Metrology of Complex Refractive Index for Solids in the Terahertz Regime Using Frequency Domain Spectroscopy

Frequency domain spectroscopy allows an experimenter to establish optical properties of solids in a wide frequency band including the technically challenging 10 THz region, and in other bands enables metrological comparison between competing techniques. We advance a method for extracting the optical properties of high-index solids using only transmission-mode frequency domain spectroscopy of plane-parallel Fabry-Perot optical flats. We show that different data processing techniques yield different kinds of systematic error, and that some commonly used techniques have inherent systematic errors which are underappreciated. We use model datasets to cross-compare algorithms in isolation from experimental errors, and propose a new algorithm which has qualitatively different systematic errors to its competitors. We show that our proposal is more robust to experimental non-idealities such as noise or apodization, and extract the complex refractive index spectrum of crystalline silicon as a practical example. Finally, we advance the idea that algorithms are complementary rather than competitive, and should be used together as part of a toolbox for better metrology.Comment: 21 pages, 11 figures, 4 appendice

Si/SiGe bound-to-continuum quantum cascade emitters

Si/SiGe bound-to-continuum quantum cascade emitters designed by self-consistent 6-band k.p modeling and grown by low energy plasma enhanced chemical vapour deposition are presented demonstrating electroluminescence between 1.5 and 3 THz. The electroluminescence is Stark shifted by an electric field and demonstrates polarized emission consistent with the design. Transmission electron microscopy and x-ray diffraction are also presented to characterize the thick heterolayer structure

Virus lasers for biological detection

The selective amplification of DNA in the polymerase chain reaction is used to exponentially increase the signal in molecular diagnostics for nucleic acids, but there are no analogous techniques for signal enhancement in clinical tests for proteins or cells. Instead, the signal from affinity-based measurements of these biomolecules depends linearly on the probe concentration. Substituting antibody-based probes tagged for fluorescent quantification with lasing detection probes would create a new platform for biomarker quantification based on optical rather than enzymatic amplification. Here, we construct a virus laser which bridges synthetic biology and laser physics, and demonstrate virus-lasing probes for biosensing. Our virus-lasing probes display an unprecedented > 10,000 times increase in signal from only a 50% increase in probe concentration, using fluorimeter-compatible optics, and can detect biomolecules at sub-100 fmol mL-1 concentrations

Sediment source and mixing and the cycle of sediment transport: an example from NE Negev Desert, Israel.

Alluvial terraces represent the end product of sedimentary cycles; each includes sediment generation, transport, accumulation, and the ultimate incision that forms abandoned alluvial surfaces. We examine the middle Pleistocene to recent drainage system evolution in Makhtesh Hazera, Negev Desert, southern Israel and compare the characteristics of erosion and sediment transport in the present system with those expressed by the alluvial terraces. The Hazera drainage basin lies at the margins of the arid to hyper-arid Dead Sea rift (DSR). Makhtesh (crater) Hazera is a deeply incised erosional structure (5X7 km) that has been excavated since the early Pliocene into the crest of the Hazera asymmetric anticline. The Makhtesh floor is surrounded by cliffs rising more than 400 meters high. The cliffs are built of Upper Cretaceous hard carbonates caprocks overlying Lower Cretaceous friable quartz sandstones. Bedrock knickpoints isolate the drainage basin in the Makhtesh and above it from a direct influence of the terminal base level of the DSR. Thus, the accumulation of sediment and abandonment of terraces are controlled by climate and bedrock barriers located at the Makhtesh outlet. We use cosmogenic isotope concentrations to determine bedrock denudation rates, ages of alluvial terraces, and basin wide erosion rates in different channels throughout the basin. The use of cosmogenic isotopes enables us to determine sediment sources and reconstruct sedimentary cycles. OSL dating was used to determine the accumulation ages of alluvial sediment in alluvial terraces. These two methods enable quantitative evaluation of fluvial processes. Bedrock erosion rates suggest a strong dependence of erosion on lithology. While the Lower Cretaceous sandstone erodes at >100 mm ky-1, the overlying hard carbonate caprock yielded cosmogenic isotope concentrations that correspond to erosion rates of 1-3 mm ky-1. This significant difference in erosion rates maintains the dramatic relief of the Hazera drainage basin. We find that the quartz sediment in the present fluvial system of Makhtesh Hazera originates from two predominant sources. One is the Lower Cretaceous sandstone that crops out along the base of the Makhtesh cliffs. The second source are un consolidated Miocene sands that fill the syncline which is located north west of the Makhtesh and is drained into it. 10Be concentrations in successive samples indicate that the Miocene sand is gradually diluted by Lower Cretaceous sand as it flows down stream and the mixing of sediment from both sources is good. Alluvial terraces and bedrock units exposed inside the Makhtesh do not contribute a significant amount of sediment to the present drainage system. Three major alluvial terrace levels were identified. The highest terrace level (MKT0) was abandoned at 279±19 ky. This level probably covered most of the Makhtesh surface. The deposition of the two lower levels, MKT1 and MKT2 (which were abandoned at 160±6 and 47±9 ky, respectively), was confined to the present drainage system. Analysis of cosmogenic depth profiles from the terraces suggests significant recycling of sediment within the Mekhtesh. This is in contrast to the present system that lacks recycled sediment. We explain this difference by the fact that the terraces are the final product of a sedimentary cycle while the present drainage system presents a “snapshot” in time which does not represent the entire cycle only the present state of the system which is expressed by rapid incision and very little lateral migration.European Geosciences Unio

