6 research outputs found
Novel sources of near- and mid-infrared femtosecond pulses for applications in gas sensing, pulse shaping and material processing
In this thesis the design, construction process and the performance of two femtosecond
optical parametric oscillators and one second–harmonic generation femtosecond
pulse shaper is described. One oscillator was applied to gas sensing
while potential applications of other devices are outlined.
ATi:sapphire oscillator was used to pump a periodically–poled lithium niobate–
based optical parametric oscillator. This signal–resonant device was configured
to produce broadband idler pulses tunable in the range of 2.7–3.4 μm. This wavelength
coverage was matched to the ν3 optical absorption band of methane, and
Fourier–transform spectroscopy of a CH4:N2 mixture was implemented by employing
a mid–IR silica photonic bandgap fibre simultaneously as a gas cell and
an optical waveguide. Methane sensing below a 1% concentration was demonstrated
and the main limiting factors were identified and improvements suggested.
Another optical parametric oscillator was demonstrated which was pumped
by a commercial Yb:fibre master oscillator/power amplifier system and was based
on a periodically–poled lithium niobate crystal. The signal was tunable between
1.42–1.57 μm and was intended as a source for a subsequent project for waveguide
writing in silicon. The oscillator was a novel long–cavity device operating
at 15 MHz. The 130 nJ pump pulse energies allowed for 21 nJ signal pulses at
a pump power of 2 W. The performance of the oscillator was characterised via
temporal and spectral measurements and the next steps of its development are
outlined.
Finally a pulse shaper based on second harmonic generation in a grating–
engineered periodically–poled lithium niobate crystal was demonstrated. Pulses
from a 1.53 μm femtosecond Er:fibre laser were compressed and then used as the
input to the shaper. The performance of the shaper was tested by performing
cross–correlation frequency–resolved optical gating measurements on the output
second harmonic pulses and this confirmed the successful creation of multiple
pulses and other tailored shapes including square and chirped pulses, agreeing
well with theoretical calculations
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Noninvasive two-photon optical biopsy of retinal fluorophores
High-resolution imaging techniques capable of detecting identifiable endogenous fluorophores in the eye along with genetic testing will dramatically improve diagnostic capabilities in the ophthalmology clinic and accelerate the development of new treatments for blinding diseases. Two-photon excitation (TPE)-based imaging overcomes the filtering of ultraviolet light by the lens of the human eye and thus can be utilized to discover defects in vitamin A metabolism during the regeneration of the visual pigments required for the detection of light. Combining TPE with fluorescence lifetime imaging (FLIM) and spectral analyses offers the potential of detecting diseases of the retina at earlier stages before irreversible structural damage has occurred. The main barriers to realizing the benefits of TPE for imaging the human retina arise from concerns about the high light exposure typically needed for informative TPE imaging and the requirement to correlate the ensuing data with different states of health and disease. To overcome these hurdles, we improved TPE efficiency by controlling temporal properties of the excitation light and employed phasor analyses to FLIM and spectral data in mouse models of retinal diseases. Modeling of retinal photodamage revealed that plasma-mediated effects do not play a role and that melanin-related thermal effects are mitigated by reducing pulse repetition frequency. By using noninvasive TPE imaging we identified molecular components of individual granules in the retinal pigment epithelium and present their analytical characteristics