9,192 research outputs found
Transient charge and energy flow in the wide-band limit
The wide-band limit is a commonly used approximation to analyze transport
through nanoscale devices. In this work we investigate its applicability to the
study of charge and heat transport through molecular break junctions exposed to
voltage biases and temperature gradients. We find that while this approximation
faithfully describes the long-time charge and heat transport, it fails to
characterize the short-time behavior of the junction. In particular, we find
that the charge current flowing through the device shows a discontinuity when a
temperature gradient is applied, while the energy flow is discontinuous when a
voltage bias is switched on and even diverges when the junction is exposed to
both a temperature gradient and a voltage bias. We provide an explanation for
this pathological behavior and propose two possible solutions to this problem.Comment: 11 pages, 9 figure
Observation of a parity oscillation in the conductance of atomic wires
Using a scanning tunnel microscope or mechanically controlled break
junctions, atomic contacts of Au, Pt and Ir are pulled to form chains of atoms.
We have recorded traces of conductance during the pulling process and averaged
these for a large amount of contacts. An oscillatory evolution of conductance
is observed during the formation of the monoatomic chain suggesting a
dependence on even or odd numbers of atoms forming the chain. This behaviour is
not only present in the monovalent metal Au, as it has been previously
predicted, but is also found in the other metals which form chains suggesting
it to be a universal feature of atomic wires
Dynamics of quartz tuning fork force sensors used in scanning probe microscopy
We have performed an experimental characterization of the dynamics of
oscillating quartz tuning forks which are being increasingly used in scanning
probe microscopy as force sensors. We show that tuning forks can be described
as a system of coupled oscillators. Nevertheless, this description requires the
knowledge of the elastic coupling constant between the prongs of the tuning
fork, which has not yet been measured. Therefore tuning forks have been usually
described within the single oscillator or the weakly coupled oscillators
approximation that neglects the coupling between the prongs. We propose three
different procedures to measure the elastic coupling constant: an
opto-mechanical method, a variation of the Cleveland method and a thermal noise
based method. We find that the coupling between the quartz tuning fork prongs
has a strong influence on the dynamics and the measured motion is in remarkable
agreement with a simple model of coupled harmonic oscillators. The precise
determination of the elastic coupling between the prongs of a tuning fork
allows to obtain a quantitative relation between the resonance frequency shift
and the force gradient acting at the free end of a tuning fork prong.Comment: 16 pages, 6 figures, 2 Table
Direct estimation of electron density in the Orion Bar PDR from mm-wave carbon recombination lines
A significant fraction of the molecular gas in star-forming regions is
irradiated by stellar UV photons. In these environments, the electron density
(n_e) plays a critical role in the gas dynamics, chemistry, and collisional
excitation of certain molecules. We determine n_e in the prototypical strongly
irradiated photodissociation region (PDR), the Orion Bar, from the detection of
new millimeter-wave carbon recombination lines (mmCRLs) and existing far-IR
[13CII] hyperfine line observations. We detect 12 mmCRLs (including alpha,
beta, and gamma transitions) observed with the IRAM 30m telescope, at ~25''
angular resolution, toward the H/H2 dissociation front (DF) of the Bar. We also
present a mmCRL emission cut across the PDR. These lines trace the C+/C/CO gas
transition layer. As the much lower frequency carbon radio recombination lines,
mmCRLs arise from neutral PDR gas and not from ionized gas in the adjacent HII
region. This is readily seen from their narrow line profiles (dv=2.6+/-0.4
km/s) and line peak LSR velocities (v_LSR=+10.7+/-0.2 km/s). Optically thin
[13CII] hyperfine lines and molecular lines - emitted close to the DF by trace
species such as reactive ions CO+ and HOC+ - show the same line profiles. We
use non-LTE excitation models of [13CII] and mmCRLs and derive n_e = 60-100
cm^-3 and T_e = 500-600 K toward the DF. The inferred electron densities are
high, up to an order of magnitude higher than previously thought. They provide
a lower limit to the gas thermal pressure at the PDR edge without using
molecular tracers. We obtain P_th > (2-4)x10^8 cm^-3 K assuming that the
electron abundance is equal or lower than the gas-phase elemental abundance of
carbon. Such elevated thermal pressures leave little room for magnetic pressure
support and agree with a scenario in which the PDR photoevaporates.Comment: Accepted for publication in A&A Letters (includes language editor
corrections
A set of primers for length and nucleotide-substitution polymorphism in chloroplastic DNA of Olea europaea L. (Oleaceae)
Chloroplastic DNA (cpDNA) variation at five microsatellite motifs, two insertion-deletion sites, and eight nucleotide substitution sites was investigated in the Olea europaea complex. Primers were designed for flanking regions of these sites to amplify short cpDNA regions. They provided polymorphism when polymerase chain reaction (PCR) products from a representative sample of 128 O. europaea individuals were either resolved by size into polyacrylamide gels (length polymorphism) or digested with restriction enzymes (nucleotide-substitution polymorphism). These polymorphisms serve to distinguish most of the cytoplasmic haplotypes previously recognized. Potential application of these markers in O. europaea includes phylogeography, conservation and germplasm identification, even when using poorly preserved material from herbarium specimens or forensic and archaeological materials.This work was supported by the project BIOD-IBERIA (A82).Peer Reviewe
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