6,091 research outputs found
Giant vesicles at the prolate-oblate transition: A macroscopic bistable system
Giant phospholipid vesicles are shown to exhibit thermally activated
transitions between a prolate and an oblate shape on a time scale of several
seconds. From the fluctuating contour of such a vesicle we extract ellipticity
as an effective reaction coordinate whose temporal probability distribution is
bimodal. We then reconstruct the effective potential from which we derive an
activation energy of the order of in agreement with theoretical
calculations. The dynamics of this transition is well described within a
Kramers model of overdamped diffusion in a bistable potential. Thus, this
system can serve as a model for macroscopic bistability.Comment: 10 pages, LaTeX, epsfig, 4 eps figures included, to appear in
Europhys. Let
Reconstructing the global topology of the universe from the cosmic microwave background
If the universe is multiply-connected and sufficiently small, then the last
scattering surface wraps around the universe and intersects itself. Each circle
of intersection appears as two distinct circles on the microwave sky. The
present article shows how to use the matched circles to explicitly reconstruct
the global topology of space.Comment: 6 pages, 2 figures, IOP format. To be published in the proceedings of
the Cleveland Cosmology and Topology Workshop 17-19 Oct 1997. Submitted to
Class. Quant. Gra
Tidal controls on trace gas dynamics in a seagrass meadow of the Ria Formosa lagoon (southern Portugal)
Coastal zones are important source regions for a variety of trace gases, including halocarbons and sulfur-bearing species. While salt marshes, macroalgae and phyto-plankton communities have been intensively studied, little is known about trace gas fluxes in seagrass meadows. Here we report results of a newly developed dynamic flux chamber system that can be deployed in intertidal areas over full tidal cycles allowing for highly time-resolved measurements. The fluxes of CO2, methane (CH4) and a range of volatile organic compounds (VOCs) showed a complex dynamic mediated by tide and light. In contrast to most previous studies, our data indicate significantly enhanced fluxes during tidal immersion relative to periods of air exposure. Short emission peaks occurred with onset of the feeder current at the sampling site. We suggest an overall strong effect of advective transport processes to explain the elevated fluxes during tidal immersion. Many emission estimates from tidally influenced coastal areas still rely on measurements carried out during low tide only. Hence, our results may have significant implications for budgeting trace gases in coastal areas. This dynamic flux chamber system provides intensive time series data of community respiration (at night) and net community production (during the day) of shallow coastal systems.German Federal Ministry of Education and Research (BMBF) [03F0611E, 03F0662E]; EU FP7 ASSEMBLE research infrastructure initiative
The ultrafast laser ablation of Li(NiMnCo)O electrodes with high mass loading
Lithium-ion batteries have become the most promising energy storage devices in recent years. However, the simultaneous increase of energy density and power density is still a huge challenge. Ultrafast laser structuring of electrodes is feasible to increase power density of lithium-ion batteries by improving the lithium-ion diffusion kinetics. The influences of laser processing pattern and film thickness on the rate capability and energy density were investigated using Li(Ni0.6Mn0.2Co0.2)O2 (NMC 622) as cathode material. NMC 622 electrodes with thicknesses from 91 µm to 250 µm were prepared, while line patterns with pitch distances varying from 200 µm to 600 µm were applied. The NMC 622 cathodes were assembled opposing lithium using coin cell design. Cells with structured, 91 µm thick film cathodes showed lesser capacity losses with C-rates 3C compared to cells with unstructured cathode. Cells with 250 µm thick film cathode showed higher discharge capacity with low C-rates of up to C/5, and the structured cathodes showed higher discharge capacity, with C-rates of up to 1C. However, the discharge capacity deteriorated with higher C-rate. An appropriate choice of laser generated patterns and electrode thickness depends on the requested battery application scenario; i.e., charge/discharge rate and specific/volumetric energy density
Mobility and Diffusion of a Tagged Particle in a Driven Colloidal Suspension
We study numerically the influence of density and strain rate on the
diffusion and mobility of a single tagged particle in a sheared colloidal
suspension. We determine independently the time-dependent velocity
autocorrelation functions and, through a novel method, the response functions
with respect to a small force. While both the diffusion coefficient and the
