1,647 research outputs found
Gap ratio in anharmonic charge-density-wave systems
Many experimental systems exist that possess charge-density-wave order in
their ground state. While this order should be able to be described with models
similar to those used for superconductivity, nearly all systems have a ratio of
the charge-density-wave order parameter to the transition temperature that is
too high for conventional theories. Recent work explained how this can happen
in harmonic systems, but when the lattice distortion gets large, anharmonic
effects must play an increasingly important role. Here we study the gap ratio
for anharmonic charge-density wave systems to see whether the low-temperature
properties possess universality as was seen previously in the transition
temperature and to see whether the explanation for the large gap ratios
survives for anharmonic systems as well.Comment: (5 pages, 3 figures, ReVTeX
Sodium Atoms in the Lunar Exotail: Observed Velocity and Spatial Distributions
The lunar sodium tail extends long distances due to radiation pressure on sodium atoms in the lunar exosphere. Our earlier observations measured the average radial velocity of sodium atoms moving down the lunar tail beyond Earth (i.e., near the anti-lunar point) to be ~ 12.5 km/s. Here we use the Wisconsin H-alpha Mapper to obtain the first kinematically resolved maps of the intensity and velocity distribution of this emission over a 15 x 15 deg region on the sky near the anti-lunar point. We present both spatially and spectrally resolved observations obtained over four nights bracketing new Moon in October 2007. The spatial distribution of the sodium atoms is elongated along the ecliptic with the location of the peak intensity drifting 3 deg east along the ecliptic per night. Preliminary modeling results suggest the spatial and velocity distributions in the sodium exotail are sensitive to the near surface lunar sodium velocity distribution. Future observations of this sort along with detailed modeling offer new opportunities to describe the time history of lunar surface sputtering over several days
Nonresonant inelastic light scattering in the Hubbard model
Inelastic light scattering from electrons is a symmetry-selective probe of
the charge dynamics within correlated materials. Many measurements have been
made on correlated insulators, and recent exact solutions in large dimensions
explain a number of anomalous features found in experiments. Here we focus on
the correlated metal, as described by the Hubbard model away from half filling.
We can determine the B1g Raman response and the inelastic X-ray scattering
along the Brillouin zone diagonal exactly in the large dimensional limit. We
find a number of interesting features in the light scattering response which
should be able to be seen in correlated metals such as the heavy fermions.Comment: 9 pages, 7 figures, typeset with ReVTe
Characterizing the metabolic effects of the selective inhibition of gut microbial β-glucuronidases in mice
The hydrolysis of xenobiotic glucuronides by gut bacterial glucuronidases reactivates previously detoxified compounds resulting in severe gut toxicity for the host. Selective bacterial β-glucuronidase inhibitors can mitigate this toxicity but their impact on wider host metabolic processes has not been studied. To investigate this the inhibitor 4-(8-(piperazin-1-yl)-1,2,3,4-tetrahydro-[1,2,3]triazino[4′,5′:4,5]thieno[2,3-c]isoquinolin-5-yl)morpholine (UNC10201652, Inh 9) was administered to mice to selectively inhibit a narrow range of bacterial β-glucuronidases in the gut. The metabolomic profiles of the intestinal contents, biofluids, and several tissues involved in the enterohepatic circulation were measured and compared to control animals. No biochemical perturbations were observed in the plasma, liver or gall bladder. In contrast, the metabolite profiles of urine, colon contents, feces and gut wall were altered compared to the controls. Changes were largely restricted to compounds derived from gut microbial metabolism. This work establishes that inhibitors targeted towards bacterial β-glucuronidases modulate the functionality of the intestinal microbiota without adversely impacting the host metabolic system
Gap to Transition Temperature Ratio in Density Wave Ordering: a Dynamical Mean Field Study
We use the dynamical mean-field method to determine the origin of the large
ratio of the zero temperature gap to the transition temperature observed in
most charge density wave materials. The method is useful because it allows an
exact treatment of thermal fluctuations. We establish the relation of the
dynamical mean-field results to conventional diagrammatics and thereby
determine that in the physically relevant regime the origin of the large ratio
is a strong inelastic scattering.Comment: 4 figure
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Air-breathing fuel cell stacks for portable power applications
