickel thin films

We revisit the quantitative analysis of the ultrafast magneto-acoustic experiment in a freestanding nickel thin film by Kim and Bigot [1] by applying our recently proposed approach of magnetic and acoustic eigenmodes decomposition by Vernik et al. [2]. We show that the application of our modeling to the analysis of time-resolved reflectivity measurements allows for the determination of amplitudes and lifetimes of standing perpendicular acoustic phonon resonances with unprecedented accuracy. The acoustic damping is found to scale as $\propto\omega^2$ for frequencies up to 80~GHz and the peak amplitudes reach $10^{-3}$. The experimentally measured magnetization dynamics for different orientations of an external magnetic field agrees well with numerical solutions of magneto-elastically driven magnon harmonic oscillators. Symmetry-based selection rules for magnon-phonon interactions predicted by our modeling approach allow for the unambiguous discrimination between spatially uniform and non-uniform modes, as confirmed by comparing the resonantly enhanced magneto-elastic dynamics simultaneously measured on opposite sides of the film. Moreover, the separation of time scales for (early) rising and (late) decreasing precession amplitudes provide access to magnetic (Gilbert) and acoustic damping parameters in a single measurement.Comment: 9 pages, 7 figure

Magnetoplasmonic design rules for active magneto-optics

Light polarization rotators and non-reciprocal optical isolators are essential building blocks in photonics technology. These macroscopic passive devices are commonly based on magneto-optical Faraday and Kerr polarization rotation. Magnetoplasmonics - the combination of magnetism and plasmonics - is a promising route to bring these devices to the nanoscale. We introduce design rules for highly tunable active magnetoplasmonic elements in which we can tailor the amplitude and sign of the Kerr response over a broad spectral range

Terahertz spectroscopy for all-optical spintronic characterization of the spin-Hall-effect metals Pt, W and Cu80Ir20

Identifying materials with an efficient spin-to-charge conversion is crucial for future spintronic applications. In this respect, the spin Hall effect is a central mechanism as it allows for the interconversion of spin and charge currents. Spintronic material research aims at maximizing its efficiency, quantified by the spin Hall angle and the spin-current relaxation length . We develop an all-optical contact-free method with large sample throughput that allows us to extract and . Employing terahertz spectroscopy and an analytical model, magnetic metallic heterostructures involving Pt, W and Cu80Ir20 are characterized in terms of their optical and spintronic properties. The validity of our analytical model is confirmed by the good agreement with literature DC values. For the samples considered here, we find indications that the interface plays a minor role for the spin-current transmission. Our findings establish terahertz emission spectroscopy as a reliable tool complementing the spintronics workbench

Resonant phonon-magnon interactions in free-standing metal-ferromagnet multilayer structures

We analyze resonant magneto-elastic interactions between standing perpendicular spin wave modes (exchange magnons) and longitudinal acoustic phonon modes in free-standing hybrid metal-ferromagnet bilayer and trilayer structures. Whereas the ferromagnetic layer acts as a magnetic cavity, all metal layers control the frequencies and eigenmodes of acoustic vibrations. The here proposed design allows for achieving and tuning the spectral and spatial modes overlap between phonons and magnons that results in their strong resonant interaction. Realistic simulations for gold-nickel multilayers show that sweeping the external magnetic field should allow for observing resonantly enhanced interactions between individual magnon and phonon modes in a broad range of frequencies spanning from tens of GHz up to several hundreds of GHz, which can be finely tuned through the multilayer design. Our results would enable the systematic study and the deep understanding of resonantly enhanced magneto-elastic coupling between individual phonon and magnon modes up to frequencies of great contemporary fundamental and applied interest.Comment: 9 pages, 6 figure