62,685 research outputs found
Stability boundaries of roll and square convection in binary fluid mixtures with positive separation ratio
Rayleigh-B\'{e}nard convection in horizontal layers of binary fluid mixtures
heated from below with realistic horizontal boundary conditions is studied
theoretically using multi-mode Galerkin expansions. For positive separation
ratios the main difference between the mixtures and pure fluids lies in the
existence of stable three dimensional patterns near onset in a wide range of
the parameter space. We evaluated the stationary solutions of roll, crossroll,
and square convection and we determined the location of the stability
boundaries for many parameter combinations thereby obtaining the Busse balloon
for roll and square patterns.Comment: 19 pages + 15 figures, accepted by Journal of Fluid Mechanic
The role of ferroelectric-ferromagnetic layers on the properties of superlattice-based multiferroics
A series of superlattices and trilayers composed of ferromagnetic and
ferroelectric or paraelectric layers were grown on (100) SrTiO3 by the pulsed
laser deposition technique. Their structural and magneto-electric properties
were examined. The superlattices made of ferromagnetic Pr0.85Ca0.15MnO3 (PCMO)
and a ferroelectric, namely Ba0.6Sr0.4TiO3 (BST) or BaTiO3, showed enhanced
magnetoresistance (MR) at high applied magnetic field, whereas such enhancement
was absent in Pr0.85Ca0.15MnO3/SrTiO3 superlattices, which clearly demonstrates
the preponderant role of the ferroelectric layers in this enhanced MR.
Furthermore, the absence of enhanced MR in trilayers of PCMO/BST indicates that
the magneto-electric coupling which is responsible for MR in these systems is
stronger in multilayers than in their trilayer counterparts.Comment: to be published in J. Appl. Phy
Magnetocapacitance effect in perovskite-superlattice based multiferroics
We report the structural and magnetoelectrical properties of
LaCaMnO/BaTiO perovskite superlattices grown on
(001)-oriented SrTiO by the pulsed laser deposition technique. Magnetic
hysteresis loops together with temperature dependent magnetic properties
exhibit well-defined coercivity and magnetic transition temperature (T)
\symbol{126}140 K. electrical studies of films show that the
magnetoresistance (MR) is dependent on the BaTiO thickness and negative
as high as 30% at 100K are observed. The electrical studies reveal
that the impedance and capacitance in these films vary with the applied
magnetic field due to the magnetoelectrical coupling in these structures - a
key feature of multiferroics. A negative magnetocapacitance value in the film
as high as 3% per tesla at 1kHz and 100K is demonstrated, opening the route for
designing novel functional materials.Comment: To be published in Applied Physics Letter
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Operando STM study of the interaction of imidazolium-based ionic liquid with graphite
Understanding interactions at the interfaces of carbon with ionic liquids (ILs) is crucially beneficial for the diagnostics and performance improvement of electrochemical devices containing carbon as active materials or conductive additives in electrodes and ILs as solvents or additives in electrolytes. The interfacial interactions of three typical imidazolium-based ILs, 1-alkyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide (AMImTFSI) ILs having ethyl (C2), butyl (C4) and octyl (C8) chains in their cations, with highly oriented pyrolytic graphite (HOPG) were studied in-situ by electrochemical scanning tunneling microscopy (EC-STM). The etching of HOPG surface and the exfoliation of graphite/graphene flakes as well as cation intercalation were observed at the HOPG/C2MImTFSI interface. The etching also takes place in C4MImTFSI at −1.5 V vs Pt but only at step edges with a much slower rate, whereas C8MIm+ cations adsorbs strongly on the HOPG surface under similar conditions with no observable etching or intercalation. The EC-STM observations can be explained by the increase in van der Waals interaction between the cations and the graphite surface with increasing length of alkyl chains
Inclusion Matrices and Chains
Given integers , , and such that , let
be the inclusion matrix of -subsets vs. -subsets of a
-set. We modify slightly the concept of standard tableau to study the notion
of rank of a finite set of positive integers which was introduced by Frankl.
