Absence of Long-Range Coherence in the Parametric Emission from Photonic Wires

We analytically investigate the spatial coherence properties of the signal emission from one-dimensional optical parametric oscillators. Because of the reduced dimensionality, quantum fluctuations are able to destroy the long-range phase coherence even far above threshold. The spatial decay of coherence is exponential and, for realistic parameters of semiconductor photonic wires in the strong exciton-photon coupling regime, it is predicted to occur on an experimentally accessible length scale.Comment: 6 pages, 3 figure

Probing few-particle Laughlin states of photons via correlation measurements

We propose methods to create and observe Laughlin-like states of photons in a strongly nonlinear optical cavity. Such states of strongly interacting photons can be prepared by pumping the cavity with a Laguerre-Gauss beam, which has a well-defined orbital angular momentum per photon. The Laughlin-like states appear as sharp resonances in the particle-number-resolved transmission spectrum. Power spectrum and second-order correlation function measurements yield unambiguous signatures of these few-particle strongly-correlated states.Comment: 11 pages including appendice

A practical guide to density matrix embedding theory in quantum chemistry

Density matrix embedding theory (DMET) provides a theoretical framework to treat finite fragments in the presence of a surrounding molecular or bulk environment, even when there is significant correlation or entanglement between the two. In this work, we give a practically oriented and explicit description of the numerical and theoretical formulation of DMET. We also describe in detail how to perform self-consistent DMET optimizations. We explore different embedding strategies with and without a self-consistency condition in hydrogen rings, beryllium rings, and a sample S$_{\text{N}}$2 reaction. The source code for the calculations in this work can be obtained from \url{https://github.com/sebwouters/qc-dmet}.Comment: 41 pages, 10 figure

Observation of long-lived polariton states in semiconductor microcavities across the parametric threshold

The excitation spectrum around the pump-only stationary state of a polariton optical parametric oscillator (OPO) in semiconductor microcavities is investigated by time-resolved photoluminescence. The response to a weak pulsed perturbation in the vicinity of the idler mode is directly related to the lifetime of the elementary excitations. A dramatic increase of the lifetime is observed for a pump intensity approaching and exceeding the OPO threshold. The observations can be explained in terms of a critical slowing down of the dynamics upon approaching the threshold and the following onset of the soft Goldstone mode

Unstable and stable regimes of polariton condensation

Modulational instabilities play a key role in a wide range of nonlinear optical phenomena, leading e.g. to the formation of spatial and temporal solitons, rogue waves and chaotic dynamics. Here we experimentally demonstrate the existence of a modulational instability in condensates of cavity polaritons, arising from the strong coupling of cavity photons with quantum well excitons. For this purpose we investigate the spatiotemporal coherence properties of polariton condensates in GaAs-based microcavities under continuous-wave pumping. The chaotic behavior of the instability results in a strongly reduced spatial and temporal coherence and a significantly inhomogeneous density. Additionally we show how the instability can be tamed by introducing a periodic potential so that condensation occurs into negative mass states, leading to largely improved coherence and homogeneity. These results pave the way to the exploration of long-range order in dissipative quantum fluids of light within a controlled platform.Comment: 7 pages, 5 figure

Drag of superfluid current in bilayer Bose systems

An effect of nondissipative drag of a superfluid flow in a system of two Bose gases confined in two parallel quasi two-dimensional traps is studied. Using an approach based on introduction of density and phase operators we compute the drag current at zero and finite temperatures for arbitrary ratio of densities of the particles in the adjacent layers. We demonstrate that in a system of two ring-shape traps the "drag force" influences on the drag trap in the same way as an external magnetic flux influences on a superconducting ring. It allows to use the drag effect to control persistent current states in superfluids and opens a possibility for implementing a Bose analog of the superconducting Josephson flux qubit.Comment: 12 pages, 2 figures, new section is added, refs are adde

Many-body physics of a quantum fluid of exciton-polaritons in a semiconductor microcavity

Some recent results concerning nonlinear optics in semiconductor microcavities are reviewed from the point of view of the many-body physics of an interacting photon gas. Analogies with systems of cold atoms at thermal equilibrium are drawn, and the peculiar behaviours due to the non-equilibrium regime pointed out. The richness of the predicted behaviours shows the potentialities of optical systems for the study of the physics of quantum fluids.Comment: Proceedings of QFS2006 conference to appear on JLT

Quantised Vortices in an Exciton-Polariton Fluid

One of the most striking quantum effects in a low temperature interacting Bose gas is superfluidity. First observed in liquid 4He, this phenomenon has been intensively studied in a variety of systems for its amazing features such as the persistence of superflows and the quantization of the angular momentum of vortices. The achievement of Bose-Einstein condensation (BEC) in dilute atomic gases provided an exceptional opportunity to observe and study superfluidity in an extremely clean and controlled environment. In the solid state, Bose-Einstein condensation of exciton polaritons has now been reported several times. Polaritons are strongly interacting light-matter quasi-particles, naturally occurring in semiconductor microcavities in the strong coupling regime and constitute a very interesting example of composite bosons. Even though pioneering experiments have recently addressed the propagation of a fluid of coherent polaritons, still no conclusive evidence is yet available of its superfluid nature. In the present Letter, we report the observation of spontaneous formation of pinned quantised vortices in the Bose-condensed phase of a polariton fluid by means of phase and amplitude imaging. Theoretical insight into the possible origin of such vortices is presented in terms of a generalised Gross-Pitaevskii equation. The implications of our observations concerning the superfluid nature of the non-equilibrium polariton fluid are finally discussed.Comment: 14 pages, 4 figure