Visible quantum plasmonics from metallic nanodimers

We report theoretical evidence that bulk nonlinear materials weakly interacting with highly localized plasmonic modes in ultra-sub-wavelength metallic nanostructures can lead to nonlinear effects at the single plasmon level in the visible range. In particular, the two-plasmon interaction energy in such systems is numerically estimated to be comparable with the typical plasmon linewidths. Localized surface plasmons are thus predicted to exhibit a purely nonclassical behavior, which can be clearly identified by a sub-Poissonian second-order correlation in the signal scattered from the quantized plasmonic field under coherent electromagnetic excitation. We explicitly show that systems sensitive to single-plasmon scattering can be experimentally realized by combining electromagnetic confinement in the interstitial region of gold nanodimers with local infiltration or deposition of ordinary nonlinear materials. We also propose configurations that could allow to realistically detect such an effect with state-of-the-art technology, overcoming the limitations imposed by the short plasmonic lifetime

Social Housing in the 60s in São Paulo

The 60s was a decade of profound change in Brazil. The federal capital was transferred to Brasília, which represented the realization of the ideal of the modern city envisaged at CIAM IV. Modern architecture, which in its Brazilian version, was characterized by the Escola Carioca (Rio de Janeiro School), gave way to the São Paulo avant-garde, concerned with truth to materials and social aspirations. In politics we saw the shift from a democratic government to a military dictatorship, which sought to legitimize itself through the creation of a state funding system to solve the nation’s housing deficit. These factors created the conditions for the development of a series of housing projects, including the exemplary project discussed in this paper

Spontaneous rotating vortex rings in a parametrically driven polariton fluid

We present the theoretical prediction of spontaneous rotating vortex rings in a parametrically driven quantum fluid of polaritons -- coherent superpositions of coupled quantum well excitons and microcavity photons. These rings arise not only in the absence of any rotating drive, but also in the absence of a trapping potential, in a model known to map quantitatively to experiments. We begin by proposing a novel parametric pumping scheme for polaritons, with circular symmetry and radial currents, and characterize the resulting nonequilibrium condensate. We show that the system is unstable to spontaneous breaking of circular symmetry via a modulational instability, following which a vortex ring with large net angular momentum emerges, rotating in one of two topologically distinct states. Such rings are robust and carry distinctive experimental signatures, and so they could find applications in the new generation of polaritonic devices.Comment: 6 pages, 4 figure

Exciting polaritons with quantum light

We discuss the excitation of polaritons---strongly-coupled states of light and matter---by quantum light, instead of the usual laser or thermal excitation. As one illustration of the new horizons thus opened, we introduce Mollow spectroscopy, a theoretical concept for a spectroscopic technique that consists in scanning the output of resonance fluorescence onto an optical target, from which weak nonlinearities can be read with high precision even in strongly dissipative environments.Comment: 5 pages, 3 figure

Linear and nonlinear coupling of quantum dots in microcavities

We discuss the topical and fundamental problem of strong-coupling between a quantum dot an the single mode of a microcavity. We report seminal quantitative descriptions of experimental data, both in the linear and in the nonlinear regimes, based on a theoretical model that includes pumping and quantum statistics.Comment: Proceedings of the symposium Nanostructures: Physics and Technology 2010 (http://www.ioffe.ru/NANO2010), 2 pages in proceedings styl

Dynamics of formation and decay of coherence in a polariton condensate

We study the dynamics of formation and decay of a condensate of microcavity polaritons. We investigate the relationship between the number of particles, the emission's linewidth and its degree of linear polarization which serves as the order parameter. Tracking the condensate's formation, we show that, even when interactions are negligible, coherence is not determined only by occupation of the ground state. As a result of the competition between the coherent and thermal fractions of the condensate, the highest coherence is obtained some time after the particle number has reached its maximum

Interaction and coherence of a plasmon-exciton polariton condensate

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical nanocavities have attracted increasing interests in the last decade. This interest results from their sub-diffraction mode volume, which offers access to extremely high photonic densities by exploiting strong scattering cross-sections. However, high absorption losses in metals have hindered the observation of collective coherent phenomena, such as condensation. In this work we demonstrate the formation of a non-equilibrium room temperature plasmon-exciton-polariton condensate with a long range spatial coherence, extending a hundred of microns, well over the excitation area, by coupling Frenkel excitons in organic molecules to a multipolar mode in a lattice of plasmonic nanoparticles. Time-resolved experiments evidence the picosecond dynamics of the condensate and a sizeable blueshift, thus measuring for the first time the effect of polariton interactions in plasmonic cavities. Our results pave the way to the observation of room temperature superfluidity and novel nonlinear phenomena in plasmonic systems, challenging the common belief that absorption losses in metals prevent the realization of macroscopic quantum states.Comment: 23 pages, 5 figures, SI 7 pages, 5 figure

Shake-up Processes in Intersubband Magneto-photoabsorption of a Two-Dimensional Electron Gas

I theoretically study shake-up processes in photoabsorption of an interacting low-density two-dimensional electron gas (2DEG) in magnetic fields. Such processes, in which an incident photon creates an electron-hole pair and simultaneously excites one electron to one of the higher Landau levels, were observed experimentally [D.R. Yakovlev et al., Phys. Rev. Lett. 79, 3974 (1997)] and were called combined exciton-cyclotron resonance (ExCR). The recently developed theory of ExCR [A.B. Dzyubenko, Phys. Rev. B 64, 241101 (2001)] allows for a consistent treatment of the Coulomb correlations, establishes the exact ExCR selection rules, and predicts the high field features of ExCR. In this work, I generalize the existing theory of high-field ExCR in the 2DEG to the case when the hole is excited to higher hole Landau levels.Comment: 4 pages, 3 figures; Proceedings NGS-11 (June 2003, Buffalo, NY, USA