12,218 research outputs found
Active colloids in complex fluids
We review recent work on active colloids or swimmers, such as self-propelled
microorganisms, phoretic colloidal particles, and artificial micro-robotic
systems, moving in fluid-like environments. These environments can be
water-like and Newtonian but can frequently contain macromolecules, flexible
polymers, soft cells, or hard particles, which impart complex, nonlinear
rheological features to the fluid. While significant progress has been made on
understanding how active colloids move and interact in Newtonian fluids, little
is known on how active colloids behave in complex and non-Newtonian fluids. An
emerging literature is starting to show how fluid rheology can dramatically
change the gaits and speeds of individual swimmers. Simultaneously, a moving
swimmer induces time dependent, three dimensional fluid flows, that can modify
the medium (fluid) rheological properties. This two-way, non-linear coupling at
microscopic scales has profound implications at meso- and macro-scales: steady
state suspension properties, emergent collective behavior, and transport of
passive tracer particles. Recent exciting theoretical results and current
debate on quantifying these complex active fluids highlight the need for
conceptually simple experiments to guide our understanding.Comment: 6 figure
The Geometric Structure of Complex Fluids
This paper develops the theory of affine Euler-Poincar\'e and affine
Lie-Poisson reductions and applies these processes to various examples of
complex fluids, including Yang-Mills and Hall magnetohydrodynamics for fluids
and superfluids, spin glasses, microfluids, and liquid crystals. As a
consequence of the Lagrangian approach, the variational formulation of the
equations is determined. On the Hamiltonian side, the associated Poisson
brackets are obtained by reduction of a canonical cotangent bundle. A
Kelvin-Noether circulation theorem is presented and is applied to these
examples
Nonlinear viscoelasticity of metastable complex fluids
Many metastable complex fluids such as colloidal glasses and gels show
distinct nonlinear viscoelasticity with increasing oscillatory-strain
amplitude; the storage modulus decreases monotonically as the strain amplitude
increases whereas the loss modulus has a distinct peak before it decreases at
larger strains. We present a qualitative argument to explain this ubiquitous
behavior and use mode coupling theory (MCT) to confirm it. We compare
theoretical predictions to the measured nonlinear viscoelasticity in a dense
hard sphere colloidal suspensions; reasonable agreement is obtained. The
argument given here can be used to obtain new information about linear
viscoelasticity of metastable complex fluids from nonlinear strain
measurements.Comment: 7 pages, 3 figures, accepted for publication in Europhys. Let
Lattice Boltzmann Models for Complex Fluids
We present various Lattice Boltzmann Models which reproduce the effects of
rough walls, shear thinning and granular flow. We examine the boundary layers
generated by the roughness of the walls. Shear thinning produces plug flow with
a sharp density contrast at the boundaries. Density waves are spontaneously
generated when the viscosity has a nonlinear dependence on density which
characterizes granular flow.Comment: 11 pages, plain TeX, preprint HLRZ 23/9
Probing structural relaxation in complex fluids by critical fluctuations
Complex fluids, such as polymer solutions and blends, colloids and gels, are
of growing interest in fundamental and applied soft-condensed-matter science. A
common feature of all such systems is the presence of a mesoscopic structural
length scale intermediate between atomic and macroscopic scales. This
mesoscopic structure of complex fluids is often fragile and sensitive to
external perturbations. Complex fluids are frequently viscoelastic (showing a
combination of viscous and elastic behaviour) with their dynamic response
depending on the time and length scales. Recently, non-invasive methods to
infer the rheological response of complex fluids have gained popularity through
the technique of microrheology, where the diffusion of probe spheres in a
viscoelastic fluid is monitored with the aid of light scattering or microscopy.
Here we propose an alternative to traditional microrheology that does not
require doping of probe particles in the fluid (which can sometimes drastically
alter the molecular environment). Instead, our proposed method makes use of the
phenomenon of "avoided crossing" between modes associated with the structural
relaxation and critical fluctuations that are spontaneously generated in the
system.Comment: 4 pages, 4 figure
- …