Temperature-controlled entangled-photon absorption spectroscopy

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this technique has remained elusive, mainly because of two major difficulties: first, the need to perform multiple experiments with two-photon states bearing different temporal correlations, which translates into the necessity to have at the experimenter’s disposal tens, if not hundreds, of sources of entangled photons; second, the need to have a priori knowledge of the absorbing medium’s lowest-lying intermediate energy level. In this work, we put forward a simple experimental scheme that successfully overcomes these two limitations. By making use of a temperature-controlled entangled-photon source, which allows the tuning of the central frequencies of the absorbed photons, we show that the TPA signal, measured as a function of the temperature of the nonlinear crystal that generates the paired photons, and a controllable delay between them, carries all information about the electronic level structure of the absorbing medium, which can be revealed by a simple Fourier transformation.Peer ReviewedPostprint (author's final draft

Two-particle quantum correlations in stochastically-coupled networks

Quantum walks in dynamically-disordered networks have become an invaluable tool for understanding the physics of open quantum systems. In this work, we introduce a novel approach to describe the dynamics of indistinguishable particles in noisy quantum networks. By making use of stochastic calculus, we derive a master equation for the propagation of two non-interacting correlated particles in tight-binding networks affected by off-diagonal dynamical disorder. We show that the presence of noise in the couplings of a quantum network creates a pure-dephasing-like process that destroys all coherences in the single-particle Hilbert subspace. Remarkably, we find that when two or more correlated particles propagate in the network, coherences accounting for particle indistinguishability are robust against the impact of noise, thus showing that it is possible, in principle, to find specific conditions for which many indistinguishable particles can traverse dynamically-disordered systems without losing their ability to interfere. These results shed light on the role of particle indistinguishability in the preservation of quantum coherence in dynamically-disordered quantum networks.Comment: 15 pages, 4 figure

Endurance of quantum coherence due to particle indistinguishability in noisy quantum networks

Quantum coherence, the physical property underlying fundamental phenomena such as multi-particle interference and entanglement, has emerged as a valuable resource upon which modern technologies are founded. In general, the most prominent adversary of quantum coherence is noise arising from the interaction of the associated dynamical system with its environment. Under certain conditions, however, the existence of noise may drive quantum and classical systems to endure intriguing nontrivial effects. In this vein, here we demonstrate, both theoretically and experimentally, that when two indistinguishable non-interacting particles co-propagate through quantum networks affected by non-dissipative noise, the system always evolves into a steady state in which coherences accounting for particle indistinguishabilty perpetually prevail. Furthermore, we show that the same steady state with surviving quantum coherences is reached even when the initial state exhibits classical correlations.Comment: arXiv admin note: substantial text overlap with arXiv:1709.0433

Generating high-order exceptional points in coupled electronic oscillators using complex synthetic gauge fields

Exceptional points (EPs) are degeneracies of non-Hermitian systems, where both eigenvalues and eigenvectors coalesce. Classical and quantum systems exhibiting high-order EPs have recently been identified as fundamental building blocks for the development of novel, ultra-sensitive opto-electronic devices. However, arguably one of their major drawbacks is that they rely on non-linear amplification processes that could limit their potential applications, particularly in the quantum realm. In this work, we show that high-order EPs can be designed by means of linear, time-modulated, chain of inductively coupled RLC (where R stands for resistance, L for inductance, and C for capacitance) electronic circuits. With a general theory, we show that $N$ coupled circuits with $2N$ dynamical variables and time-dependent parameters can be mapped onto an $N$-site, time-dependent, non-Hermitian Hamiltonian, and obtain constraints for $\mathcal{PT}$-symmetry in such models. With numerical calculations, we obtain the Floquet exceptional contours of order $N$ by studying the energy dynamics in the circuit. Our results pave the way toward realizing robust, arbitrary-order EPs by means of synthetic gauge fields, with important implications for sensing, energy transfer, and topology