16 research outputs found
Limitation on holographic storage in photorefractive waveguides
We show that photorefractive waveguide devices are subject to a limitation on their holographic storage capability owing to transversely nonuniform nonlinear losses to evanescent and radiation modes
Table-Top Milliwatt-Class Extreme Ultraviolet High Harmonic Light Source
Extreme ultraviolet (XUV) lasers are essential for the investigation of
fundamental physics. Especially high repetition rate, high photon flux sources
are of major interest for reducing acquisition times and improving signal to
noise ratios in a plethora of applications. Here, an XUV source based on
cascaded frequency conversion is presented, which delivers due to the drastic
better single atom response for short wavelength drivers, an average output
power of (832 +- 204) {\mu}W at 21.7 eV. This is the highest average power
produced by any HHG source in this spectral range surpassing precious
demonstrations by more than a factor of four. Furthermore, a narrow-band
harmonic at 26.6 eV with a relative energy bandwidth of only {\Delta}E/E= 1.8 x
10E-3 has been generated, which is of high interest for high precision
spectroscopy experiments.Comment: 4 Pages, 4 Picture
High-repetition-rate and high-photon-flux 70 eV high-harmonic source for coincidence ion imaging of gas-phase molecules
Unraveling and controlling chemical dynamics requires techniques to image
structural changes of molecules with femtosecond temporal and picometer spatial
resolution. Ultrashort-pulse x-ray free-electron lasers have significantly
advanced the field by enabling advanced pump-probe schemes. There is an
increasing interest in using table-top photon sources enabled by high-harmonic
generation of ultrashort-pulse lasers for such studies. We present a novel
high-harmonic source driven by a 100 kHz fiber laser system, which delivers
10 photons/s in a single 1.3 eV bandwidth harmonic at 68.6 eV. The
combination of record-high photon flux and high repetition rate paves the way
for time-resolved studies of the dissociation dynamics of inner-shell ionized
molecules in a coincidence detection scheme. First coincidence measurements on
CHI are shown and it is outlined how the anticipated advancement of fiber
laser technology and improved sample delivery will, in the next step, allow
pump-probe studies of ultrafast molecular dynamics with table-top XUV-photon
sources. These table-top sources can provide significantly higher repetition
rates than the currently operating free-electron lasers and they offer very
high temporal resolution due to the intrinsically small timing jitter between
pump and probe pulses
Rapid internal bubble formation in a microwave heated polymer observed in real-time by x-ray scattering
International audienceA combined study of small-angle and wide-angle X-rayscattering (SAXS/WAXS) of the melting of a nylon-6 sample by localized microwave radiation has shown that this method can reveal the presence of bubbles forming and disappearing rapidly in realtime in the interior of the sample due to its thermal decomposition
Nanoparticle plasma ejected directly from solid copper by localized microwaves
International audienceA plasma column ejected directly from solid copper by localized microwaves is studied. The effect stems from an induced hotspot that melts and emits ionized copper vapors as a confined fire column. Nanoparticles of ~20-120 nm size were revealed in the ejected column by in situ small-angle x-ray scattering. Optical spectroscopy confirmed the dominance of copper particles in the plasma column originating directly from the copper substrate. Nano- and macroparticles of copper were verified also by ex situ scanning electron microscopy. The direct conversion of solid metals to nanoparticles is demonstrated and various applications are proposed