1,238 research outputs found
Double resonant absorption measurement of acetylene symmetric vibrational states probed with cavity ring down spectroscopy
A novel mid-infrared/near-infrared double resonant absorption setup for
studying infrared-inactive vibrational states is presented. A strong
vibrational transition in the mid-infrared region is excited using an idler
beam from a singly resonant continuous-wave optical parametric oscillator, to
populate an intermediate vibrational state. High output power of the optical
parametric oscillator and the strength of the mid-infrared transition result in
efficient population transfer to the intermediate state, which allows measuring
secondary transitions from this state with a high signal-to-noise ratio. A
secondary, near-infrared transition from the intermediate state is probed using
cavity ring down spectroscopy, which provides high sensitivity in this
wavelength region. Due to the narrow linewidths of the excitation sources, the
rovibrational lines of the secondary transition are measured with sub-Doppler
resolution. The setup is used to access a previously unreported symmetric
vibrational state of acetylene, in the
normal mode notation. Single-photon transitions to this state from the
vibrational ground state are forbidden. Ten lines of the newly measured state
are observed and fitted with the linear least-squares method to extract the
band parameters. The vibrational term value was measured to be at 9775.0018(45)
, the rotational parameter was 1.162222 ,
and the quartic centrifugal distortion parameter was 3.998(62), where the numbers in the parenthesis are one-standard
errors in the least significant digits
Fringe spacing and phase of interfering matter waves
We experimentally investigate the outcoupling of atoms from Bose-Einstein
condensates using two radio-frequency (rf) fields in the presence of gravity.
We show that the fringe separation in the resulting interference pattern
derives entirely from the energy difference between the two rf fields and not
the gravitational potential difference. We subsequently demonstrate how the
phase and polarisation of the rf radiation directly control the phase of the
matter wave interference and provide a semi-classical interpretation of the
results.Comment: 4 pages, 3 figure
Experimental cell for molecular beam deposition and magnetic resonance studies of matrix isolated radicals at temperatures below 1 K
We present the design and performance of an experimental cell constructed for matrix isolation studies of H and D atoms in solid H 2 /D 2 ïŹlms, which are created by molecular beam deposition at temperatures below 1 K. The sample cell allows sensitive weighing of the ïŹlms by a quartz microbalance (QM) and their studies by magnetic resonance techniques in a strong magnetic ïŹeld of 4.6 T. We are able to regulate the deposition rate in the range from 0.01 to 10 molecular layers/s, and measure the thickness with ≈ 0.2 monolayer resolution. The upper QM electrode serves as a mirror for a 128 GHz Fabry-Perot resonator connected to an electron spin resonance (ESR) spectrometer. H and D atoms were created by RF discharge in situ in the sample cell, and characterized by ESR and electron-nuclear double resonance. From the magnetic resonance measurements we conclude that the ïŹlms are smooth and provide homogeneous trapping conditions for embedded atoms. The current sample cell design also makes it possible to calibrate the ESR signal and estimate the average and local concentrations of H and D radicals in the ïŹlm.</p
Solar interacting protons versus interplanetary protons in the core plus halo model of diffusive shock acceleration and stochastic re-acceleration
With the first observations of solar Îł-rays from the decay of pions, the relationship of protons producing ground level enhancements (GLEs) on the Earth to those of similar energies producing the Îł-rays on the Sun has been debated. These two populations may be either independent and simply coincident in large flares, or they may be, in fact, the same population stemming from a single accelerating agent and jointly distributed at the Sun and also in space. Assuming the latter, we model a scenario in which particles are accelerated near the Sun in a shock wave with a fraction transported back to the solar surface to radiate, while the remainder is detected at Earth in the form of a GLE. Interplanetary ions versus ions interacting at the Sun are studied for a spherical shock wave propagating in a radial magnetic field through a highly turbulent radial ray (the acceleration core) and surrounding weakly turbulent sector in which the accelerated particles can propagate toward or away from the Sun. The model presented here accounts for both the first-order Fermi acceleration at the shock front and the second-order, stochastic re-acceleration by the turbulence enhanced behind the shock. We find that the re-acceleration is important in generating the Îł-radiation and we also find that up to 10% of the particle population can find its way to the Sun as compared to particles escaping to the interplanetary space
Overdiagnosis and overtreatment of breast cancer: Overdiagnosis in randomised controlled trials of breast cancer screening
Data from randomised controlled trials of mammographic screening can be used to determine the extent of any overdiagnosis, as soon as either a time equivalent to the lead-time has elapsed after the final screen, or the control arm has been offered screening. This paper reviews those randomised trials for which breast cancer incidence data are available. In recent trials in which the control group has not been offered screening, an excess incidence of breast cancer remains after many years of follow-up. In those trials in which the control arm has been offered screening, although there is a possible shift from invasive to in situ disease, there is no evidence of overdiagnosis as a result of incident screens
Cantilever-Enhanced Photoacoustic Spectroscopy of Radioactive Methane
We report the first high-resolution spectroscopy study of radiocarbon methane, 14CH4. Several absorption lines of the fundamental vibrational band v3 were measured using a continuous-wave mid-infrared optical parametric oscillator with cantilever-enhanced photoacoustic spectroscopy. © 2020 OSA.Peer reviewe
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