Picosecond acoustics in single quantum wells of cubic GaN/(Al,Ga)N

A picosecond acoustic pulse is used to study the photoelastic interaction in single zinc-blende GaN/AlxGa1−xN quantum wells. We use an optical time-resolved pump-probe setup and demonstrate that tuning the photon energy to the quantum well’s lowest electron-hole transition makes the experiment sensitive to the quantum well only. Because of the small width, its temporal and spatial resolution allows us to track the few-picosecond-long transit of the acoustic pulse. We further deploy a model to analyze the unknown photoelastic coupling strength of the quantum well for different photon energies and find good agreement with the experiments

Controlled lasing from active optomechanical resonators

Planar microcavities with distributed Bragg reflectors (DBRs) host, besides confined optical modes, also mechanical resonances due to stop bands in the phonon dispersion relation of the DBRs. These resonances have frequencies in the sub-terahertz (10E10-10E11 Hz) range with quality factors exceeding 1000. The interaction of photons and phonons in such optomechanical systems can be drastically enhanced, opening a new route toward manipulation of light. Here we implemented active semiconducting layers into the microcavity to obtain a vertical-cavity surface-emitting laser (VCSEL). Thereby three resonant excitations -photons, phonons, and electrons- can interact strongly with each other providing control of the VCSEL laser emission: a picosecond strain pulse injected into the VCSEL excites long-living mechanical resonances therein. As a result, modulation of the lasing intensity at frequencies up to 40 GHz is observed. From these findings prospective applications such as THz laser control and stimulated phonon emission may emerge

Systematic study of the influence of coherent phonon wave packets on the lasing properties of a quantum dot ensemble

Kohärente Phononen können die Licht-Materie-Wechselwirkung in Halbleiter Nanostrukturen stark ändern. Bei einem Ensemble von Quantenpunkten (QP) als aktivem Lasermedium sind Phononen im Stande, die Laserintensität deutlich zu verstärken oder abzuschwächen. Die Physik des gekoppelten Phonon-Exziton-Licht-Systems wird von verschiedenen Mechanismen dominiert, die im Experiment nicht eindeutig unterschieden werden können, da die komplizierte Probenstruktur zu einem komplexen Verspannungspuls führt, der auf das QP-Ensemble trifft. Hier zeigen wir durch eine umfassende theoretische Studie, wie die Laseremission durch Phononpulse verschiedener Form und QP-Ensembles verschiedener spektraler Verteilung beeinflusst wird. Dies erlaubt einen Einblick in die grundlegenden Wechselspiele des gekoppelten Gesamtsystems. Dadurch können wir zwischen zwei Mechanismen unterschieden: der adiabatischen Verschiebung des Ensembles und dem Schüttel-Effekt. Dies ebnet den Weg zu einer gezielten Kontrolle der Laser Emission durch kohärente Phononen.Coherent phonons can greatly vary light–matter interaction in semiconductor nanostructures placed inside an optical resonator on a picosecond time scale. For an ensemble of quantum dots (QDs) as active laser medium, phonons are able to induce a large enhancement or attenuation of the emission intensity, as has been recently demonstrated. The physics of this coupled phonon–exciton–light system consists of various effects, which in the experiment typically cannot be clearly separated, in particular, due to the complicated sample structure a rather complex strain pulse impinges on the QD ensemble. Here we present a comprehensive theoretical study how the laser emission is affected by phonon pulses of various shapes as well as by ensembles with different spectral distributions of the QDs. This gives insight into the fundamental interaction dynamics of the coupled phonon–exciton–light system, while it allows us to clearly discriminate between two prominent effects: the adiabatic shifting of the ensemble and the shaking effect. This paves the way to a tailored laser emission controlled by phonons.</p

Picosecond control of quantum dot laser emission by coherent phonons

A picosecond acoustic pulse can be used to control the lasing emission from semiconductor nanostructures by shifting their electronic transitions. When the active medium, here an ensemble of (In,Ga)As quantum dots, is shifted into or out of resonance with the cavity mode, a large enhancement or suppression of the lasing emission can dynamically be achieved. Most interesting, even in the case when gain medium and cavity mode are in resonance, we observe an enhancement of the lasing due to shaking by coherent phonons. In order to understand the interactions of the nonlinearly coupled photon-exciton-phonon subsystems, we develop a semiclassical model and find an excellent agreement between theory and experiment

Impact of nanomechanical resonances on lasing from electrically pumped quantum dot micropillars

The work was sponsored by the German Ministry of Education and Research (BMBF) within the RELQUSA project (FKZ: 13N12462) and the Deutsche Forschungsgemeinschaft (Ba1549/14-1 and Collaborative Research Centre TRR 142). The work was also supported by the state of Bavaria. A.V.A. acknowledges the Alexander-von-Humboldt Foundation. S.H. acknowledges support by the Royal Society and the Wolfson Foundation. Date of Acceptance: 06/01/2015We use a picosecond acoustics technique to modulate the laser output of electrically pumped GaAs/AlAs micropillar lasers with InGaAs quantum dots. The modulation of the emission wavelength takes place on the frequencies of the nanomechanical extensional and breathing (radial) modes of the micropillars. The amplitude of the modulation for various nanomechanical modes is different for every micropillar which is explained by a various elastic contact between the micropillar walls and polymer environment.Publisher PDFPeer reviewe

Nonlinear spectroscopy of exciton-polaritons in a GaAs-based microcavity

We present a systematic investigation of two-photon excitation processes in a GaAs-based microcavity in the strong-coupling regime. We observe second harmonic generation resonant to the upper and lower polariton level, which exhibits a strong dependence on the photonic fraction of the corresponding polariton. In addition, we have performed two-photon excitation spectroscopy to identify 2p exciton states which are crucial for the operation as a terahertz lasing device, which was suggested recently [A. V. Kavokin et al., Phys. Rev. Lett. 108, 197401 (2012)]. However, no distinct signatures of a 2p exciton state could be identified, which indicates a low two-photon pumping efficiency

Acousto-optical nanoscopy of buried photonic nanostructures

We develop a nanoscopy method with in-depth resolution for layered photonic devices. Photonics often require tailored light field distributions for the operated optical modes and an exact knowledge of the geometry of a device is crucial to assess its performance. We present an acousto-optical nanoscopy method for the characterization of layered photonic structures based on the uniqueness of the light field distributions: for a given wavelength, we record the reflectivity modulation during the transit of a picosecond acoustic pulse. The obtained temporal profile can be linked to the internal light field distribution. From this information, a reverse-engineering procedure allows us to reconstruct the light field and the underlying photonic structure very precisely. We apply this method to the slow light mode of an AlAs/GaAs micropillar resonator and show its validity for the tailored experimental conditions

Picosecond control of quantum dot laser emission by coherent phonons

A picosecond acoustic pulse can be used to control the lasing emission from semiconductor nanostructures by shifting their electronic transitions. When the active medium, here an ensemble of (In,Ga)As quantum dots, is shifted into or out of resonance with the cavity mode, a large enhancement or suppression of the lasing emission can dynamically be achieved. Most interesting, even inthe case when gain medium and cavity mode are in resonance, we observe an enhancement of the lasing due to shaking by coherent phonons. In order to understand the interactions of the nonlinearly coupled photon-exciton-phonon subsystems, we develop a semiclassical model and find an excellent agreement between theory and experiment