563 research outputs found
Optical Activities as Computing Resources for Space-time Symmetries
It is known that optical activities can perform rotations. It is shown that
the rotation, if modulated by attenuations, can perform symmetry operations of
Wigner's little group which dictates the internal space-time symmetries of
elementary particles.Comment: 13 pages, to be published in J. Mod. Optic
Carrier recombination dynamics in InGaN/GaN multiple quantum wells
We have mesured the carrier recombination dynamics in InGaN/GaN multiple
quantum wells over an unprecedented range in intensity. We find that at times
shorter than 30\,ns, they follow an exponential form, and a power law at times
longer than 1\,s. To explain these biphasic dynamics, we propose a simple
three-level model where a charge-separated state interplays with the radiative
state through charge transfer following a tunneling mechanism. We show how the
distribution of distances in charge-separated states controls the dynamics at
long time. Our results imply that charge recombination happens on
nearly-isolated clusters of localization centers.Comment: 11 pages, 3 figures, accepted for publication in PHYSICAL REVIEW
Gain properties of dye-doped polymer thin films
Hybrid pumping appears as a promising compromise in order to reach the much
coveted goal of an electrically pumped organic laser. In such configuration the
organic material is optically pumped by an electrically pumped inorganic device
on chip. This engineering solution requires therefore an optimization of the
organic gain medium under optical pumping. Here, we report a detailed study of
the gain features of dye-doped polymer thin films. In particular we introduce
the gain efficiency , in order to facilitate comparison between different
materials and experimental conditions. The gain efficiency was measured with
various setups (pump-probe amplification, variable stripe length method, laser
thresholds) in order to study several factors which modify the actual gain of a
layer, namely the confinement factor, the pump polarization, the molecular
anisotropy, and the re-absorption. For instance, for a 600 nm thick 5 wt\% DCM
doped PMMA layer, the different experimental approaches give a consistent value
80 cm.MW. On the contrary, the usual model predicting the gain
from the characteristics of the material leads to an overestimation by two
orders of magnitude, which raises a serious problem in the design of actual
devices. In this context, we demonstrate the feasibility to infer the gain
efficiency from the laser threshold of well-calibrated devices. Besides,
temporal measurements at the picosecond scale were carried out to support the
analysis.Comment: 15 pages, 17 figure
Fifth-order two-quantum absorptive two-dimensional electronic spectroscopy of CdSe quantum dots
Two-quantum variants of two-dimensional electronic spectroscopy (2DES) have previously been used to characterize multi-exciton interactions in molecules and semiconductor nanostructures though many implementations are limited by phasing procedures or non-resonant signals. We implement 2DES using phase-cycling to simultaneously measure one-quantum and two-quantum spectra in colloidal CdSe quantum dots. In the pump–probe geometry, fully absorptive spectra are automatically acquired by measuring the sum of the rephasing and nonrephasing signals. Fifth-order two-quantum spectroscopy allows for direct access to multi-exciton states that may be obscured in excited state absorption signals due to population relaxation or third-order two-quantum spectra due to the non-resonant response
First-principles calculations for the adsorption of water molecules on the Cu(100) surface
First-principles density-functional theory and supercell models are employed
to calculate the adsorption of water molecules on the Cu(100) surface. In
agreement with the experimental observations, the calculations show that a H2O
molecule prefers to bond at a one-fold on-top (T1) surface site with a tilted
geometry. At low temperatures, rotational diffusion of the molecular axis of
the water molecules around the surface normal is predicted to occur at much
higher rates than lateral diffusion of the molecules. In addition, the
calculated binding energy of an adsorbed water molecule on the surfaces is
significantly smaller than the water sublimation energy, indicating a tendency
for the formation of water clusters on the Cu(100) surface.Comment: 5 pages, 3 figures, submitted to Phys. Rev.
An insight into polarization states of solid-state organic lasers
The polarization states of lasers are crucial issues both for practical
applications and fundamental research. In general, they depend in a combined
manner on the properties of the gain material and on the structure of the
electromagnetic modes. In this paper, we address this issue in the case of
solid-state organic lasers, a technology which enables to vary independently
gain and mode properties. Different kinds of resonators are investigated:
in-plane micro-resonators with Fabry-Perot, square, pentagon, stadium, disk,
and kite shapes, and external vertical resonators. The degree of polarization P
is measured in each case. It is shown that although TE modes prevail generally
(P>0), kite-shaped micro-laser generates negative values for P, i.e. a flip of
the dominant polarization which becomes mostly TM polarized. We at last
investigated two degrees of freedom that are available to tailor the
polarization of organic lasers, in addition to the pump polarization and the
resonator geometry: upon using resonant energy transfer (RET) or upon pumping
the laser dye to an higher excited state. We then demonstrate that
significantly lower P factors can be obtained.Comment: 12 pages, 12 figure
Assessing the Polarization of a Quantum Field from Stokes Fluctuation
We propose an operational degree of polarization in terms of the variance of
the projected Stokes vector minimized over all the directions of the Poincar\'e
sphere. We examine the properties of this degree and show that some problems
associated with the standard definition are avoided. The new degree of
polarization is experimentally determined using two examples: a bright squeezed
state and a quadrature squeezed vacuum.Comment: 4 pages, 2 figures. Comments welcome
Maximally polarized states for quantum light fields
The degree of polarization of a quantum state can be defined as its
Hilbert-Schmidt distance to the set of unpolarized states. We demonstrate that
the states optimizing this degree for a fixed average number of photons
present a fairly symmetric, parabolic photon statistics, with a
variance scaling as . Although no standard optical process yields
such a statistics, we show that, to an excellent approximation, a highly
squeezed vacuum can be considered as maximally polarized.Comment: 4 pages, 3 eps-color figure
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