55 research outputs found
Phase transitions in open quantum systems
We consider the behaviour of open quantum systems in dependence on the
coupling to one decay channel by introducing the coupling parameter
being proportional to the average degree of overlapping. Under critical
conditions, a reorganization of the spectrum takes place which creates a
bifurcation of the time scales with respect to the lifetimes of the resonance
states. We derive analytically the conditions under which the reorganization
process can be understood as a second-order phase transition and illustrate our
results by numerical investigations. The conditions are fulfilled e.g. for a
picket fence with equal coupling of the states to the continuum. Energy
dependencies within the system are included. We consider also the generic case
of an unfolded Gaussian Orthogonal Ensemble. In all these cases, the
reorganization of the spectrum occurs at the critical value of
the control parameter globally over the whole energy range of the spectrum. All
states act cooperatively.Comment: 28 pages, 22 Postscript figure
Interfering Doorway States and Giant Resonances. I: Resonance Spectrum and Multipole Strengths
A phenomenological schematic model of multipole giant resonances (GR) is
considered which treats the external interaction via common decay channels on
the same footing as the coherent part of the internal residual interaction. The
damping due to the coupling to the sea of complicated states is neglected. As a
result, the formation of GR is governed by the interplay and competition of two
kinds of collectivity, the internal and the external one. The mixing of the
doorway components of a GR due to the external interaction influences
significantly their multipole strengths, widths and positions in energy. In
particular, a narrow resonance state with an appreciable multipole strength is
formed when the doorway components strongly overlap.Comment: 20 pages, LaTeX, 3 ps-figures, to appear in PRC (July 1997
Resonance trapping and saturation of decay widths
Resonance trapping appears in open many-particle quantum systems at high
level density when the coupling to the continuum of decay channels reaches a
critical strength. Here a reorganization of the system takes place and a
separation of different time scales appears. We investigate it under the
influence of additional weakly coupled channels as well as by taking into
account the real part of the coupling term between system and continuum. We
observe a saturation of the mean width of the trapped states. Also the decay
rates saturate as a function of the coupling strength. The mechanism of the
saturation is studied in detail. In any case, the critical region of
reorganization is enlarged. When the transmission coefficients for the
different channels are different, the width distribution is broadened as
compared to a chi_K^2 distribution where K is the number of channels. Resonance
trapping takes place before the broad state overlaps regions beyond the
extension of the spectrum of the closed system.Comment: 18 pages, 8 figures, accepted by Phys. Rev.
Eco-friendly one-pot synthesis of Prussian blue-embedded magnetic hydrogel beads for the removal of cesium from water
A simple one-step approach to fabricating Prussian blue-embedded magnetic hydrogel beads (PBMHBs) was fabricated for the effective magnetic removal of radioactive cesium (Cs-137) from water. Through the simple dropwise addition of a mixed aqueous solution of iron salts, commercial PB and polyvinyl alcohol (PVA) to an ammonium hydroxide (NH4OH) solution, the formation of hydrogel beads and the encapsulation of PB in beads were achieved in one pot through the gelation of PVA with in situ-formed iron oxide nanoparticles as the cross-linker. The obtained PB-MHBs, with 43.77 weight %of PB, were stable without releasing PB for up to 2 weeks and could be effectively separated from aqueous solutions by an external magnetic field, which is convenient for the large-scale treatment of Cs-contaminated water. Detailed Cs adsorption studies revealed that the adsorption isotherms and kinetics could be effectively described by the Langmuir isotherm model and the pseudo-second-order model, respectively. Most importantly, the PB-MHBs exhibited excellent selectivity for Cs-137 in (137)Cscontaminated simulated groundwater (55 Bq/g) with a high removal efficiency (>99.5%), and the effective removal of Cs-137 from real seawater by these PB-MHBs demonstrated the excellent potential of this material for practical application in the decontamination of Cs-137-contaminated seawate
Holey Fibers Filling with Liquids and Sol-Gel Materials
Hollow-core fibers have been filled by photolumiscent and Raman active materials. The filling can be obtained
by capillarity for liquid phase materials, or by pressure for more viscous solutions. An experimental set-up to
measure attenuation changes due to the filling process has been arranged and the variations of the transmission
properties have been measured over a broad band. The Raman activity of the filling materials has been
determined by spectroscopic measurements
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