139 research outputs found

    Developments for resonance ionization laser spectroscopy of the heaviest elements at SHIP

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    The experimental determination of atomic levels and the first ionization potential of the heaviest elements (Z >= 100) is key to challenge theoretical predictions and to reveal changes in the atomic shell structure. These elements are only artificially produced in complete-fusion evaporation reactions at on-line facilities such as the GSI in Darmstadt at a rate of, at most, a few atoms per second. Hence, highly sensitive spectroscopic methods are required. Laser spectroscopy is one of the most powerful and valuable tools to investigate atomic properties. In combination with a buffer-gas filled stopping cell, the Radiation Detected Resonance Ionization Spectroscopy (RADRIS) technique provides the highest sensitivity for laser spectroscopy on the heaviest elements. The RADRIS setup, as well as the measurement procedure, have been optimized and characterized using the a-emitter 155Yb in on-line conditions, resulting in an overall efficiency well above 1%. This paves the way for a successful search of excited atomic levels in nobelium and heavier elements.publisher: Elsevier articletitle: Developments for resonance ionization laser spectroscopy of the heaviest elements at SHIP journaltitle: Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms articlelink: http://dx.doi.org/10.1016/j.nimb.2016.06.001 content_type: article copyright: © 2016 Elsevier B.V. All rights reserved.status: publishe

    Precision Measurement of the First Ionization Potential of Nobelium

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    One of the most important atomic properties governing an element’s chemical behavior is the energy required to remove its least-bound electron, referred to as the first ionization potential. For the heaviest elements, this fundamental quantity is strongly influenced by relativistic effects which lead to unique chemical properties. Laser spectroscopy on an atom-at-a-time scale was developed and applied to probe the optical spectrum of neutral nobelium near the ionization threshold. The first ionization potential of nobelium is determined here with a very high precision from the convergence of measured Rydberg series to be 6.626   21 ± 0.000   05     eV . This work provides a stringent benchmark for state-of-the-art many-body atomic modeling that considers relativistic and quantum electrodynamic effects and paves the way for high-precision measurements of atomic properties of elements only available from heavy-ion accelerator facilities

    Collateral Damage: Educational Attainment and Labor Market Outcomes Among German War and Post-War Cohorts

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    We use data from the West German 1970 census to explore the link between being born during or shortly after World War II and educational and labor market outcomes 25 years later. We document, for the first time, that men and women born in the relatively short period between November 1945 and May 1946 have significantly and substantially lower educational attainment and occupational status than cohorts born shortly before or after. Several alternative explanations for this new finding are put to test. Most likely, a short but severe spell of quantitative and qualitative malnutrition immediately around the end of the war has impaired intrauterine conditions in first trimester pregnancies and resulted in longterm detriments among the affected cohorts. This conjecture is corroborated by evidence from Austria

    Tuning Reactivity and Electronic Properties through Ligand Reorganization within a Cerium Heterobimetallic Framework

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