16 research outputs found

    Limitation on holographic storage in photorefractive waveguides

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    We show that photorefractive waveguide devices are subject to a limitation on their holographic storage capability owing to transversely nonuniform nonlinear losses to evanescent and radiation modes

    Table-Top Milliwatt-Class Extreme Ultraviolet High Harmonic Light Source

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    Extreme ultraviolet (XUV) lasers are essential for the investigation of fundamental physics. Especially high repetition rate, high photon flux sources are of major interest for reducing acquisition times and improving signal to noise ratios in a plethora of applications. Here, an XUV source based on cascaded frequency conversion is presented, which delivers due to the drastic better single atom response for short wavelength drivers, an average output power of (832 +- 204) {\mu}W at 21.7 eV. This is the highest average power produced by any HHG source in this spectral range surpassing precious demonstrations by more than a factor of four. Furthermore, a narrow-band harmonic at 26.6 eV with a relative energy bandwidth of only {\Delta}E/E= 1.8 x 10E-3 has been generated, which is of high interest for high precision spectroscopy experiments.Comment: 4 Pages, 4 Picture

    High-repetition-rate and high-photon-flux 70 eV high-harmonic source for coincidence ion imaging of gas-phase molecules

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    Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced the field by enabling advanced pump-probe schemes. There is an increasing interest in using table-top photon sources enabled by high-harmonic generation of ultrashort-pulse lasers for such studies. We present a novel high-harmonic source driven by a 100 kHz fiber laser system, which delivers 1011^{11} photons/s in a single 1.3 eV bandwidth harmonic at 68.6 eV. The combination of record-high photon flux and high repetition rate paves the way for time-resolved studies of the dissociation dynamics of inner-shell ionized molecules in a coincidence detection scheme. First coincidence measurements on CH3_3I are shown and it is outlined how the anticipated advancement of fiber laser technology and improved sample delivery will, in the next step, allow pump-probe studies of ultrafast molecular dynamics with table-top XUV-photon sources. These table-top sources can provide significantly higher repetition rates than the currently operating free-electron lasers and they offer very high temporal resolution due to the intrinsically small timing jitter between pump and probe pulses

    Rapid internal bubble formation in a microwave heated polymer observed in real-time by x-ray scattering

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    International audienceA combined study of small-angle and wide-angle X-rayscattering (SAXS/WAXS) of the melting of a nylon-6 sample by localized microwave radiation has shown that this method can reveal the presence of bubbles forming and disappearing rapidly in realtime in the interior of the sample due to its thermal decomposition

    Nanoparticle plasma ejected directly from solid copper by localized microwaves

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    International audienceA plasma column ejected directly from solid copper by localized microwaves is studied. The effect stems from an induced hotspot that melts and emits ionized copper vapors as a confined fire column. Nanoparticles of ~20-120 nm size were revealed in the ejected column by in situ small-angle x-ray scattering. Optical spectroscopy confirmed the dominance of copper particles in the plasma column originating directly from the copper substrate. Nano- and macroparticles of copper were verified also by ex situ scanning electron microscopy. The direct conversion of solid metals to nanoparticles is demonstrated and various applications are proposed
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