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Improving LMOF luminescence quantum yield through guest-mediated rigidification
Rotation of a specific pyridyl ring in LMOF-236 is locked by loading guest molecules into the MOF's pore, improving quantum yield by nearly 400%βan example of a generalizable strategy for maximizing quantum yield via guest-packing rigidification
Localized exciton-polariton modes in dye-doped nanospheres: a quantum approach
We model a dye-doped polymeric nanosphere as an ensemble of quantum emitters
and use it to investigate the localized exciton-polaritons supported by such a
nanosphere. By determining the time evolution of the density matrix of the
collective system, we explore how an incident laser field may cause transient
optical field enhancement close to the surface of such nanoparticles. Our
results provide further evidence that excitonic materials can be used to good
effect in nanophotonics.Comment: 16 pages, 4 figure
Chemical and forensic analysis of JFK assassination bullet lots: Is a second shooter possible?
The assassination of President John Fitzgerald Kennedy (JFK) traumatized the
nation. In this paper we show that evidence used to rule out a second assassin
is fundamentally flawed. This paper discusses new compositional analyses of
bullets reportedly to have been derived from the same batch as those used in
the assassination. The new analyses show that the bullet fragments involved in
the assassination are not nearly as rare as previously reported. In particular,
the new test results are compared to key bullet composition testimony presented
before the House Select Committee on Assassinations (HSCA). Matches of bullets
within the same box of bullets are shown to be much more likely than indicated
in the House Select Committee on Assassinations' testimony. Additionally, we
show that one of the ten test bullets is considered a match to one or more
assassination fragments. This finding means that the bullet fragments from the
assassination that match could have come from three or more separate bullets.
Finally, this paper presents a case for reanalyzing the assassination bullet
fragments and conducting the necessary supporting scientific studies. These
analyses will shed light on whether the five bullet fragments constitute three
or more separate bullets. If the assassination fragments are derived from three
or more separate bullets, then a second assassin is likely, as the additional
bullet would not easily be attributable to the main suspect, Mr. Oswald, under
widely accepted shooting scenarios [see Posner (1993), Case Closed, Bantam, New
York].Comment: Published in at http://dx.doi.org/10.1214/07-AOAS119 the Annals of
Applied Statistics (http://www.imstat.org/aoas/) by the Institute of
Mathematical Statistics (http://www.imstat.org
Quantum metrology beyond the classical limit under the effect of dephasing
Quantum sensors have the potential to outperform their classical
counterparts. For classical sensing, the uncertainty of the estimation of the
target fields scales inversely with the square root of the measurement time T.
On the other hand, by using quantum resources, we can reduce this scaling of
the uncertainty with time to 1/T. However, as quantum states are susceptible to
dephasing, it has not been clear whether we can achieve sensitivities with a
scaling of 1/T for a measurement time longer than the coherence time. Here, we
propose a scheme that estimates the amplitude of globally applied fields with
the uncertainty of 1/T for an arbitrary time scale under the effect of
dephasing. We use one-way quantum computing based teleportation between qubits
to prevent any increase in the correlation between the quantum state and its
local environment from building up and have shown that such a teleportation
protocol can suppress the local dephasing while the information from the target
fields keeps growing. Our method has the potential to realize a quantum sensor
with a sensitivity far beyond that of any classical sensor
Quantifying the impact and relevance of scientific research
Qualitative and quantitative methods are being developed to measure the impacts of research on society, but they suffer
from serious drawbacks associated with linking a piece of research to its subsequent impacts. We have developed a method to derive impact scores for individual research publications according to their contribution to answering questions of quantified importance to end users of research. To demonstrate the approach, here we evaluate the impacts of research into means of conserving wild bee populations in the UK. For published papers, there is a weak positive correlation between our impact score and the impact factor of the journal. The process identifies publications that provide high quality evidence relating to issues of strong concern. It can also be used to set future research agendas
The Histone 3'-Terminal Stem-Loop-Binding Protein Enhances Translation through a Functional and Physical Interaction with Eukaryotic Initiation Factor 4G (eIF4G) and eIF3
Metazoan cell cycle-regulated histone mRNAs are unique cellular mRNAs in that they terminate in a highly conserved stem-loop structure instead of a poly(A) tail. Not only is the stem-loop structure necessary for 3'-end formation but it regulates the stability and translational efficiency of histone mRNAs. The histone stem-loop structure is recognized by the stem-loop-binding protein (SLBP), which is required for the regulation of mRNA processing and turnover. In this study, we show that SLBP is required for the translation of mRNAs containing the histone stem-loop structure. Moreover, we show that the translation of mRNAs ending in the histone stem-loop is stimulated in Saccharomyces cerevisiae cells expressing mammalian SLBP. The translational function of SLBP genetically required eukaryotic initiation factor 4E (eIF4E), eIF4G, and eIF3, and expressed SLBP coisolated with S. cerevisiae initiation factor complexes that bound the 5' cap in a manner dependent on eIF4G and eIF3. Furthermore, eIF4G coimmunoprecipitated with endogenous SLBP in mammalian cell extracts and recombinant SLBP and eIF4G coisolated. These data indicate that SLBP stimulates the translation of histone mRNAs through a functional interaction with both the mRNA stem-loop and the 5' cap that is mediated by eIF4G and eIF3
Corrigendum: hypoxic induced decrease in oxygen consumption in cuttlefish (Sepia officinalis) Is Associated with minor increases in Mantle Octopine but no changes in markers of protein turnover
Corrige o artigo http://hdl.handle.net/10400.1/10858 [This corrects the article DOI: 10.3389/fphys.2017.00344.].info:eu-repo/semantics/publishedVersio
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