Experimental study of neutron-rich nuclei 89Rb and 91Rb

Neutron-rich 89,91Rb nuclei populated as fission products in heavy-ion reactions have been studied with the Gammasphere array. The previously known level schemes have been extended to higher excitation energies and spins. Spin and parity assignments were based on angular correlation analyses. A value of T1/2 = 8(2) ns was extracted for the isomeric g9/2 state in 89Rb

The soil geochemistry in the Beardmore Glacier Region, Antarctica: Implications for terrestrial ecosystem history

Although most models suggest continental Antarctica was covered by ice during the Last Glacial Maximum (LGM) it has been speculated that endemic species of soil invertebrates could have survived the Pleistocene at high elevation habitats protruding above the ice sheets. We analyzed a series of soil samples from different elevations at three locations along the Beardmore Glacier in the Transantarctic Mountains (in order of increasing elevation): Ebony Ridge (ER), Cloudmaker (CM), and Meyer Desert (MD). Geochemical analyses show the MD soils, which were exposed during the LGM, were the least weathered compared to lower elevations, and also had the highest total dissolved solids (TDS). MD soils are dominated by nitrate salts (NO₃/Cl ratios >10) that can be observed in SEM images. High δ¹⁷O and δ¹⁸O values of the nitrate indicate that its source is solely of atmospheric origin. It is suggested that nitrate concentrations in the soil may be utilized to determine a relative “wetting age” to better assess invertebrate habitat suitability. The highest elevation sites at MD have been exposed and accumulating salts for the longest times, and because of the salt accumulations, they were not suitable as invertebrate refugia during the LGM

Revised B(E3) transition rate and structure of the 3− level in 96Zr

The B(E3) transition strength from the 1897-keV, 3− level in 96Zr has been reevaluated from six high-statistics, independent data sets. The measured value of 42(3) W.u. is significantly lower than that adopted in recent compilations. It is, however, in line with the global systematics of collective B(E3) rates found throughout the periodic table. Thus, the “exceptional” character of this transition, that challenged theory, no longer applies. Monte Carlo shell-model calculations indicate that the collectivity of the octupole vibration arises from both proton and neutron excitations involving a large number of orbitals

Revised B(E3) transition rate and structure of the 3− level in 96Zr

The B(E3) transition strength from the 1897-keV, 3− level in 96Zr has been reevaluated from six high-statistics, independent data sets. The measured value of 42(3) W.u. is significantly lower than that adopted in recent compilations. It is, however, in line with the global systematics of collective B(E3) rates found throughout the periodic table. Thus, the “exceptional” character of this transition, that challenged theory, no longer applies. Monte Carlo shell-model calculations indicate that the collectivity of the octupole vibration arises from both proton and neutron excitations involving a large number of orbitals

Shape coexistence from lifetime and branching-ratio measurements in 68,70Ni

© 2016 The Author(s) Shape coexistence near closed-shell nuclei, whereby states associated with deformed shapes appear at relatively low excitation energy alongside spherical ones, is indicative of the rapid change in structure that can occur with the addition or removal of a few protons or neutrons. Near 68Ni (Z=28, N=40), the identification of shape coexistence hinges on hitherto undetermined transition rates to and from low-energy 0+ states. In 68,70Ni, new lifetimes and branching ratios have been measured. These data enable quantitative descriptions of the 0+ states through the deduced transition rates and serve as sensitive probes for characterizing their nuclear wave functions. The results are compared to, and consistent with, large-scale shell-model calculations which predict shape coexistence. With the firm identification of this phenomenon near 68Ni, shape coexistence is now observed in all currently accessible regions of the nuclear chart with closed proton shells and mid-shell neutrons

Multinucleon transfer in the interaction of 977 MeV and 1143 MeV Hg 204 with Pb 208

