Thermodynamics of nuclei in thermal contact

The behaviour of a di-nuclear system in the regime of strong pairing correlations is studied with the methods of statistical mechanics. It is shown that the thermal averaging is strong enough to assure the application of thermodynamical methods to the energy exchange between the two nuclei in contact. In particular, thermal averaging justifies the definition of a nuclear temperature.Comment: 9 pages, 1 figur

Final excitation energy of fission fragments

We study how the excitation energy of the fully accelerated fission fragments is built up. It is stressed that only the intrinsic excitation energy available before scission can be exchanged between the fission fragments to achieve thermal equilibrium. This is in contradiction with most models used to calculate prompt neutron emission where it is assumed that the total excitation energy of the final fragments is shared between the fragments by the condition of equal temperatures. We also study the intrinsic excitation-energy partition according to a level density description with a transition from a constant-temperature regime to a Fermi-gas regime. Complete or partial excitation-energy sorting is found at energies well above the transition energy.Comment: 8 pages, 3 figure

Non-stoichiometric oxide and metal interfaces and reactions

We have employed a combination of experimental surface science techniques and density functional calculations to study the reduction of TiO2(110) surfaces through the doping with submonolayer transition metals. We concentrate on the role of Ti adatoms in self doping of rutile and contrast the behaviour to that of Cr. DFT+U calculations enable identification of probable adsorption structures and their spectroscopic characteristics. Adsorption of both metals leads to a broken symmetry and an asymmetric charge transfer localised around the defect site of a mixed localised/delocalised character. Charge transfer creates defect states with Ti 3d character in the band gap at similar to 1-eV binding energy. Cr adsorption, however, leads to a very large shift in the valence-band edge to higher binding energy and the creation of Cr 3d states at 2.8-eV binding energy. Low-temperature oxidation lifts the Ti-derived band-gap states and modifies the intensity of the Cr features, indicative of a change of oxidation state from Cr3+ to Cr4+. Higher temperature processing leads to a loss of Cr from the surface region, indicative of its substitution into the bulk

Modelling of compound nucleus formation in fusion of heavy nuclei

A new model that includes the time-dependent dynamics of the single-particle (s.p.) motion in conjunction with the macroscopic evolution of the system is proposed for describing the compound nucleus (CN) formation in fusion of heavy nuclei. The diabaticity initially keeps the entrance system around its contact configuration, but the gradual transition from the diabatic to the adiabatic potential energy surface (PES) leads to fusion or quasifission. Direct measurements of the probability for CN formation are crucial to discriminate between the current models.Comment: 4 pages,2 figures,1 table, Submitted to PR

Mechanical and chemical spinodal instabilities in finite quantum systems

Self consistent quantum approaches are used to study the instabilities of finite nuclear systems. The frequencies of multipole density fluctuations are determined as a function of dilution and temperature, for several isotopes. The spinodal region of the phase diagrams is determined and it appears that instabilities are reduced by finite size effects. The role of surface and volume instabilities is discussed. It is indicated that the important chemical effects associated with mechanical disruption may lead to isospin fractionation.Comment: 4 pages, 4 figure

Liquid-Drop Model and Quantum Resistance Against Noncompact Nuclear Geometries

The importance of quantum effects for exotic nuclear shapes is demonstrated. Based on the example of a sheet of nuclear matter of infinite lateral dimensions but finite thickness, it is shown that the quantization of states in momentum space, resulting from the confinement of the nucleonic motion in the conjugate geometrical space, generates a strong resistance against such a confinement and generates restoring forces driving the system towards compact geometries. In the liquid-drop model, these quantum effects are implicitly included in the surface energy term, via a choice of interaction parameters, an approximation that has been found valid for compact shapes, but has not yet been scrutinized for exotic shapes.Comment: 9 pages with 3 figure

Au+Au central collisions at 150, 250 and 400 AMeV energies in QMD with relativistic forces

An extensive comparison of the recent experimental data published by the FOPI collaboration at GSI with the results of a relativistically covariant formulation of a QMD code is presented. For most of the quantities we find agreement with the experimental results showing that the derived force has a reasonable momentum dependence.Comment: 33 pages with 18 EPSF figures included. Final version to appear in Nucl. Phys.

Production of Neutron-rich Heavy Residues and the Freeze-out Temperature in the Fragmentation of Relativistic 238U Projectiles Determined by the Isospin Thermometer

Isotope yields of heavy residues produced in collisions of 238U with lead at 1AGeV show indications for a simultaneous break-up process. From the average N-over-Z ratio of the final residues up to Z = 70, the average limiting temperature of the break-up configuration at freeze out was determined to T approximately 5 MeV using the isospin-thermometer method. Consequences for the understanding of other phenomena in highly excited nuclear systems are discussed.Comment: 22 pages, 9 figures, accepted by Nucl. Phys.

Modeling Complex Nuclear Spectra - Regularity versus Chaos

A statistical analysis of the spectrum of two particle - two hole doorway states in a finite nucleus is performed. On the unperturbed mean-field level sizable attractive correlations are present in such a spectrum. Including particle-hole rescattering effects via the residual interaction introduces repulsive dynamical correlations which generate the fluctuation properties characteristic of the Gaussian Orthogonal Ensemble. This signals that the underlying dynamics becomes chaotic. This feature turns out to be independent of the detailed form of the residual interaction and hence reflects the generic nature of the fluctuations studied.Comment: 8 pages of text (LATEX), figures (not included, available from the authors), Feb 9

Random Matrices and Chaos in Nuclear Physics

The authors review the evidence for the applicability of random--matrix theory to nuclear spectra. In analogy to systems with few degrees of freedom, one speaks of chaos (more accurately: quantum chaos) in nuclei whenever random--matrix predictions are fulfilled. An introduction into the basic concepts of random--matrix theory is followed by a survey over the extant experimental information on spectral fluctuations, including a discussion of the violation of a symmetry or invariance property. Chaos in nuclear models is discussed for the spherical shell model, for the deformed shell model, and for the interacting boson model. Evidence for chaos also comes from random--matrix ensembles patterned after the shell model such as the embedded two--body ensemble, the two--body random ensemble, and the constrained ensembles. All this evidence points to the fact that chaos is a generic property of nuclear spectra, except for the ground--state regions of strongly deformed nuclei.Comment: 54 pages, 28 figure