73 research outputs found

    Pressure-induced melting of the orbital polaron lattice in La1-xSrxMnO3

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    We report on the pressure effects on the orbital polaron lattice in the lightly doped manganites La1−xSrxMnO3\mathrm{La_{1-x}Sr_xMnO_{3}}, with x∼1/8x\sim 1/8. The dependence of the orbital polaron lattice on negativenegative chemical pressure is studied by substituting Pr for La in (La1−yPry)7/8Sr1/8MnO3\mathrm{(La_{1-y}Pr_y)_{7/8}Sr_{1/8}MnO_{3}}. In addition, we have studied its hydrostatic pressure dependence in (La0.9Pr0.1)7/8Sr1/8MnO3\mathrm{(La_{0.9}Pr_{0.1})_{7/8}Sr_{1/8}MnO_{3}}. Our results strongly indicate that the hopping tt significantly contributes to the stabilization of the orbital polaron lattice and that the orbital polarons are ferromagnetic objects which get stabilized by local double exchange processes. The analysis of short range orbital correlations and the verification of the Grueneisen scaling by hard x-ray, specific heat and thermal expansion data reinforces our conclusions.Comment: 7 figure

    Approach to the metal-insulator transition in La(1-x)CaxMnO3 (0<x<.2): magnetic inhomogeneity and spin wave anomaly

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    We describe the evolution of the static and dynamic spin correlations of La1−x_{1-x}Cax_xMnO3_3, for x=0.1, 0.125 and 0.2, where the system evolves from the canted magnetic state towards the insulating ferromagnetic state, approaching the metallic transition (x=0.22). In the x=0.1 sample, the observation of two spin wave branches typical of two distinct types of magnetic coupling, and of a modulation in the elastic diffuse scattering characteristic of ferromagnetic inhomogeneities, confirms the static and dynamic inhomogeneous features previously observed at x<<0.1. The anisotropic q-dependence of the intensity of the low-energy spin wave suggests a bidimensionnal character for the static inhomogeneities. At x=0.125, which corresponds to the occurence of a ferromagnetic and insulating state, the two spin wave branches reduce to a single one, but anisotropic. At this concentration, an anomaly appears at {\bf q0_0}=(1.25,1.25,0), that could be related to an underlying periodicity, as arising from (1.5,1.5,0) superstructures. At x=0.2, the spin-wave branch is isotropic. In addition to the anomaly observed at q0_0, extra magnetic excitations are observed at larger q, forming an optical branch. The two dispersion curves suggest an anti-crossing behavior at some {\bf q0_0'} value, which could be explained by a folding due to an underlying perodicity involving four cubic lattice spacings

    The COSPIX mission: focusing on the energetic and obscured Universe

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    Tracing the formation and evolution of all supermassive black holes, including the obscured ones, understanding how black holes influence their surroundings and how matter behaves under extreme conditions, are recognized as key science objectives to be addressed by the next generation of instruments. These are the main goals of the COSPIX proposal, made to ESA in December 2010 in the context of its call for selection of the M3 mission. In addition, COSPIX, will also provide key measurements on the non thermal Universe, particularly in relation to the question of the acceleration of particles, as well as on many other fundamental questions as for example the energetic particle content of clusters of galaxies. COSPIX is proposed as an observatory operating from 0.3 to more than 100 keV. The payload features a single long focal length focusing telescope offering an effective area close to ten times larger than any scheduled focusing mission at 30 keV, an angular resolution better than 20 arcseconds in hard X-rays, and polarimetric capabilities within the same focal plane instrumentation. In this paper, we describe the science objectives of the mission, its baseline design, and its performances, as proposed to ESA.Comment: 7 pages, accepted for publication in Proceedings of Science, for the 25th Texas Symposium on Relativistic Astrophysics (eds. F. Rieger &amp; C. van Eldik), PoS(Texas 2010)25

    Optical study of orbital excitations in transition-metal oxides

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    The orbital excitations of a series of transition-metal compounds are studied by means of optical spectroscopy. Our aim was to identify signatures of collective orbital excitations by comparison with experimental and theoretical results for predominantly local crystal-field excitations. To this end, we have studied TiOCl, RTiO3 (R=La, Sm, Y), LaMnO3, Y2BaNiO5, CaCu2O3, and K4Cu4OCl10, ranging from early to late transition-metal ions, from t_2g to e_g systems, and including systems in which the exchange coupling is predominantly three-dimensional, one-dimensional or zero-dimensional. With the exception of LaMnO3, we find orbital excitations in all compounds. We discuss the competition between orbital fluctuations (for dominant exchange coupling) and crystal-field splitting (for dominant coupling to the lattice). Comparison of our experimental results with configuration-interaction cluster calculations in general yield good agreement, demonstrating that the coupling to the lattice is important for a quantitative description of the orbital excitations in these compounds. However, detailed theoretical predictions for the contribution of collective orbital modes to the optical conductivity (e.g., the line shape or the polarization dependence) are required to decide on a possible contribution of orbital fluctuations at low energies, in particular in case of the orbital excitations at about 0.25 eV in RTiO3. Further calculations are called for which take into account the exchange interactions between the orbitals and the coupling to the lattice on an equal footing.Comment: published version, discussion of TiOCl extended to low T, improved calculation of orbital excitation energies in TiOCl, figure 16 improved, references updated, 33 pages, 20 figure

    The Athena X-ray Integral Field Unit: a consolidated design for the system requirement review of the preliminary definition phase

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