116 research outputs found
Mechanical, Electrical, and Magnetic Properties of Ni Nanocontacts
The dynamic deformation upon stretching of Ni nanowires as those formed with
mechanically controllable break junctions or with a scanning tunneling
microscope is studied both experimentally and theoretically. Molecular dynamics
simulations of the breaking process are performed. In addition, and in order to
compare with experiments, we also compute the transport properties in the last
stages before failure using the first-principles implementation of Landauer's
formalism included in our transport package ALACANT.Comment: 5 pages, 6 figure
Observation of a parity oscillation in the conductance of atomic wires
Using a scanning tunnel microscope or mechanically controlled break
junctions, atomic contacts of Au, Pt and Ir are pulled to form chains of atoms.
We have recorded traces of conductance during the pulling process and averaged
these for a large amount of contacts. An oscillatory evolution of conductance
is observed during the formation of the monoatomic chain suggesting a
dependence on even or odd numbers of atoms forming the chain. This behaviour is
not only present in the monovalent metal Au, as it has been previously
predicted, but is also found in the other metals which form chains suggesting
it to be a universal feature of atomic wires
Formation of a Metallic Contact: Jump to Contact Revisited
The transition from tunneling to metallic contact between two surfaces does
not always involve a jump, but can be smooth. We have observed that the
configuration and material composition of the electrodes before contact largely
determines the presence or absence of a jump. Moreover, when jumps are found
preferential values of conductance have been identified. Through combination of
experiments, molecular dynamics, and first-principles transport calculations
these conductance values are identified with atomic contacts of either
monomers, dimers or double-bond contacts.Comment: 4 pages, 5 figure
Analysis of the Kondo effect in ferromagnetic atomic-sized contacts
Atomic contacts made of ferromagnetic metals present zero-bias anomalies in
the differential conductance due to the Kondo effect. These systems provide a
unique opportunity to perform a statistical analysis of the Kondo parameters in
nanostructures since a large number of contacts can be easily fabricated using
break-junction techniques. The details of the atomic structure differ from one
contact to another so a large number of different configurations can be
statistically analyzed. Here we present such a statistical analysis of the
Kondo effect in atomic contacts made from the ferromagnetic transition metals
Ni, Co and Fe. Our analysis shows clear differences between materials that can
be understood by fundamental theoretical considerations. This combination of
experiments and theory allow us to extract information about the origin and
nature of the Kondo effect in these systems and to explore the influence of
geometry and valence in the Kondo screening of atomic-sized nanostructures.Comment: 17 pages, 11 figure
Circles of Connection: Finding Social Connectedness and Meaning within Group Process
Social participation is an area of occupation that can increase and enhance an individual’s participation in life. This is particularly true in senior housing communities where common issues of aging and adjustment can be addressed while reducing feelings of social isolation. The purpose of this demonstration project was to provide a venue where older adults living at The Redwoods, a senior housing community in Mill Valley, California, could share and develop meaningful strategies for living, and ultimately foster a sense of connectedness, which would affect quality of life. The project’s goals were to create and implement a series of process groups to benefit the well-being of the residents of The Redwoods, and to produce a resource manual for Dominican University occupational therapy graduate students in co-facilitating the process groups. The project and manual were used as the basis for a Community Practice Lab during which the students were able to gain experience in the psychosocial occupational therapy skills for which they had been trained, while simultaneously providing the residents with an opportunity for social engagement and meaningful activity. Within the scope of occupational therapy practice, therapists can develop and facilitate psychosocial process groups that promote connectedness and well-being among residents of senior housing communities
Onset of dissipation in ballistic atomic wires
Electronic transport at finite voltages in free-standing gold atomic chains
of up to 7 atoms in length is studied at low temperatures using a scanning
tunneling microscope (STM). The conductance vs voltage curves show that
transport in these single-mode ballistic atomic wires is non-dissipative up to
a finite voltage threshold of the order of several mV. The onset of dissipation
and resistance within the wire corresponds to the excitation of the atomic
vibrations by the electrons traversing the wire and is very sensitive to
strain.Comment: Revtex4, 4 pages, 3 fig
Stretching dependence of the vibration modes of a single-molecule Pt-H2-Pt bridge
A conducting bridge of a single hydrogen molecule between Pt electrodes is
formed in a break junction experiment. It has a conductance near the quantum
unit, G_0 = 2e^2/h, carried by a single channel. Using point contact
spectroscopy three vibration modes are observed and their variation upon
stretching and isotope substitution is obtained. The interpretation of the
experiment in terms of a Pt-H_2-Pt bridge is verified by Density Functional
Theory calculations for the stability, vibrational modes, and conductance of
the structure.Comment: 5 pages, 4 figure
Dynamic bonding of metallic nanocontacts: Insights from experiments and atomistic simulations
The conductance across an atomically narrow metallic contact can be measured by using scanning tunneling microscopy. In certain situations, a jump in the conductance is observed right at the point of contact between the tip and the surface, which is known as "jump to contact" (JC). Such behavior provides a way to explore, at a fundamental level, how bonding between metallic atoms occurs dynamically. This phenomenon depends not only on the type of metal but also on the geometry of the two electrodes. For example, while some authors always find JC when approaching two atomically sharp tips of Cu, others find that a smooth transition occurs when approaching a Cu tip to an adatom on a flat surface of Cu. In an attempt to show that all these results are consistent, we make use of atomistic simulations; in particular, classical molecular dynamics together with density functional theory transport calculations to explore a number of possible scenarios. Simulations are performed for two different materials: Cu and Au in a [100] crystal orientation and at a temperature of 4.2 K. These simulations allow us to study the contribution of short- and long-range interactions to the process of bonding between metallic atoms, as well as to compare directly with experimental measurements of conductance, giving a plausible explanation for the different experimental observations. Moreover, we show a correlation between the cohesive energy of the metal, its Young's modulus, and the frequency of occurrence of a jump to contactW. Dednam thanks Dr. A. E. Botha for helpful discussions and acknowledges support from the National Research Foundation of South Africa through the Scarce Skills Masters scholarship funding programme (Grant Unique Number 92138). This work is supported by the Generalitat Valenciana through Grant Reference PROMETEO2012/011 and MINECO under Grant No. FIS2013-47328, by European Union structural funds and the Comunidad de Madrid Programs S2013/MIT-3007 and P2013/MIT-2850. This work is also part of the research programme of the Foundation for Fundamental Research on Matter (FOM), which is financially supported by the Netherlands Organisation for Scientific Research (NWO
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