Increasing attention is being directed towards polymer electrolyte fuel cells as battery replacements because of their potentially superior energy densities and the possibility of `mechanical` refueling. On the low end of the power requirement scale (ca. 10 W), fuel cells can compete with primary and secondary batteries only if the fuel cell systems are simple, inexpensive, and reliable. Considerations of cost and simplicity (and minimal parasitic power) discourage the use of conventional performance enhancing subsystems (e.g., humidification, cooling, or forced-reactant flow). We are developing a stack design that is inherently self-regulating to allow effective operation without the benefit of such auxiliary components. The air cathode does not use forced flow to replenish the depleted oxygen. Instead, the oxygen in the air must diffuse into the stack from the periphery of the unit cells. For this reason the stack is described as `air-breathing.` This configuration limits the ability of water to escape which prevents the polymer electrolyte membranes from drying out, even at relatively high continuous operation temperatures (+60 degrees C). This results in stacks with reliable and stable performance. This air-breathing configuration assumes a unique stack geometry that utilizes circular flow-field plates with an annular hydrogen feed manifold and the single tie-bolt extending up through the central axis of the stack. With this geometry, the hydrogen supply to the unit cells is radially outward, and the air supply is from the periphery inward. This configuration has several advantages. The entire periphery is free to air access and allows greater heat conduction to enhance cooling. Furthermore, all of the components in the stack (e.g., the flow-fields, seals and membrane/electrode assemblies), are radially symmetrical, so part fabrication is simple and the entire system is potentially low-cost. Lastly, this configuration is compact and lightweight
The architecture of the Gram-positive bacterial cell wall
The primary structural component of the bacterial cell wall is peptidoglycan, which is essential for viability and the synthesis of which is the target for crucial antibiotics1,2. Peptidoglycan is a single macromolecule made of glycan chains crosslinked by peptide side branches that surrounds the cell, acting as a constraint to internal turgor1,3. In Gram-positive bacteria, peptidoglycan is tens of nanometres thick, generally portrayed as a homogeneous structure that provides mechanical strength4,5,6. Here we applied atomic force microscopy7,8,9,10,11,12 to interrogate the morphologically distinct Staphylococcus aureus and Bacillus subtilis species, using live cells and purified peptidoglycan. The mature surface of live cells is characterized by a landscape of large (up to 60 nm in diameter), deep (up to 23 nm) pores constituting a disordered gel of peptidoglycan. The inner peptidoglycan surface, consisting of more nascent material, is much denser, with glycan strand spacing typically less than 7 nm. The inner surface architecture is location dependent; the cylinder of B. subtilis has dense circumferential orientation, while in S. aureus and division septa for both species, peptidoglycan is dense but randomly oriented. Revealing the molecular architecture of the cell envelope frames our understanding of its mechanical properties and role as the environmental interface13,14, providing information complementary to traditional structural biology approaches
Electrically pumped single-defect light emitters in WSe
Recent developments in fabrication of van der Waals heterostructures enable new type of devices assembled by stacking atomically thin layers of two-dimensional materials. Using this approach, we fabricate light-emitting devices based on a monolayer WSe, and also comprising boron nitride tunnelling barriers and graphene electrodes, and observe sharp luminescence spectra from individual defects in WSe under both optical and electrical excitation. This paves the way towards the realization of electrically-pumped quantum emitters in atomically thin semiconductors. In addition we demonstrate tuning by more than 1 meV of the emission energy of the defect luminescence by applying a vertical electric field. This provides an estimate of the permanent electric dipole created by the corresponding electron-hole pair. The light-emitting devices investigated in our work can be assembled on a variety of substrates enabling a route to integration of electrically pumped single quantum emitters with existing technologies in nano-photonics and optoelectronics
Non-linear regression models for Approximate Bayesian Computation
Approximate Bayesian inference on the basis of summary statistics is
well-suited to complex problems for which the likelihood is either
mathematically or computationally intractable. However the methods that use
rejection suffer from the curse of dimensionality when the number of summary
statistics is increased. Here we propose a machine-learning approach to the
estimation of the posterior density by introducing two innovations. The new
method fits a nonlinear conditional heteroscedastic regression of the parameter
on the summary statistics, and then adaptively improves estimation using
importance sampling. The new algorithm is compared to the state-of-the-art
approximate Bayesian methods, and achieves considerable reduction of the
computational burden in two examples of inference in statistical genetics and
in a queueing model.Comment: 4 figures; version 3 minor changes; to appear in Statistics and
Computin
Chlorophyll fluorescence-based high-throughput phenotyping facilitates the genetic dissection of photosynthetic heat tolerance in African (Oryza glaberrima) and Asian (Oryza sativa) rice.
Acknowledgements We are grateful to the University of Nottingham glasshouse staff for their assistance with general plant maintenance. We acknowledge the insight of two anonymous reviews whose comments greatly improved this manuscript. JR and JNF were supported by the Palaeobenchmarking Resilient Agriculture Systems (PalaeoRAS) project funded by the Future Food Beacon of the University of Nottingham.Peer reviewedPostprin
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