131 research outputs found
Monitoring surface resonances on Co2MnSi(100) by spin-resolved photoelectron spectroscopy
The magnitude of the spin polarization at the Fermi level of ferromagnetic
materials at room temperature is a key property for spintronics. Investigating
the Heusler compound CoMnSi a value of 93 for the spin polarization has
been observed at room temperature, where the high spin polarization is related
to a stable surface resonance in the majority band extending deep into the
bulk. In particular, we identified in our spectroscopical analysis that this
surface resonance is embedded in the bulk continuum with a strong coupling to
the majority bulk states. The resonance behaves very bulk-like, as it extends
over the first six atomic layers of the corresponding (001)-surface. Our study
includes experimental investigations, where the bulk electronic structure as
well as surface-related features have been investigated using spin-resolved
photoelectron spectroscopy (SR-UPS) and for a larger probing depth
spin-integrated high energy x-ray photoemission spectroscopy (HAXPES). The
results are interpreted in comparison with first-principles band structure and
photoemission calculations which consider all relativistic, surface and
high-energy effects properly.Comment: 9 pages, 8 figures, Heusler alloy, electronic structure and
photoemissio
Observation and theoretical description of the pure Fano-effect in the valence-band photo-emission of ferromagnets
The pure Fano-effect in angle-integrated valence-band photo-emission of
ferromagnets has been observed for the first time. A contribution of the
intrinsic spin polarization to the spin polarization of the photo-electrons has
been avoided by an appropriate choice of the experimental parameters. The
theoretical description of the resulting spectra reveals a complete analogy to
the Fano-effect observed before for paramagnetic transition metals. While the
theoretical photo-current and spin difference spectra are found in good
quantitative agreement with experiment in the case of Fe and Co only a
qualitative agreement could be achieved in the case of Ni by calculations on
the basis of plain local spin density approximation (LSDA). Agreement with
experimental data could be improved in this case in a very substantial way by a
treatment of correlation effects on the basis of dynamical mean field theory
(DMFT).Comment: 11 pages, 3 figures accepted by PR
Orbital magnetism in transition-metal systems: The role of local correlation effects
The influence of correlation effects on the orbital moments for transition
metals and their alloys is studied by first-principle relativistic Density
Functional Theory in combination with the Dynamical Mean-Field Theory. In
contrast to the previous studies based on the orbital polarization corrections
we obtain an improved description of the orbital moments for wide range of
studied systems as bulk Fe, Co and Ni, Fe-Co disordered alloys and 3
impurities in Au. The proposed scheme can give simultaneously a correct
dynamical description of the spectral function as well as static magnetic
properties of correlated disordered metals.Comment: EPL accepte
Momentum resolved spin dynamics of bulk and surface excited states in the topological insulator
The prospective of optically inducing a spin polarized current for spintronic
devices has generated a vast interest in the out-of-equilibrium electronic and
spin structure of topological insulators (TIs). In this Letter we prove that
only by measuring the spin intensity signal over several order of magnitude in
spin, time and angle resolved photoemission spectroscopy (STAR-PES) experiments
is it possible to comprehensively describe the optically excited electronic
states in TIs materials. The experiments performed on
reveal the existence of a Surface-Resonance-State in the 2nd bulk band gap
interpreted on the basis of fully relativistic ab-initio spin resolved
photoemission calculations. Remarkably, the spin dependent relaxation of the
hot carriers is well reproduced by a spin dynamics model considering two
non-interacting electronic systems, derived from the excited surface and bulk
states, with different electronic temperatures.Comment: 5 pages and 4 figure
Effect of chemical disorder on NiMnSb investigated by Appearance Potential Spectroscopy: a theoretical study
The half-Heusler alloy NiMnSb is one of the local-moment ferromagnets with
unique properties for future applications. Band structure calculations predict
exclusively majority bands at the Fermi level, thus indicating {100%} spin
polarization there. As one thinks about applications and the design of
functional materials, the influence of chemical disorder in these materials
must be considered. The magnetization, spin polarization, and electronic
structure are expected to be sensitive to structural and stoichiometric
changes. In this contribution, we report on an investigation of the
