673 research outputs found
Crystal-field effects in the mixed-valence compounds Yb2M3Ga9 (M= Rh, Ir)
Magnetic susceptibility, heat capacity, and electrical resistivity
measurements have been carried out on single crystals of the intermediate
valence compounds Yb2Rh3Ga9 and Yb2Ir3Ga9. These measurements reveal a large
anisotropy due apparently to an interplay between crystalline electric field
(CEF) and Kondo effects. The temperature dependence of magnetic susceptibility
can be modelled using the Anderson impurity model including CEF within an
approach based on the Non-Crossing Approximation.Comment: Accepted to Phys. Rev.
Field-induced magnetic transitions in the quasi-two-dimensional heavy-fermion antiferromagnets Ce_{n}RhIn_{3n+2} (n=1 or 2)
We have measured the field-dependent heat capacity in the tetragonal
antiferromagnets CeRhIn and CeRhIn, both of which have an
enhanced value of the electronic specific heat coefficient
mJ/mol-Ce K above . For the specific heat data at zero
applied magnetic field are consistent with the existence of an anisotropic
spin-density wave opening a gap in the Fermi surface for CeRhIn while
CeRhIn shows behavior consistent with a simple antiferromagnetic
magnon. From these results, the magnetic structure, in a manner similar to the
crystal structure, appears more two-dimensional in CeRhIn than in
CeRhIn where only about 12% of the Fermi surface remains ungapped
relative to 92% for CeRhIn. When both compounds behave in a
manner expected for heavy fermion systems as both and the electronic
heat capacity decrease as field is applied. When the field is applied in the
tetragonal basal plane (), CeRhIn and CeRhIn have very
similar phase diagrams which contain both first- and second-order field-induced
magnetic transitions .Comment: 15 pages, 4 figure
Charge-Doping driven Evolution of Magnetism and non-Fermi-Liquid Behavior in the Filled Skutterudite CePt4Ge12-xSbx
The filled-skutterudite compound CePt4Ge12 is situated close to the border
between intermediate-valence of Ce and heavy-fermion behavior. Substitution of
Ge by Sb drives the system into a strongly correlated and ultimately upon
further increasing the Sb concentration into an antiferromagnetically ordered
state. Our experiments evidence a delicate interplay of emerging Kondo physics
and the formation of a local 4f moment. An extended non-Fermi-liquid region,
which can be understood in the framework of a Kondo-disorder model, is
observed. Band-structure calculations support the conclusion that the physical
properties are governed by the interplay of electron supply via Sb substitution
and the concomitant volume effects.Comment: 5 pages, 3 Figur
High spin polarization in the ferromagnetic filled skutterudites KFe4Sb12 and NaFe4Sb12
The spin polarization of ferromagnetic alkali-metal iron antimonides KFe4Sb12
and NaFe4Sb12 is studied by point-contact Andreev reflection using
superconducting Nb and Pb tips. From these measurements an intrinsic transport
spin polarization Pt of 67% and 60% for the K and Na compound, respectively, is
inferred which establishes these materials as a new class of highly spin
polarized ferromagnets. The results are in accord with band structure
calculations within the local spin density approximation (LSDA) that predict
nearly 100% spin polarization in the density of states. We discuss the impact
of calculated Fermi velocities and spin fluctuations on Pt.Comment: Pdf file with fi
Inertial parameters and superfluid-to-normal phase transition in superdeformed bands
The quasiclassically exact solution for the second inertial parameter is found in self-consistent way. It is shown that superdeformation and
nonuniform pairing arising from the rotation induced pair density significantly
reduce this inertial parameter. The different limiting cases for ,
which allow to study an interplay between rapid rotation, pairing correlations,
and mean field deformation, are considered. The new signature for the
transition from pairing to normal phase is suggested in terms of the variation
of versus spin. Experimental data indicate the existence of
such transition in the three superdeformed mass regions.Comment: 8 pages, LaTeX, 3 figure
Interobserver Agreement for Endometrial Cancer Characteristics Evaluated on Biopsy Material
A shift toward a disease-based therapy designed according to patterns of failure and likelihood of nodal involvement predicted by pathologic determinants has recently led to considering a selective approach to lymphadenectomy for endometrial cancer. Therefore, it became critical to examine reproducibility of diagnosing the key determinants of risk, on preoperative endometrial tissue samples as well as the concordance between preoperative and postresection specimens. Six gynaecologic pathologists assessed 105 consecutive endometrial biopsies originally reported as positive for endometrial cancer for cell type (endometrioid versus nonendometrioid), tumor grade (FIGO 3-tiered and 2-tiered), nuclear grade, and risk category (low risk defined as endometrioid histology, grade 1 + 2 and nuclear grade <3). Interrater agreement levels were substantial for identification of nonendometrioid histology (κ = 0.63; SE = 0.025), high tumor grade (κ = 0.64; SE = 0.025), and risk category (κ = 0.66; SE = 0.025). The overall agreement was fair for nuclear grade (κ = 0.21; SE = 0.025). There is agreement amongst pathologists in identifying high-risk pathologic determinants on endometrial cancer biopsies, and these highly correlate with postresection specimens. This is ascertainment prerequisite adaptation of the paradigm shift in surgical staging of patients with endometrial cancer
Participation in Transition(s):Reconceiving Public Engagements in Energy Transitions as Co-Produced, Emergent and Diverse
This paper brings the transitions literature into conversation with constructivist Science and Technology Studies (STS) perspectives on participation for the first time. In doing so we put forward a conception of public and civil society engagement in sustainability transitions as co-produced, relational, and emergent. Through paying close attention to the ways in which the subjects, objects, and procedural formats of public engagement are constructed through the performance of participatory collectives, our approach offers a framework to open up to and symmetrically compare diverse and interconnected forms of participation that make up wider socio-technical systems. We apply this framework in a comparative analysis of four diverse cases of civil society involvement in UK low carbon energy transitions. This highlights similarities and differences in how these distinct participatory collectives are orchestrated, mediated, and subject to exclusions, as well as their effects in producing particular visions of the issue at stake and implicit models of participation and ‘the public’. In conclusion we reflect on the value of this approach for opening up the politics of societal engagement in transitions, building systemic perspectives of interconnected ‘ecologies of participation’, and better accounting for the emergence, inherent uncertainties, and indeterminacies of all forms of participation in transitions
Compressibility of and (M = Rh, Ir and Co) Compounds
The lattice parameters of the tetragonal compounds CeIn and
CeIn(Rh, Ir and Co) have been studied as a function of
pressure up to 15 GPa using a diamond anvil cell under both hydrostatic and
quasihydrostatic conditions at room temperature. The addition of In
layers to the parent CeIn compound is found to stiffen the lattice as the
2-layer systems (average of bulk modulus values is 70.4 GPa) have a
larger than CeIn (67 GPa), while the 1-layer systems with the are
even stiffer (average of is 81.4 GPa). Estimating the hybridization
using parameters from tight binding calculations shows that the dominant
hybridization is in nature between the Ce and In atoms. The values of
at the pressure where the superconducting transition temperature
reaches a maximum is the same for all CeIn compounds. By
plotting the maximum values of the superconducting transition temperature
versus for the studied compounds and Pu-based superconductors, we
find a universal versus behavior when these quantities are
normalized appropriately. These results are consistent with magnetically
mediated superconductivity.Comment: Updated version resubmitted to Phys. Rev.
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