107 research outputs found

    Impact of ex-situ rapid thermal annealing on the magneto-optical properties and the oscillator strength of In(Ga)As quantum dots

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    The authors acknowledge financial support by the State of Bavaria and the German Ministry of Education and Research (BMBF) within the project Q.com-HL.We discuss the influence of a rapid thermal annealing step on the magneto-optical emission properties of In(Ga)As/GaAs quantum dots. We map out a strong influence of the growth- and anneling parameters on the quantum excitons' effective Land\'e g-factors and in particular on their diamagnetic coefficients, which we directly correlate with the modification of the emitters shape and material composition. In addition, we study the excitons' spontaneous emission lifetime as a function of the annealing temperature and the dot height, and observe a strong increase of the emission rate with the quantum dot volume. The corresponding increase in oscillator strenth yields fully consistent results with the analysis of the diamagenic behavior. In particular, we demonstrate that a rapid thermal annealing step of 850ÂşC can be employed to increase the oscillator strength of as-grown InAs/GaAs QDs by more than a factor of 2.PostprintPeer reviewe

    Monolayered MoSe2: a candidate for room temperature polaritonics

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    We acknowledge financial support by the state of Bavaria. EC, AK and SH acknowledge the EPSRC Programme "Hybrid Polaritonics" (EP/M025330/1) for support. ST acknowledges support from NSF DMR-1552220. CS acknowledges support by the European Research Council within the project UnLiMIt-2D (grant number 679288).Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying excitonic transition, the so-called A-valley exciton, with temperature. We find a strong, phonon-induced temperature broadening of the resonance, and more importantly, a reduction of the oscillator strength for increased temperatures, which we describe in the framework of a microscopic model. Based on these experimentally extracted, temperature dependent parameters, we apply a coupled oscillator model to elucidate the possibility to observe the strong coupling regime between the A-exciton and a microcavity resonance in three prototypical photonic architectures with varying mode volumes. We find that the formation of exciton-polaritons up to ambient conditions in compact, monolithic dielectric and Tamm-based structures seems feasible. In contrast, a temperature-induced transition into the weak coupling regime can be expected for structures with extended effective cavity length. Based on these findings, we calculate and draw the phase diagram of polariton Bosonic condensation in a microcavity with embedded MoSe2 monolayers.PostprintPeer reviewe

    Observation of macroscopic valley-polarized monolayer exciton-polaritons at room temperature

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    Funding: the State of Bavaria and the ERC (unlimit-2D), the DFG via SFB689, GRK 1570 and KO3612/1-1.In this Rapid Communication, we address the chiral properties of valley exciton-polaritons in a monolayer of WS2 in the regime of strong light-matter coupling with a Tamm-plasmon resonance. We observe that the effect of valley polarization, which manifests in the circular polarization of the emitted photoluminescence as the sample is driven by a circularly polarized laser, is strongly enhanced in comparison to bare WS2 monolayers and can even be observed under strongly nonresonant excitation at ambient conditions. In order to explain this effect in more detail, we study the relaxation and decay dynamics of exciton-polaritons in our device, elaborate the role of the dark state, and present a microscopic model to explain the wave-vector-dependent valley depolarization by the linear polarization splitting inherent to the microcavity. We believe that our findings are crucial for designing novel polariton-valleytronic devices which can be operated at room temperature.PostprintPeer reviewe

    Single and Multi-Person Face Recognition Using the Enhanced Eigenfaces Method

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    This research studies and analyzes the possibility of single-person and multi-person face detection and recognition. Face detection is performed by the Viola-Jones face detection method and recognition is performed by the Eigenfaces method. Unchanged face detection and recognition methods are explained and tested to their limits. Improvement in face recognition is achieved by observing the flaws of the Eigenfaces method and their enhancement

    Valley polarized relaxation and upconversion luminescence from Tamm-plasmon trion-polaritons with a MoSe2 monolayer

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    This work has been supported by the State of Bavaria and the ERC (unlimit-2D) as well as the DFG via grants GRK 1570, KO3612/1-1 and SFB 689.Transition metal dichalcogenides represent an ideal testbed to study excitonic effects, spin-related phenomena and fundamental light-matter coupling in nanoscopic condensed matter systems. In particular, the valley degree of freedom, which is unique to such direct band gap monolayers with broken inversion symmetry, adds fundamental interest in these materials. Here, we implement a Tamm-plasmon structure with an embedded MoSe2 monolayer and study the formation of polaritonic quasi-particles. Strong coupling conditions between the Tamm-mode and the trion resonance of MoSe2 are established, yielding bright luminescence from the polaritonic ground state under non-resonant optical excitation. We demonstrate, that tailoring the electrodynamic environment of the monolayer results in a significantly increased valley polarization. This enhancement can be related to change in recombination dynamics shown in time-resolved photoluminescence measurements. We furthermore observe strong upconversion luminescence from resonantly excited polariton states in the lower polariton branch. This upconverted polariton luminescence is shown to preserve the valley polarization of the trion–polariton, which paves the way towards combining spin-valley physics and exciton scattering experiments.PostprintPeer reviewe

