61 research outputs found
Measurement of non-Gaussian shot noise: influence of the environment
We present the first measurements of the third moment of the voltage
fluctuations in a conductor. This technique can provide new and complementary
information on the electronic transport in conducting systems. The measurement
was performed on non-superconducting tunnel junctions as a function of voltage
bias, for various temperatures and bandwidths up to 1GHz. The data demonstrate
the significant effect of the electromagnetic environment of the sample.Comment: 13 pages, for the SPIE International Symposium on Fluctuations and
Noise, Maspalomas, Gran Canaria, Spain (May 2004
Environmental effects in the third moment of voltage fluctuations in a tunnel junction
We present the first measurements of the third moment of the voltage
fluctuations in a conductor. This technique can provide new and complementary
information on the electronic transport in conducting systems. The measurement
was performed on non-superconducting tunnel junctions as a function of voltage
bias, for various temperatures and bandwidths up to 1GHz. The data demonstrate
the significant effect of the electromagnetic environment of the sample.Comment: Major revision. More experimental results. New interpretation. 4
pages, 3 figure
Self-organization of charge under pressure in the organic conductor (TMTSF)2ReO4
(TMTSF)2ReO4 presents a phase coexistence between two anion orderings defined
by their wave vectors q_2=(1/2,1/2,1/2) and q_3=(0,1/2,1/2) in a wide range of
pressure (8-11kbar) and temperature. From the determination of the anisotropy
of the conductivity and the superconducting transitions in this regime we were
able to extract the texture which results from a self-organization of the
orientations of the ReO4 anions in the sample. At the lowest pressures, the
metallic parts, related to the q_3 order, form droplets elongated along the
a-axis embedded in the semiconducting matrix associated with the q_2 order.
Above 10kbar, filaments along the a-axis extend from one end of the sample to
the other nearly up to the end of the coexistence regime. A mapping of the
system into an anisotropic Ising lattice is satisfactory to analyze the data.
satisfactory to analyze the data.Comment: 7 pages, 3 figures, EPL forma
Aperiodic quantum oscillations of particle-hole asymmetric Dirac cones
We report experimental measurements and theoretical analysis of Shubnikov-de
Haas (SdH) oscillations in a Dirac cone system: the a-(BEDT-TTF)2I3 organic
metal under hydrostatic pressure. The measured SdH oscillations reveal
anomalies at high magnetic fields B where the 1/B oscillations periodicity is
lost above 7 T. We interpret these unusual results within a theoretical model
that takes into account intrinsic distortions of the a-(BEDT-TTF)2I3 Dirac
cones such as a parabolic particle-hole asymmetric correction. Others possible
causes, such as a cone tilting or a Zeeman effect, are carefully ruled out. The
observations are consistent among a-(BEDT-TTF)2I3 samples with different Fermi
levels
Strongly correlated properties of the thermoelectric cobalt oxide Ca3Co4O9
We have performed both in-plane resistivity, Hall effect and specific heat
measurements on the thermoelectric cobalt oxide CaCoO. Four
distinct transport regimes are found as a function of temperature,
corresponding to a low temperature insulating one up to 63 K,
a strongly correlated Fermi liquid up to 140 K, with
and , followed
by an incoherent metal with and a high temperature insulator above
T510 K . Specific heat Sommerfeld coefficient
mJ/(mol.K) confirms a rather large value of the electronic effective mass
and fulfils the Kadowaki-Woods ratio 10 . Resistivity measurements under pressure reveal a
decrease of the Fermi liquid transport coefficient A with an increase of
as a function of pressure while the product remains constant and
of order . Both thermodynamic and transport properties suggest a strong
renormalization of the quasiparticles coherence scale of order that seems
to govern also thermopower.Comment: 5 pages, 6 figures, accepted for publication in Physical Review
Radical cation salts of TTF donors with XF6 (X = Re,Ta) anions
Electrocrystallization of the dianionic Re(IV)F6 species with different organic π electron donors was carried out. Depending on the first oxidation potential of the TTF derivatives this crystallization technique gave rise to various radical cations salts involving Re(IV) or Re(V) anions. With tetramethyltetrathiafulvalene (TMTTF) the (TMTTF)2Re(IV)F6 salt was obtained. However, with tetramethyltetraselenafulvalene (TMTSF) we obtained very small needles of the (TMTSeF)2Re(V)F6 system, analogue to the so called “Bechgaard salts” [1].
