1,084 research outputs found

    Thermodynamic quantum critical behavior of the Kondo necklace model

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    We obtain the phase diagram and thermodynamic behavior of the Kondo necklace model for arbitrary dimensions dd using a representation for the localized and conduction electrons in terms of local Kondo singlet and triplet operators. A decoupling scheme on the double time Green's functions yields the dispersion relation for the excitations of the system. We show that in d3d\geq 3 there is an antiferromagnetically ordered state at finite temperatures terminating at a quantum critical point (QCP). In 2-d, long range magnetic order occurs only at T=0. The line of Neel transitions for d>2d>2 varies with the distance to the quantum critical point QCP g|g| as, TNgψT_N \propto |g|^{\psi} where the shift exponent ψ=1/(d1)\psi=1/(d-1). In the paramagnetic side of the phase diagram, the spin gap behaves as Δg\Delta\approx \sqrt{|g|} for d3d \ge 3 consistent with the value z=1z=1 found for the dynamical critical exponent. We also find in this region a power law temperature dependence in the specific heat for kBTΔk_BT\gg\Delta and along the non-Fermi liquid trajectory. For kBTΔk_BT \ll\Delta, in the so-called Kondo spin liquid phase, the thermodynamic behavior is dominated by an exponential temperature dependence.Comment: Submitted to PR

    Algorithms For Extracting Timeliness Graphs

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    We consider asynchronous message-passing systems in which some links are timely and processes may crash. Each run defines a timeliness graph among correct processes: (p; q) is an edge of the timeliness graph if the link from p to q is timely (that is, there is bound on communication delays from p to q). The main goal of this paper is to approximate this timeliness graph by graphs having some properties (such as being trees, rings, ...). Given a family S of graphs, for runs such that the timeliness graph contains at least one graph in S then using an extraction algorithm, each correct process has to converge to the same graph in S that is, in a precise sense, an approximation of the timeliness graph of the run. For example, if the timeliness graph contains a ring, then using an extraction algorithm, all correct processes eventually converge to the same ring and in this ring all nodes will be correct processes and all links will be timely. We first present a general extraction algorithm and then a more specific extraction algorithm that is communication efficient (i.e., eventually all the messages of the extraction algorithm use only links of the extracted graph)

    Implementing the weakest failure detector for solving consensus

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    The concept of unreliable failure detector was introduced by Chandra and Toueg as a mechanism that provides information about process failures. This mechanism has been used to solve several agreement problems, such as the consensus problem. In this paper, algorithms that implement failure detectors in partially synchronous systems are presented. First two simple algorithms of the weakest class to solve the consensus problem, namely the Eventually Strong class (⋄S), are presented. While the first algorithm is wait-free, the second algorithm is f-resilient, where f is a known upper bound on the number of faulty processes. Both algorithms guarantee that, eventually, all the correct processes agree permanently on a common correct process, i.e. they also implement a failure detector of the class Omega (Ω). They are also shown to be optimal in terms of the number of communication links used forever. Additionally, a wait-free algorithm that implements a failure detector of the Eventually Perfect class (⋄P) is presented. This algorithm is shown to be optimal in terms of the number of bidirectional links used forever

    Microfluidic Continuous Approaches to Produce Magnetic Nanoparticles with Homogeneous Size Distribution

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    We present a gas-liquid microfluidic system as a reactor to obtain magnetite nanoparticles with an excellent degree of control regarding their crystalline phase, shape and size. Several types of microflow approaches were selected to prevent nanomaterial aggregation and to promote homogenous size distribution. The selected reactor consists of a mixer stage aided by ultrasound waves and a reaction stage using a N2-liquid segmented flow to prevent magnetite oxidation to non-magnetic phases. A milli-fluidic reactor was developed to increase the production rate where a magnetite throughput close to 450 mg/h in a continuous fashion was obtained

    Gas Slug Microfluidics: A Unique Tool for Ultrafast, Highly Controlled Growth of Iron Oxide Nanostructures

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    The use of nanomaterials in real life applications is often hampered by our inability to produce them in large quantities while preserving their desired properties in terms of size, shape, and crystalline phase. Here we present a novel continuous method to synthesize nanostructures with an unprecedented degree of control regarding their properties. In particular, the excellent properties of microreactors for chemical synthesis are enhanced by the introduction of gas slugs of tailored composition. Slug dynamics accelerate mixing, reduce processing times (from hours in batch processes to minutes or even seconds), and, depending on the gas atmosphere used, allows one to accurately control the crystalline phase and shape of the resulting nanostructures. Inert (N2), oxidizing (O2), or reducing (CO, H2) gases were used, leading to different morphologies and crystalline structures in a high yield, highly reproducible fabrication process