mobility depend on the strain rate the latter exhibits a rather weak
dependency. Somewhat surprisingly, we find that the initial decay of response
and correlation functions coincide, allowing for an interpretation in terms of
an 'effective temperature'. Such a phenomenological effective temperature
recovers the Einstein relation in nonequilibrium. We show that our data is well
described by two expansions to lowest order in the strain rate.Comment: submitted to EP
Two-Component Fluid Membranes Near Repulsive Walls: Linearized Hydrodynamics of Equilibrium and Non-equilibrium States
We study the linearized hydrodynamics of a two-component fluid membrane near
a repulsive wall, via a model which incorporates curvature- concentration
coupling as well as hydrodynamic interactions. This model is a simplified
version of a recently proposed one [J.-B. Manneville et al. Phys. Rev. E, 64,
021908 (2001)] for non-equilibrium force-centres embedded in fluid membranes,
such as light-activated bacteriorhodopsin pumps incorporated in phospholipid
(EPC) bilayers. The pump/membrane system is modeled as an impermeable,
two-component bilayer fluid membrane in the presence of an ambient solvent, in
which one component, representing active pumps, is described in terms of force
dipoles displaced with respect to the bilayer midpoint. We first discuss the
case in which such pumps are rendered inactive, computing the mode structure in
the bulk as well as the modification of hydrodynamic properties by the presence
of a nearby wall. We then discuss the fluctuations and mode structure in steady
state of active two-component membranes near a repulsive wall. We find that
proximity to the wall smoothens membrane height fluctuations in the stable
regime, resulting in a logarithmic scaling of the roughness even for initially
tensionless membranes. This explicitly non-equilibrium result, a consequence of
the incorporation of curvature-concentration coupling in our treatment, also
indicates that earlier scaling arguments which obtained an increase in the
roughness of active membranes near repulsive walls may need to be reevaluated.Comment: 39 page Latex file, 3 encapsulated Postscript figure
SPH Simulations of Counterrotating Disk Formation in Spiral Galaxies
We present the results of Smoothed Particle Hydrodynamics (SPH) simulations
of the formation of a massive counterrotating disk in a spiral galaxy. The
current study revisits and extends (with SPH) previous work carried out with
sticky particle gas dynamics, in which adiabatic gas infall and a retrograde
gas-rich dwarf merger were tested as the two most likely processes for
producing such a counterrotating disk. We report on experiments with a cold
primary similar to our Galaxy, as well as a hot, compact primary modeled after
NGC 4138. We have also conducted numerical experiments with varying amounts of
prograde gas in the primary disk, and an alternative infall model (a spherical
shell with retrograde angular momentum). The structure of the resulting
counterrotating disks is dramatically different with SPH. The disks we produce
are considerably thinner than the primary disks and those produced with sticky
particles. The time-scales for counterrotating disk formation are shorter with
SPH because the gas loses kinetic energy and angular momentum more rapidly.
Spiral structure is evident in most of the disks, but an exponential radial
profile is not a natural byproduct of these processes. The infalling gas shells
that we tested produce counterrotating bulges and rings rather than disks. The
presence of a considerable amount of preexisting prograde gas in the primary
causes, at least in the absence of star formation, a rapid inflow of gas to the
center and a subsequent hole in the counterrotating disk. In general, our SPH
experiments yield stronger evidence to suggest that the accretion of massive
counterrotating disks drives the evolution of the host galaxies towards earlier
(S0/Sa) Hubble types.Comment: To appear in ApJ. 20 pages LaTex 2-column with 3 tables, 23 figures
(GIF) available at this site. Complete gzipped postscript preprint with
embedded figures available from http://tarkus.pha.jhu.edu/~thakar/cr3.html (3
Mb
Photoconductance of a submicron oxidized line in surface conductive single crystalline diamond
We report on sub-bandgap optoelectronic phenomena of hydrogen-terminated
diamond patterned with a submicron oxidized line. The line acts as an energy
barrier for the two-dimensional hole gas located below the hydrogenated diamond
surface. A photoconductive gain of the hole conductivity across the barrier is
measured for sub-bandgap illumination. The findings are consistent with
photogenerated electrons being trapped in defect levels within the barrier. We
discuss the spatial and energetic characteristics of the optoelectronic
phenomena, as well as possible photocurrent effects
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