535 research outputs found
Minimum Wage Effects in the Longer Run
Exposure to minimum wages at young ages may lead to longer-run effects. Among the
possible adverse longer-run effects are decreased labor market experience and
accumulation of tenure, lower current labor supply because of lower wages, and diminished
training and skill acquisition. Beneficial longer-run effects could arise if minimum wages
increase skill acquisition, or if short-term wage increases are long-lasting. We estimate the
longer-run effects of minimum wages by using information on the minimum wage history that
workers have faced since potentially entering the labor market. The evidence indicates that
even as individuals reach their late 20?s, they earn less and perhaps work less the longer
they were exposed to a higher minimum wage, especially as a teenager. The adverse longerrun
effects of facing high minimum wages as a teenager are stronger for blacks. From a
policy perspective, these longer-run effects of minimum wages are likely more significant
than the contemporaneous effects of minimum wages on youths that are the focus of most
research and policy debate
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Disentangling conical intersection and coherent molecular dynamics in methyl bromide with attosecond transient absorption spectroscopy
Attosecond probing of core-level electronic transitions provides a sensitive tool for studying valence molecular dynamics with atomic, state, and charge specificity. In this report, we employ attosecond transient absorption spectroscopy to follow the valence dynamics of strong-field initiated processes in methyl bromide. By probing the 3d core-to-valence transition, we resolve the strong field excitation and ensuing fragmentation of the neutral σ* excited states of methyl bromide. The results provide a clear signature of the non-adiabatic passage of the excited state wavepacket through a conical intersection. We additionally observe competing, strong field initiated processes arising in both the ground state and ionized molecule corresponding to vibrational and spin-orbit motion, respectively. The demonstrated ability to resolve simultaneous dynamics with few-femtosecond resolution presents a clear path forward in the implementation of attosecond XUV spectroscopy as a general tool for probing competing and complex molecular phenomena with unmatched temporal resolution
Electron affinity of Li: A state-selective measurement
We have investigated the threshold of photodetachment of Li^- leading to the
formation of the residual Li atom in the state. The excited residual
atom was selectively photoionized via an intermediate Rydberg state and the
resulting Li^+ ion was detected. A collinear laser-ion beam geometry enabled
both high resolution and sensitivity to be attained. We have demonstrated the
potential of this state selective photodetachment spectroscopic method by
improving the accuracy of Li electron affinity measurements an order of
magnitude. From a fit to the Wigner law in the threshold region, we obtained a
Li electron affinity of 0.618 049(20) eV.Comment: 5 pages,6 figures,22 reference
Spectroscopy of free radicals and radical containing entrance-channel complexes in superfluid helium nano-droplets
The spectroscopy of free radicals and radical containing entrance-channel
complexes embedded in superfluid helium nano-droplets is reviewed. The
collection of dopants inside individual droplets in the beam represents a
micro-canonical ensemble, and as such each droplet may be considered an
isolated cryo-reactor. The unique properties of the droplets, namely their low
temperature (0.4 K) and fast cooling rates ( K s) provides
novel opportunities for the formation and high-resolution studies of molecular
complexes containing one or more free radicals. The production methods of
radicals are discussed in light of their applicability for embedding the
radicals in helium droplets. The spectroscopic studies performed to date on
molecular radicals and on entrance / exit-channel complexes of radicals with
stable molecules are detailed. The observed complexes provide new information
on the potential energy surfaces of several fundamental chemical reactions and
on the intermolecular interactions present in open-shell systems. Prospects of
further experiments of radicals embedded in helium droplets are discussed,
especially the possibilities to prepare and study high-energy structures and
their controlled manipulation, as well as the possibility of fundamental
physics experiments.Comment: 25 pages, 12 figures, 4 tables (RevTeX
Revealing electronic state-switching at conical intersections in alkyl iodides by ultrafast XUV transient absorption spectroscopy
