Lifetime of the surface magnetoplasmons in metallic nanoparticles

We study the influence of an external magnetic field on the collective electronic excitations in metallic nanoparticles. While the usual surface plasmon corresponding to the collective oscillation of the electrons with respect to the ionic background persists in the direction parallel to the magnetic field, the components in the perpendicular plane are affected by the field and give rise to two collective modes with field-dependent frequencies, the surface magnetoplasmons. We analyze the decay of these collective excitations by their coupling to particle-hole excitations and determine how their lifetimes are modified by the magnetic field. In particular, we show that the lifetime of the usual surface plasmon is not modified by the magnetic field, while the lifetime of the two surface magnetoplasmons present a weak magnetic-field dependence. Optical spectroscopy experiments are suggested in which signatures of the surface magnetoplasmons may be observed.Comment: 11 pages, 6 figures; published versio

Transmission phase of a quantum dot and statistical fluctuations of partial-width amplitudes

Experimentally, the phase of the amplitude for electron transmission through a quantum dot (transmission phase) shows the same pattern between consecutive resonances. Such universal behavior, found for long sequences of resonances, is caused by correlations of the signs of the partial-width amplitudes of the resonances. We investigate the stability of these correlations in terms of a statistical model. For a classically chaotic dot, the resonance eigenfunctions are assumed to be Gaussian distributed. Under this hypothesis, statistical fluctuations are found to reduce the tendency towards universal phase evolution. Long sequences of resonances with universal behavior only persist in the semiclassical limit of very large electron numbers in the dot and for specific energy intervals. Numerical calculations qualitatively agree with the statistical model but quantitatively are closer to universality.Comment: 8 pages, 4 figure

Decay of dark and bright plasmonic modes in a metallic nanoparticle dimer

We develop a general quantum theory of the coupled plasmonic modes resulting from the near-field interaction between localized surface plasmons in a heterogeneous metallic nanoparticle dimer. In particular, we provide analytical expressions for the frequencies and decay rates of the bright and dark plasmonic modes. We show that, for sufficiently small nanoparticles, the main decay channel for the dark plasmonic mode, which is weakly coupled to light and, hence, immune to radiation damping, is of nonradiative origin and corresponds to Landau damping, i.e., decay into electron-hole pairs.Comment: 9 pages, 3 figures; published versio

Surface plasmon in metallic nanoparticles: renormalization effects due to electron-hole excitations

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the surface plasmon resonance. A redshift with respect to the classical Mie frequency appears in addition to the one caused by the spill-out of the electronic density outside the nanoparticle. We characterize the spill-out effect by means of a semiclassical expansion and obtain its dependence on temperature and the size of the nanoparticle. We demonstrate that both, the spill-out and the environment-induced shift are necessary to explain the experimentally observed frequencies and confirm our findings by time-dependent local density approximation calculations of the resonance frequency. The size and temperature dependence of the environmental influence results in a qualitative agreement with pump-probe spectroscopic measurements of the differential light transmission.Comment: 15 pages, 8 figures; version accepted in PR

Topological plasmons in dimerized chains of nanoparticles: robustness against long-range quasistatic interactions and retardation effects

We present a simple model of collective plasmons in a dimerized chain of spherical metallic nanoparticles, an elementary example of a topologically nontrivial nanoplasmonic system. Taking into account long-range quasistatic dipolar interactions throughout the chain, we provide an exact analytical expression for the full quasistatic bandstructure of the collective plasmons. An explicit calculation of the Zak phase proves the robustness of the topological physics of the system against the inclusion of long-range Coulomb interactions, despite the broken chiral symmetry. Using an open quantum systems approach, which includes retardation through the plasmon-photon coupling, we go on to analytically evaluate the resulting radiative frequency shifts of the plasmonic spectrum. The bright plasmonic bands experience size-dependent radiative shifts, while the dark bands are essentially unaffected by the light-matter coupling. Notably, the upper transverse-polarized band presents a logarithmic singularity where the quasistatic spectrum intersects the light cone. At wavevectors away from this intersection and for subwavelength nanoparticles, the plasmon-photon coupling only leads to a quantitative reconstruction of the bandstructure and the topologically-protected states at the edge of the first Brillouin zone are essentially unaffected.Comment: 15 pages, 6 figures, published versio

Nonradiative limitations to plasmon propagation in chains of metallic nanoparticles

We investigate the collective plasmonic modes in a chain of metallic nanoparticles that are coupled by near-field interactions. The size- and momentum-dependent nonradiative Landau damping and radiative decay rates are calculated analytically within an open quantum system approach. These decay rates determine the excitation propagation along the chain. In particular, the behavior of the radiative decay rate as a function of the plasmon wavelength leads to a transition from an exponential decay of the collective excitation for short distances to an algebraic decay for large distances. Importantly, we show that the exponential decay is of a purely nonradiative origin. Our transparent model enables us to provide analytical expressions for the polarization-dependent plasmon excitation profile along the chain and for the associated propagation length. Our theoretical analysis constitutes an important step in the quest for the optimal conditions for plasmonic propagation in nanoparticle chains.Comment: 14 pages, 6 figures; v2: published versio

Manipulating type-I and type-II Dirac polaritons in cavity-embedded honeycomb metasurfaces

Pseudorelativistic Dirac quasiparticles have emerged in a plethora of artificial graphene systems that mimic the underlying honeycomb symmetry of graphene. However, it is notoriously difficult to manipulate their properties without modifying the lattice structure. Here we theoretically investigate polaritons supported by honeycomb metasurfaces and, despite the trivial nature of the resonant elements, we unveil rich Dirac physics stemming from a non-trivial winding in the light-matter interaction. The metasurfaces simultaneously exhibit two distinct species of massless Dirac polaritons, namely type-I and type-II. By modifying only the photonic environment via an enclosing cavity, one can manipulate the location of the type-II Dirac points, leading to qualitatively different polariton phases. This enables one to alter the fundamental properties of the emergent Dirac polaritons while preserving the lattice structure - a unique scenario which has no analog in real or artificial graphene systems. Exploiting the photonic environment will thus give rise to unexplored Dirac physics at the subwavelength scale

Euler buckling instability and enhanced current blockade in suspended single-electron transistors

Single-electron transistors embedded in a suspended nanobeam or carbon nanotube may exhibit effects originating from the coupling of the electronic degrees of freedom to the mechanical oscillations of the suspended structure. Here, we investigate theoretically the consequences of a capacitive electromechanical interaction when the supporting beam is brought close to the Euler buckling instability by a lateral compressive strain. Our central result is that the low-bias current blockade, originating from the electromechanical coupling for the classical resonator, is strongly enhanced near the Euler instability. We predict that the bias voltage below which transport is blocked increases by orders of magnitude for typical parameters. This mechanism may make the otherwise elusive classical current blockade experimentally observable.Comment: 15 pages, 10 figures, 1 table; published versio

Large current noise in nanoelectromechanical systems close to continuous mechanical instabilities

We investigate the current noise of nanoelectromechanical systems close to a continuous mechanical instability. In the vicinity of the latter, the vibrational frequency of the nanomechanical system vanishes, rendering the system very sensitive to charge fluctuations and, hence, resulting in very large (super-Poissonian) current noise. Specifically, we consider a suspended single-electron transistor close to the Euler buckling instability. We show that such a system exhibits an exponential enhancement of the current noise when approaching the Euler instability which we explain in terms of telegraph noise.Comment: 11 pages, 12 figures; v2: minor changes, published versio