    Phase Transition Study of Superconducting Microstructures

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    The presented results are part of a feasibility study of superheated superconducting microstructure detectors. The microstructures (dots) were fabricated using thin film patterning techniques with diameters ranging from 50μ50\mum up to 500μ500\mum and thickness of 1μ1\mum. We used arrays and single dots to study the dynamics of the superheating and supercooling phase transitions in a magnetic field parallel to the dot surface. The phase transi- tions were produced by either varying the applied magnetic field strength at a constant temperature or changing the bath temperature at a constant field. Preliminary results on the dynamics of the phase transitions of arrays and single indium dots will be reported.Comment: 7pages in LaTex format, five figures available upon request by [email protected], preprint Bu-He 93/

    Petrology and structure of Campanario-La Haba pluton and Los Berrocales stock (Badajoz): preliminary dates

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    [Abstract] The Campanario-La Haba pluton and Los Berrocales stock are situated in the southern part ofthe Central-Iberian zone. They form part ofthe late-Hercynian alignement named Caceres-Linares or Pedroches-Alburquerque. During the last years these two granitoids have been related, based on spatial and/or genetic criteria, with Los Pedroches Batholith. These igneous bodies are different. Campanario-La Haba pluton is a coarse grained peraluminous granite with large megaphenocrysts ofcordierite. Three facies are differenciated based on petrographic criteria: coarse grained porfiric granite with megaphenocryst of cordierite, fine grained porfiric granite with megaphenocryst of cordierire and fine-medium granite. Los Berrocales is a zoned stock formed by granodiorites graded to granites in the center. Structure-studies indicates that the Campanario-La Haba pluton has been structurated in magmatic state. The magmatic foliation and lineation direction show the orientation ofN12üE, parallel to the pluton lenghtening. The magnetic susceptibility values show that the magnetic behaviour of the granites is dominated by paramagnetic minerals, fine for apply the Anisotropy ofthe Magnetic Susceptibility. The magnetic structure is rather homogeneous and the magnetic lineation and foliation show the N12üE direction. This paper shows premier dates and conclusions of the work that Mineralogy and Petrology department (University of Basque Country) has being done in conjunction with the Geodinamic department (University ofBasque Country) on the westhern end of the Los Pedroches Batholith

    Identification of two conserved aspartic acid residues required for DNA digestion by a novel thermophilic Exonuclease VII in Thermotoga maritima

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    Exonuclease VII was first identified in 1974 as a DNA exonuclease that did not require any divalent cations for activity. Indeed, Escherichia coli ExoVII was identified in partially purified extracts in the presence of EDTA. ExoVII is comprised of two subunits (XseA and XseB) that are highly conserved and present in most sequenced prokaryotic genomes, but are not seen in eukaryotes. To better understand this exonuclease family, we have characterized an ExoVII homolog from Thermotoga maritima. Thermotoga maritima XseA/B homologs TM1768 and TM1769 were co-expressed and purified, and show robust nuclease activity at 80°C. This activity is magnesium dependent and is inhibited by phosphate ions, which distinguish it from E. coli ExoVII. Nevertheless, both E. coli and T. maritima ExoVII share a similar putative active site motif with two conserved aspartate residues in the large (XseA/TM1768) subunit. We show that these residues, Asp235 and Asp240, are essential for the nuclease activity of T. maritima ExoVII. We hypothesize that the ExoVII family of nucleases can be sub-divided into two sub-families based on EDTA resistance and that T. maritima ExoVII is the first member of the branch that is characterized by EDTA sensitivity and inhibition by phosphate

    Sequential localization of a complex electron fluid

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    Complex and correlated quantum systems with promise for new functionality often involve entwined electronic degrees of freedom. In such materials, highly unusual properties emerge and could be the result of electron localization. Here, a cubic heavy fermion metal governed by spins and orbitals is chosen as a model system for this physics. Its properties are found to originate from surprisingly simple low-energy behavior, with two distinct localization transitions driven by a single degree of freedom at a time. This result is unexpected, but we are able to understand it by advancing the notion of sequential destruction of an SU(4) spin-orbital-coupled Kondo entanglement. Our results implicate electron localization as a unified framework for strongly correlated materials and suggest ways to exploit multiple degrees of freedom for quantum engineering.Comment: 21 pages, 4 figures (preprint format
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