    Magnetic-field-induced splitting and polarization of monolayer-based valley exciton polaritons

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    he Würzburg group acknowledges support by the state of Bavaria. C.S. acknowledges support by the European Research council (ERC) under the European Union's Horizon 2020 Research and Innovation Programme (UnLiMIt-2D), Grant Agreement No. 679288. This work has been supported by the Fraunhofer-Gesellschaft zur Föderung der angewandten Forschung e.V. F.E. and H.K. gratefully acknowledge the financial support by the German Federal Ministry of Education and Research under Grant No. 13XP5053A. E.S. acknowledges support from the Grant of the President of the Russian Federation for state support of Young Russian Scientists, Grant No. MK-2839.2019.2 and RFBR Grant No. 17-52-10006. The work of A.K. is supported by Westlake University (Project No. 041020100118). S.T. acknowledges support from NSF, Grant No. DMR-1838443.Atomically thin crystals of transition metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization, and magnetic field effects. In this work, we investigate the formation of exciton-polaritons in a MoSe2 monolayer, which is integrated in a fully-grown, monolithic microcavity. Due to the narrow linewidth of the polaritonic resonances, we are able to directly investigate the emerging valley Zeeman splitting of the hybrid light-matter resonances in the presence of a magnetic field. At a detuning of -54.5 meV (13.5 % matter constituent of the lowerpolariton branch), we find a Zeeman splitting of the lower polariton branch of 0.36 meV, which can be directly associated with an excitonic g factor of 3.94±0.13. Remarkably, we find that a magnetic field of 6 T is suffcient to induce a notable valley polarization of 15 % in our polariton system, which approaches 30% at 9 T. This circular polarization degree of the polariton (ground) state exceeds the polarization of the exciton reservoir for equal magnetic field magnitudes by approximately 50%, which is a clear hint of valley-dependent bosonic stimulation in our strongly coupled system in the sub-threshold, fluctuation dominated regime.PostprintPeer reviewe

    Valley coherent exciton-polaritons in a monolayer semiconductor

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    Two-dimensional transition metal dichalcogenides (TMDs) provide a unique possibility to generate and read-out excitonic valley coherence using linearly polarized light, opening the way to valley information transfer between distant systems. However, these excitons have short lifetimes (ps) and efficiently lose their valley coherence via the electron-hole exchange interaction. Here, we show that control of these processes can be gained by embedding a monolayer of WSe2 in an optical microcavity, forming part-light-part-matter exciton-polaritons. We demonstrate optical initialization of valley coherent polariton populations, exhibiting luminescence with a linear polarization degree up to 3 times higher than displayed by bare excitons. We utilize an external magnetic field alongside selective exciton-cavity-mode detuning to control the polariton valley pseudospin vector rotation, which reaches 45° at B = 8 T. This work provides unique insight into the decoherence mechanisms in TMDs and demonstrates the potential for engineering the valley pseudospin dynamics in monolayer semiconductors embedded in photonic structures

    Cutaneous lesions of the nose

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    Skin diseases on the nose are seen in a variety of medical disciplines. Dermatologists, otorhinolaryngologists, general practitioners and general plastic and dermatologic surgeons are regularly consulted regarding cutaneous lesions on the nose. This article is the second part of a review series dealing with cutaneous lesions on the head and face, which are frequently seen in daily practice by a dermatologic surgeon. In this review, we focus on those skin diseases on the nose where surgery or laser therapy is considered a possible treatment option or that can be surgically evaluated

    Valley-addressable polaritons in atomically thin semiconductors

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    The locking of the electron spin to the valley degree of freedom in transition metal dichalcogenide (TMD) monolayers has seen these materials emerge as a promising platform in valleytronics. When embedded in optical microcavities, the large oscillator strengths of excitonic transitions in TMDs allow the formation of polaritons that are part-light part-matter quasiparticles. Here, we report that polaritons in MoSe2 show an efficient retention of the valley pseudospin contrasting them with excitons and trions in this material. We find that the degree of the valley pseudospin retention is dependent on the photon, exciton and trion fractions in the polariton states. This allows us to conclude that in the polaritonic regime, cavity-modified exciton relaxation inhibits loss of the valley pseudospin. The valley-addressable exciton-polaritons and trion-polaritons presented here offer robust valley-polarized states with the potential for valleytronic devices based on TMDs embedded in photonic structures and valley-dependent nonlinear polariton–polariton interactions
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