36 research outputs found

    Appearance of the Single Gyroid Network Phase in Nuclear Pasta Matter

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    Nuclear matter under the conditions of a supernova explosion unfolds into a rich variety of spatially structured phases, called nuclear pasta. We investigate the role of periodic network-like structures with negatively curved interfaces in nuclear pasta structures, by static and dynamic Hartree-Fock simulations in periodic lattices. As the most prominent result, we identify for the first time the {\it single gyroid} network structure of cubic chiral I4123I4_123 symmetry, a well known configuration in nanostructured soft-matter systems, both as a dynamical state and as a cooled static solution. Single gyroid structures form spontaneously in the course of the dynamical simulations. Most of them are isomeric states. The very small energy differences to the ground state indicate its relevance for structures in nuclear pasta.Comment: 7 pages, 4 figure

    Static and Dynamic Chain Structures in the Mean-Field Theory

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    We give a brief overview of recent work examining the presence of α\alpha-clusters in light nuclei within the Skyrme-force Hartree-Fock model. Of special significance are investigations into α\alpha-chain structures in carbon isotopes and 16^{16}O. Their stability and possible role in fusion reactions are examined in static and time-dependent Hartree-Fock calculations. We find a new type of shape transition in collisions and a centrifugal stabilization of the 4α4\alpha chain state in a limited range of angular momenta. No stabilization is found for the 3α3\alpha chain.Comment: Fusionn 11 Conference, St. Malo, France, 201

    Finite temperature pasta matter with the TDHF approximation

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    Exotic cluster structures in the mean-field theory

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    Investigations of exotic cluster-like phenomena in the framework of the Skyrme-Hartree-Fock approach are reported. The occurrence of highly excited isomeric states is discussed in connection with the question of their stability in static and time-dependent Hartree Fock (TDHF) calculations. We find rotational stabilization of a 4α chain structure in 16O occurring for a limited range of angular momenta. A toroidal configuration of 40Ca was also stabilized by rotation and provides a very interesting example of rotation about a symmetry axis with a strictly quantized total angular momentum. Finally we look at the formation of nuclear pasta phases in a time-dependent approach and their classification

    From Tetrahedral Tetraphosphonic Acids E[p-C6H4P(O)(OH)(2)](4) (E=C, Si) to Porous Cu- and Zn-MOFs with Large Surface Areas

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    This study describes the porous MOFs Cu2H4STPPA⋅2 H2O (1⋅2 H2O), Zn2H4STPPA (2) and Zn2H4MTPPA (3) obtained using the tetrahedral linkers tetraphenylmethane tetrakis-4-phosphonic acid (H8MTTPA) and tetraphenylsilane tetrakis-4-phosphonic acid (H8STPPA) under solvothermal conditions. X-ray structures reveal 3D frameworks with large assessable voids. The percentage void volumes and the specific BET surface areas of 1 (48.7 %, 794 m2/g), 2 (48.1 %, 565 m2/g) and 3 (51.3 %, 927 m2/g) predicted by molecular simulations are among the highest reported for MOFs derived from phosphonic acids

    Probing Sizes and Shapes of Nobelium Isotopes by Laser Spectroscopy

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    Until recently, ground-state nuclear moments of the heaviest nuclei could only be inferred from nuclear spectroscopy, where model assumptions are required. Laser spectroscopy in combination with modern atomic structure calculations is now able to probe these moments directly, in a comprehensive and nuclear-model-independent way. Here we report on unique access to the differential mean-square charge radii of 252, 253, 254No, and therefore to changes in nuclear size and shape. State-of-the-art nuclear density functional calculations describe well the changes in nuclear charge radii in the region of the heavy actinides, indicating an appreciable central depression in the deformed proton density distribution in 252, 254No isotopes. Finally, the hyperfine splitting of 253No was evaluated, enabling a complementary measure of its (quadrupole) deformation, as well as an insight into the neutron single-particle wave function via the nuclear spin and magnetic moment

    The TDHF code Sky3D version 1.1

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    The nuclear mean-field model based on Skyrme forces or related density functionals has found widespread application to the description of nuclear ground states, collective vibrational excitations, and heavy-ion collisions. The code Sky3D solves the static or dynamic equations on a three-dimensional Cartesian mesh with isolated or periodic boundary conditions and no further symmetry assumptions. Pairing can be included in the BCS approximation for the static case. The code is implemented with a view to allow easy modifications for including additional physics or special analysis of the results
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