We present some characteristics of this new metallic phase. We compare to the diamagnetic (TMTSeF)2Ta(V)F6 obtained by the same strategy using TBATaF6 prepared according to the Browstein’s method [2] and explore electrocrystallization of the tantalum based anions [3], [4].
References:
[1] K. Bechgaard, C.S. Jacobsen, K. Mortensen, H.J. Pedersen, N. Thorup, Solid State Commun. 1980, 33, 1119-1125.
[2] S. Brownstein, Inorg. Chem. 1973, 12, N°3, 584-589.
[3] C. Lenoir, K. Boubekeur, P. Batail, E. Canadell, P. Auban, O. Traetteberg, D. Jérome, Synth. Met. 1991, 42, 1939-1942.
[4] F. Iwase, K. Sugiura, K. Furukawa, T. Nakamura, J. Phys. Soc. Jpn. 2009, 78, N°10, 104717:1-104717:7
Temperature dependent resistivity under pressure and magnetoresistance data of the organic superconductor (BEDO-TTF)2ReO4(H2O)
The temperature dependence of the resistivity under pressure (up to 6 kbar) of the organic metal (BEDO-TTF)2ReO4(H20) is reported. An increase of the resistivity below 35 K, which is observed at ambient pressure, is already suppressed at 1 kbar. In addition at this pressure the superconducting transition sharpens and the onset temperature of 2.3 K is nearly the same as at ambient pressure. Magnetoresistance data, observed at 1.3 K and 6.7 Tesla show a strong angle dependence. In addition at 1.3 K first SdH -oscillations in the magnetoresistance are found already at such low fields as 5 Tesla
Evidence for distinct polymer chain orientations in KC60 and RbC60
The KC60 and RbC60 polymer phases exhibit contrasting electronic properties
while powder diffraction studies have revealed no definite structural
difference. We have performed single crystal X-ray diffraction and diffuse
scattering studies of these compounds. It is found that KC60 and RbC60 possess
different chain orientations about their axes, which are described by distinct
space groups Pmnn and I2/m, respectively. Such a structural difference will be
of great importance to a complete understanding of the physical properties.Comment: To be published in Phys. Rev. Let
Finite-Temperature Properties across the Charge Ordering Transition -- Combined Bosonization, Renormalization Group, and Numerical Methods
We theoretically describe the charge ordering (CO) metal-insulator transition
based on a quasi-one-dimensional extended Hubbard model, and investigate the
finite temperature () properties across the transition temperature, . In order to calculate dependence of physical quantities such as the
spin susceptibility and the electrical resistivity, both above and below
, a theoretical scheme is developed which combines analytical
methods with numerical calculations. We take advantage of the renormalization
group equations derived from the effective bosonized Hamiltonian, where Lanczos
exact diagonalization data are chosen as initial parameters, while the CO order
parameter at finite- is determined by quantum Monte Carlo simulations. The
results show that the spin susceptibility does not show a steep singularity at
, and it slightly increases compared to the case without CO because
of the suppression of the spin velocity. In contrast, the resistivity exhibits
a sudden increase at , below which a characteristic dependence
is observed. We also compare our results with experiments on molecular
conductors as well as transition metal oxides showing CO.Comment: 9 pages, 8 figure
Superconductivity and Antiferromagnetism in Quasi-one-dimensional Organic Conductors
We review the current understanding of superconductivity in the
quasi-one-dimensional organic conductors of the Bechgaard and Fabre salt
families. We discuss the interplay between superconductivity,
antiferromagnetism, and charge-density-wave fluctuations. The connection to
recent experimental observations supporting unconventional pairing and the
possibility of a triplet-spin order parameter for the superconducting phase is
also presented.Comment: (v1) 30 pages, 13 figures; Review article for the 20th anniversary of
high-Tc superconductivity, to appear in J. Low Temp. Phys. (v2) 1 Ref. adde
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