Lithologic Controls on Focused Erosion and Intraplate Earthquakes in the Eastern Tennessee Seismic Zone

We present a new geomorphic model for the intraplate eastern Tennessee seismic zone (ETSZ). Previous studies document that the Upper Tennessee drainage basin is in a transient state of adjustment to ~150 m of base level fall that occurred in the Late Miocene. Using quantitative geomorphology, we demonstrate that base level fall resulted in the erosion of ~3,500 km3 of highly erodibility rock in an ~70 km wide by ~350‐km‐long corridor in the Paleozoic fold‐thrust belt above the ETSZ. Models of modern incision rates show a NE‐SW trending swath of elevated erosion ~30 km southeast of the center of the ETSZ. Stress modeling shows that lithologically focused erosion has affected fault clamping stress on preexisting, favorably oriented faults. We argue that the lithologically controlled transient erosional response to base level fall in the Upper Tennessee basin has given rise to and is sustaining earthquake activity in the ETSZ

Dynamic landscapes and human dispersal patterns : tectonics, coastlines, and the reconstruction of human habitats

Studies of the impact of physical environment on human evolution usually focus on climate as the main external forcing agent of evolutionary and cultural change. In this paper we focus on changes in the physical character of the landscape driven by geophysical processes as an equally potent factor. Most of the landscapes where finds of early human fossils and artefacts are concentrated are ones that have been subjected to high levels of geological instability, either because of especially active tectonic processes associated with faulting and volcanic activity or because of proximity to coastlines subject to dramatic changes of geographical position and physical character by changes of relative sea level. These processes can have both beneficial effects, creating ecologically attractive conditions for human settlement, and deleterious or disruptive ones, creating barriers to movement, disruption of ecological conditions, or hazards to survival. Both positive and negative factors can have powerful selective effects on human behaviour and patterns of settlement and dispersal. We consider both these aspects of the interaction, develop a framework for the reconstruction and comparison of landscapes and landscape change at a variety of scales, and illustrate this with selected examples drawn from Africa and Arabia

Precise determination of low energy electronuclear Hamiltonian for LiY1−x_{1-x}Hox_{x}F4_{4}

We use complementary optical spectroscopy methods to directly measure the lowest crystal-field energies of the rare-earth quantum magnet LiY$_{1-x}$Ho$_{x}$F$_{4}$, including their hyperfine splittings, with more than 10 times higher resolution than previous work. We are able to observe energy level splittings due to the $^6\mathrm{Li}$ and $^7\mathrm{Li}$ isotopes, as well as non-equidistantly spaced hyperfine transitions originating from dipolar and quadrupolar hyperfine interactions. We provide refined crystal field parameters and extract the dipolar and quadrupolar hyperfine constants ${A_J=0.02703\pm0.00003}$ $\textrm{cm}^{-1}$ and ${B= 0.04 \pm0.01}$ $\textrm{cm}^{-1}$, respectively. Thereupon we determine all crystal-field energy levels and magnetic moments of the $^5I_8$ ground state manifold, including the (non-linear) hyperfine corrections. The latter match the measurement-based estimates. The scale of the non-linear hyperfine corrections sets an upper bound for the inhomogeneous line widths that would still allow for unique addressing of a selected hyperfine transition. e.g. for quantum information applications. Additionally, we establish the far-infrared, low-temperature refractive index of LiY$_{1-x}$Ho$_{x}$F$_{4}$.Comment: 9 pages, 6 Figures, 3 Table

Optical response from terahertz to visible light of electronuclear transitions in LiYF_4:Ho^(3+)

Because of its role as a model system with tunable quantum fluctuations and quenched disorder, and the desire for optical control and readout of its states, we have used high-resolution optical absorption spectroscopy to measure the crystal-field excitations for Ho^(3+) ions in LiHo_xY_(1−x)F_4 from the terahertz to visible regimes. We show that many of the excitations yield very narrow lines visibly split even by the nuclear hyperfine interaction, making Ho^(3+) in LiHo_xY_(1−x)F_4 a candidate host for optically addressable electronuclear qubits with quality factors as high as Q = 4.7 × 10^5, where the higher-lying levels are electronic singlets. Optical transitions in the easily accessible near- and mid-infrared are narrow enough to allow readout of the ground-state electronuclear qubits responsible for the interesting magnetism of LiHo_xY_(1−x)F_4. While many of the higher-lying states have been observed previously, we also report here detailed spectra of terahertz excitations. The strengths of the electric and magnetic dipole crystal-field transition lines of five of the lowest excited spin-orbit manifolds of dilute LiYF_4:Ho^(3+) were calculated and compared with measurement. The magnitude of the nuclear hyperfine coupling was used to assign the correct upper and lower states to transition lines