A previous study of symmetric collisions of massive nuclei has shown that current models of multinucleon transfer (MNT) reactions do not adequately describe the transfer product yields. To gain further insight into this problem, we have measured the yields of MNT products in the interaction of 977 (E/A=4.79 MeV) and 1143 MeV (E/A=5.60 MeV) Hg204 with Pb208. We find that the yield of multinucleon transfer products are similar in these two reactions and are substantially lower than those observed in the reaction of 1257 MeV (E/A=6.16 MeV) Hg204+Pt198. We compare our measurements with the predictions of the GRAZING-F, dinuclear systems (DNS), and improved quantum molecular dynamics (ImQMD) models. For the observed isotopes of the elements Au, Hg, Tl, Pb, and Bi, the measured values of the MNT cross sections are orders of magnitude larger than the predicted values. Furthermore, the various models predict the formation of nuclides near the N=126 shell, which are not observed

Decay properties of the new isotopes 172Hg and 173Hg

The α decays of the two neutron-deficient nuclei 172Hg and 173Hg were observed for the first time using the 78Kr(96Ru,2n) and 80Kr(96Ru,3n) reactions, respectively. The reaction products were dispersed according to their mass-to-charge state ratios in the Argonne Fragment Mass Analyzer and implanted in a double-sided silicon strip detector, where their subsequent decays were studied using spatial and time correlations between implants and decays. A half-life of 250(+350-90) μs and an energy of 7350(12) keV were deduced for the α decay of 172Hg. In 173Hg the half-life was measured to be 0.93(+0.57-0.26) ms and the corresponding energy is 7211(11) keV. In addition, the half-life and energy of the α decay of 174Hg were measured more precisely. The reduced widths deduced for these Hg isotopes indicate that the observed decays correspond to unhindered Δl = 0 transitions. The α-decay Q values are compared with the values calculated using mass tables by Möller and Nix, and by Liran and Zeldes. The latter mass tables show better agreement with the data

Proton and α radioactivity of 185Bi

Proton and α emission from 185Bi have been confirmed and measured with improved statistics. The 185Bi nuclei were produced via the 95Mo(92Mo,pn) reaction at a bombarding energy of 420 MeV. The proton decay energy from the 1/2+ intruder state in 185Bi to the 184Pb ground state was measured to be 1.598(16) MeV with a proton branching ratio bp, = 0.85(6). An α decay branch from the same state was measured, bα = 0.15(6), with an energy of 8.08(3) MeV. The state has a half-life of 50(8) μs. In addition, the α branching ratio of the ground state of 184Pb was determined for the first time to be bα = 0.23(14)

Xe 136 + Pb 208 reaction: A test of models of multinucleon transfer reactions

The yields of over 200 projectile-like fragments (PLFs) and target-like fragments (TLFs) from the interaction of (Ec.m.=450 MeV) Xe136 with a thick target of Pb208 were measured using Gammasphere and off-line γ-ray spectroscopy, giving a comprehensive picture of the production cross sections in this reaction. The measured yields were compared to predictions of the grazing model and the predictions of Zagrebaev and Greiner using a quantitative metric, the theory evaluation factor tef. The grazing model predictions are adequate for describing the yields of nuclei near the target or projectile but they grossly underestimate the yields of all other products. The predictions of Zagrebaev and Greiner correctly describe the magnitude and maxima of the observed TLF transfer cross sections for a wide range of transfers (ΔZ=-8 to ΔZ=+2). However, for ΔZ=+4, the observed position of the maximum in the distribution is four neutrons richer than the predicted maximum. The predicted yields of the neutron-rich N=126 nuclei exceed the measured values by two orders of magnitude. Correlations between TLF and PLF yields are discussed

Low-energy structure of Mn61 populated following β decay of Cr61

β decay of the Cr6137 ground state has been studied. A new half-life of 233±11 ms has been deduced, and seven delayed γ rays have been assigned to the daughter Mn6136. The low-energy level structure of Mn6136 is similar to that of the less neutron-rich Mn57,59 nuclei. The odd-A25Mn isotopes follow the systematic trend in the yrast states of the even-even, Z+1 26Fe isotopes, and not that of the Z-1 24Cr isotopes, where a possible onset of collectivity has been suggested to occur already at N=36