Utilizing this, a decomposition of the poset into symmetric skipless
chains is given. Based on this decomposition, we construct an inclusion matrix,
denoted by , which is row-equivalent to . Its Smith
normal form is determined. As applications, Wilson's diagonal form of
is obtained as well as a new proof of the well known theorem on the
necessary and sufficient conditions for existence of integral solutions of the
system due to Wilson. Finally we present anotherinclusion
matrix with similar properties to those of which is in some
way equivalent to .Comment: Accepted for publication in Journal of Combinatorial Theory, Series
Correlation between structure and properties in multiferroic LaCaMnO/BaTiO superlattices
Superlattices composed of ferromagnetics, namely LaCaMnO
(LCMO), and ferroelectrics, namely, BaTiO(BTO) were grown on SrTiO at
720C by pulsed laser deposition process. While the out-of-plane lattice
parameters of the superlattices, as extracted from the X-ray diffraction
studies, were found to be dependent on the BTO layer thickness, the in-plane
lattice parameter is almost constant. The evolution of the strains, their
nature, and their distribution in the samples, were examined by the
conventional sin method. The effects of structural variation on the
physical properties, as well as the possible role of the strain on inducing the
multiferroism in the superlattices, have also been discussed.Comment: To be published in Journal of Applied Physic
Ionisation and discharge in cloud-forming atmospheres of brown dwarfs and extrasolar planets
Brown dwarfs and giant gas extrasolar planets have cold atmospheres with rich chemical compositions from which mineral cloud particles form. Their properties, like particle sizes and material composition, vary with height, and the mineral cloud particles are charged due to triboelectric processes in such dynamic atmospheres. The dynamics of the atmospheric gas is driven by the irradiating host star and/or by the rotation of the objects that changes during its lifetime. Thermal gas ionisation in these ultra-cool but dense atmospheres allows electrostatic interactions and magnetic coupling of a substantial atmosphere volume. Combined with a strong magnetic field , a chromosphere and aurorae might form as suggested by radio and x-ray observations of brown dwarfs. Non-equilibrium processes like cosmic ray ionisation and discharge processes in clouds will increase the local pool of free electrons in the gas. Cosmic rays and lighting discharges also alter the composition of the local atmospheric gas such that tracer molecules might be identified. Cosmic rays affect the atmosphere through air showers in a certain volume which was modelled with a 3D Monte Carlo radiative transfer code to be able to visualise their spacial extent. Given a certain degree of thermal ionisation of the atmospheric gas, we suggest that electron attachment to charge mineral cloud particles is too inefficient to cause an electrostatic disruption of the cloud particles. Cloud particles will therefore not be destroyed by Coulomb explosion for the local temperature in the collisional dominated brown dwarf and giant gas planet atmospheres. However, the cloud particles are destroyed electrostatically in regions with strong gas ionisation. The potential size of such cloud holes would, however, be too small and might occur too far inside the cloud to mimic the effect of, e.g. magnetic field induced star spots
Comment on `Universal relation between the Kolmogorov-Sinai entropy and the thermodynamic entropy in simple liquids'
The intriguing relations between Kolmogorov-Sinai entropy and self diffusion
coefficients and the excess (thermodynamic) entropy found by Dzugutov and
collaborators do not appear to hold for hard sphere and hard disks systems.Comment: 1 page revte
A metal–organic framework/α-alumina composite with a novel geometry for enhanced adsorptive separation
The development of a metal–organic framework/α-alumina composite leads to a novel concept: efficient adsorption occurs within a plurality of radial micro-channels with no loss of the active adsorbents during the process. This composite can effectively remediate arsenic contaminated water producing potable water recovery, whereas the conventional fixed bed requires eight times the amount of active adsorbents to achieve a similar performance
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