Conical intersections between electronic states often dictate the chemistry of photoexcited molecules. Recently developed sources of ultrashort extreme ultraviolet (XUV) pulses tuned to element-specific transitions in molecules allow for the unambiguous detection of electronic state-switching at a conical intersection. Here, the fragmentation of photoexcited iso-propyl iodide and tert-butyl iodide molecules (i-C3H7I and t-C4H9I) through a conical intersection between 3Q0/1Q1 spin–orbit states is revealed by ultrafast XUV transient absorption measuring iodine 4d core-to-valence transitions. The electronic state-sensitivity of the technique allows for a complete mapping of molecular dissociation from photoexcitation to photoproducts. In both molecules, the sub-100 fs transfer of a photoexcited wave packet from the 3Q0 state into the 1Q1 state at the conical intersection is captured. The results show how differences in the electronic state-switching of the wave packet in i-C3H7I and t-C4H9I directly lead to differences in the photoproduct branching ratio of the two systems
Classical interventions in quantum systems. I. The measuring process
The measuring process is an external intervention in the dynamics of a
quantum system. It involves a unitary interaction of that system with a
measuring apparatus, a further interaction of both with an unknown environment
causing decoherence, and then the deletion of a subsystem. This description of
the measuring process is a substantial generalization of current models in
quantum measurement theory. In particular, no ancilla is needed. The final
result is represented by a completely positive map of the quantum state
(possibly with a change of the dimensions of ). A continuous limit of the
above process leads to Lindblad's equation for the quantum dynamical semigroup.Comment: Final version, 14 pages LaTe
Language barrier and its relationship to diabetes and diabetic retinopathy
10.1186/1471-2458-12-781BMC Public Health121
Measured body mass index, body weight perception, dissatisfaction and control practices in urban, low-income African American adolescents
<p>Abstract</p> <p>Background</p> <p>Current understanding of the associations between actual body weight status, weight perception, body dissatisfaction, and weight control practices among low-income urban African American adolescents is limited. The knowledge can help direct future intervention efforts.</p> <p>Methods</p> <p>Cross-sectional data including measured weight and height and self-reported weight status collected from 448 adolescents in four Chicago Public Schools were used.</p> <p>Results</p> <p>The prevalence of overweight and obesity (BMI ≥ 85<sup>th </sup>percentile) was 39.8%, but only 27.2% considered themselves as obese, although 43.4% reported trying to lose weight. Girls were more likely to express weight dissatisfaction than boys, especially those with BMI ≥ 95<sup>th </sup>percentile (62.9% vs. 25.9%). BMI ≥ 85<sup>th </sup>percentile girls were more likely to try to lose weight than boys (84.6% vs. 66.7%). Among all adolescents, 27.2% underestimated and 67.2% correctly judged their own weight status. Multinomial logistic models show that those with BMI ≥ 85<sup>th </sup>percentile, self-perceived as obese, or expressed body dissatisfaction were more likely to try to lose weight; adjusted odds ratios and 95% confidence intervals were 4.52 (2.53–8.08), 18.04 (7.19–45.30), 4.12 (1.64–10.37), respectively. No significant differences were found in diet and physical activity between those trying to lose weight and those not trying, but boys who reported trying to lose weight still spent more television time (P < 0.05).</p> <p>Conclusion</p> <p>Gender differences in weight perception, body dissatisfaction, and weight control practices exist among African American adolescents. One-third did not appropriately classify their weight status. Weight perception and body dissatisfaction are correlates of weight control practices. Adolescents attempting to lose weight need be empowered to make adequate desirable behavioral changes.</p
Ultrafast relaxation of photoexcited superfluid He nanodroplets
The relaxation of photoexcited nanosystems is a fundamental process of light-matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ultrafast, converting electronic energy in a few fs, or slow, if the energy is trapped in a metastable state that decouples from its environment. Here, we study helium nanodroplets excited resonantly by femtosecond extreme-ultraviolet (XUV) pulses from a seeded free- electron laser. Despite their superfluid nature, we find that helium nanodroplets in the lowest electronically excited states undergo ultrafast relaxation. By comparing experimental pho- toelectron spectra with time-dependent density functional theory simulations, we unravel the full relaxation pathway: Following an ultrafast interband transition, a void nanometer-sized bubble forms around the localized excitation (He ) within 1 ps. Subsequently, the bubble collapses and releases metastable He at the droplet surface. This study highlights the high level of detail achievable in probing the photodynamics of nanosystems using tunable XUV pulses
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