spin-dependent electronic structure of NiMnSb. We studied the influence of
chemical disorder on the unoccupied electronic density of states by use of the
ab-initio Coherent Potential Approximation method. The theoretical analysis is
discussed along with corresponding spin-resolved Appearance Potential
Spectroscopy measurements. Our theoretical approach describes the spectra as
the fully-relativistic self-convolution of the matrix-element weighted,
orbitally resolved density of states.Comment: JPD submitte
Geometry-induced spin-filtering in photoemission maps from WTe surface states
We demonstrate that an important quantum material WTe exhibits a new type
of geometry-induced spin-filtering effect in photoemission, stemming from low
symmetry that is responsible for its exotic transport properties. Through the
laser-driven spin-polarized angle-resolved photoemission Fermi surface mapping,
we showcase highly asymmetric spin textures of electrons photoemitted from the
surface states of WTe. Such asymmetries are not present in the initial
state spin textures, which are bound by the time-reversal and crystal lattice
mirror plane symmetries. The findings are reproduced qualitatively by
theoretical modeling within the one-step model photoemission formalism. The
effect could be understood within the free-electron final state model as an
interference due to emission from different atomic sites. The observed effect
is a manifestation of time-reversal symmetry breaking of the initial state in
the photoemission process, and as such it cannot be eliminated, but only its
magnitude influenced, by special experimental geometries.Comment: 5 pages, 3 figure
Photoemission of BiSe with Circularly Polarized Light: Probe of Spin Polarization or Means for Spin Manipulation?
Topological insulators are characterized by Dirac cone surface states with
electron spins aligned in the surface plane and perpendicular to their momenta.
Recent theoretical and experimental work implied that this specific spin
texture should enable control of photoelectron spins by circularly polarized
light. However, these reports questioned the so far accepted interpretation of
spin-resolved photoelectron spectroscopy. We solve this puzzle and show that
vacuum ultraviolet photons (50-70 eV) with linear or circular polarization
probe indeed the initial state spin texture of BiSe while circularly
polarized 6 eV low energy photons flip the electron spins out of plane and
reverse their spin polarization. Our photoemission calculations, considering
the interplay between the varying probing depth, dipole selection rules and
spin-dependent scattering effects involving initial and final states explain
these findings, and reveal proper conditions for light-induced spin
manipulation. This paves the way for future applications of topological
insulators in opto-spintronic devices.Comment: Submitted for publication (2013
Correlation effects in total energy of transition metals and related properties
We present an accurate implementation of total energy calculations into the
local density approximation plus dynamical mean-field theory (LDA+DMFT) method.
The electronic structure problem is solved through the full potential linear
Muffin-Tin Orbital (FP-LMTO) and Korringa-Kohn-Rostoker (FP-KKR) methods with a
perturbative solver for the effective impurity suitable for moderately
correlated systems. We have tested the method in detail for the case of Ni and
investigated the sensitivity of the results to the computational scheme and to
the complete self-consistency. It is demonstrated that the LDA+DMFT method can
resolve a long-standing controversy between the LDA/GGA density functional
approach and experiment for equilibrium lattice constant and bulk modulus of
Mn.Comment: 14 pages, 5 figure
Rashba-type spin splitting at Au(111) beyond the Fermi level: the other part of the story
We present a combined experimental and theoretical study of spin–orbit-induced spin splittings in the unoccupied surface electronic structure of the prototypical Rashba system Au(111). Spin- and angle-resolved inverse-photoemission measurements reveal a Rashba-type spin splitting in the unoccupied part of the L-gap surface state. With increasing momentum parallel to the surface, the spectral intensity is lowered and the spin splitting vanishes as the surface state approaches the band-gap boundary. Furthermore, we observe significantly spin-dependent peak positions and intensities for transitions between unoccupied sp-like bulk bands. Possible reasons for this behavior are considered: initial and final-state effects as well as the transition itself, which is controlled by selection rules depending on the symmetry of the involved states. Based on model calculations, we identify the initial states as origin of the observed Rashba-type spin effects in bulk transitions
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