23 research outputs found

    Electronic structure and transport properties of CeNi9In2

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    We investigated CeNi9In2 compound, which has been considered as a mixed valence (MV) system. Electrical resistivity vs. temperature variation was analysed in terms of the model proposed by Freimuth for systems with unstable 4f shell. At low temperature the resistivity dependence is consistent with a Fermi liquid state with a contribution characteristic of electron-phonon interaction. Ultraviolet photoemission spectroscopy (UPS) studies of the valence band did not reveal a Kondo peak down to 14 K. A difference of the spectra obtained with photon energies of low and high photoionization cross sections for Ce 4f electrons indicated that 4f states are located mainly close to the Fermi energy. The peaks related to f_{5/2}^1 and f_{7/2}^1 final states cannot be resolved but form a plateau between -0.3 eV and the Fermi energy. X-ray photoemission spectroscopy (XPS) studies were realized for the cerium 3d level. The analysis of XPS spectra within the Gunnarsson-Sh\"onhammer theory yielded a hybridization parameter of 104 meV and non-integer f level occupation, being close to 3. Calculations of partial densities of states were realized by a full potential local orbital (FPLO) method. They confirm that the valence band is dominated by Ni 3d states and are in general agreement with the experiment except for the behavior of f-electrons.Comment: 10 pages, 5 figure

    Evidence of momentum dependent hybridization in Ce2Co0.8Si3.2

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    We studied the electronic structure of the Kondo lattice system Ce2Co0.8Si3.2 by angle-resolved photoemission spectroscopy (ARPES). The spectra obtained below the coherence temperature consist of a Kondo resonance, its spin-orbit partner and a number of dispersing bands. The quasiparticle weight related to the Kondo peak depends strongly on Fermi vectors associated with bulk bands. This indicates a highly anisotropic hybridization between conduction band and 4f electrons - V_{cf} in Ce2Co0.8Si3.2.Comment: 6 page

    Electronic structure of TmPdIn

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    Electronic structure of a ternary TmPdIn compound, which crystallizes in the hexagonal ZrNiAl-type structure, was studied by X-ray photoemission spectroscopy and ultraviolet photoemission spectroscopy. Density of states in the valence band was calculated by means of the augmented plane wave/local orbital method based on density functional theory. The results showed that the valence band is formed mainly of Tm 4f and Pd 4d states. In the ultraviolet photoemission spectra one can distinguish Pd 4d maximum and Tm 4f multiplet peaks, which are displaced with respect to those of pure Tm

    Lifetime of quasi-particles in the nearly-free electron metal Sodium

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    We report a high-resolution angle-resolved photoemission (ARPES) study of the prototypical nearly-free-electron metal sodium. The observed mass enhancement is slightly smaller than that derived in previous studies. The new results on the lifetime broadening increase the demand for theories beyond the random phase approximation. Our results do not support the proposed strong enhancement of the scattering rates of the charge carriers due to a coupling to spin fluctuations. Moreover, a comparison with earlier electron energy-loss data on sodium yields a strong reduction of the mass enhancement of dipolar electron-hole excitations compared to that of monopole hole excitations, measured by ARPES.Comment: 5 pages, 6 figure

    Linkage between scattering rates and superconductivity in doped ferropnictides

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    We report an angle-resolved photoemission study of a series of hole- and electron-doped iron-based superconductors, their parent compound BaFe2_{2}As2_{2}, and their cousins BaCr2_{2}As2_{2} and BaCo2_{2}As2_{2}. We focus on the inner hole pocket, which is the hot spot in these compounds. More specifically, we determine the energy (E)-dependent scattering rate (E) as a function of the 3d count. Moreover, for the compounds K0.4_{0.4}Ba0.6_{0.6}Fe2_{2}As2_{2} and BaCr2_{2}As2_{2}, we derive the energy dependence of the renormalization function Z(E) and the imaginary part of the self-energy function Im(E). We obtain a non-Fermi liquidlike linear in energy scattering rate (E>>kB_{B}T ), independent of the dopant concentration. The main result is that the slope β = (E>>kB_{B}T )/E reaches its maxima near optimal doping and scales with the superconducting transition temperature. This supports the spin fluctuation model for superconductivity for these materials. In the optimally hole-doped compound, the slope of the scattering rate of the inner hole pocket is about three times bigger than the Planckian limit T(E)/E ≈ 1. This result, together with the energy dependence of the renormalization function Z(E), signals very incoherent charge carriers in the normal state which transform at low temperatures to a coherent unconventional superconducting state

    Topological magnetic order and superconductivity in EuRbFe4As4

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    We study single crystals of the magnetic superconductor EuRbFe4As4 by magnetization, electron spin resonance ESR , angle resolved photoemission spectroscopy, and electrical resistance in pulsed magnetic fields up to 63 T. The superconducting state below 36.5 K is almost isotropic and is only weakly affected by the development of Eu2 magnetic order at 15 K. On the other hand, for the external magnetic field applied along the c axis the temperature dependence of the ESR linewidth reveals a Berezinskii Kosterlitz Thouless topological transition below 15 K. This indicates that Eu2 planes are a good realization of a two dimensional XY magnet, which reflects the decoupling of the Eu2 magnetic moments from superconducting FeAs layer

    Lifetime of quasiparticles in the nearly free electron metal sodium

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    We report a high resolution angle resolved photoemission ARPES study of the prototypical nearly free electron metal sodium. The observed mass enhancement is slightly smaller than that derived in previous studies. The new results on the lifetime broadening increase the demand for theories beyond the random phase approximation. Our results do not support the proposed strong enhancement of the scattering rates of the charge carriers due to a coupling to spin fluctuations. Moreover, a comparison with earlier electron energy loss data on sodium yields a strong reduction of the mass enhancement of dipolar electron hole excitations compared to that of monopole hole excitations, measured by ARPE
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