74 research outputs found

    Modeling soil organic carbon change in croplands of China

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    Using 1990 conditions, we modeled carbon (C) and nitrogen (N) biogeochemical cycles in croplands of China (and, for comparison, the United States) to estimate the annual soil organic-carbon (SOC) balance for all cropland. Overall, we estimate that China\u27s croplands lost 1.6% of their SOC (to a depth of 0.3 m) in 1990, and that U.S. cropland lost 0.1%. A key element in this difference was that ∼25% of aboveground crop residue in China was returned to the soil, compared to ∼90% in the United States. In China, SOC losses were greatest in the northeast (∼103 kg C·ha–1·yr–1), and were generally smaller (\u3c0.5 × 103 kg C·ha–1·yr–1) in regions with a longer cultivation history. Some regions showed SOC gains, generally \u3c103 kg C·ha–1·yr–1. Reduced organic-matter input to China\u27s cropland soils, and lower overall SOC levels in those soils, led to lower levels of N mineralization in the simulations, consistent with higher rates of synthetic-fertilizer application in China. C and N cycles are closely linked to soil fertility, crop yield, and non-point-source environmental pollution

    Chemistry of aerosols, cloud droplets, and rain in the Puerto Rican marine atmosphere

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    The chemical changes occurring during the transformation of aerosols to cloud droplets and rain were observed in orographic clouds on the eastern end of the island of Puerto Rico. Comparisons of elemental ratios in particles and rain and of elemental particle size distributions in and out of the clouds demonstrated scavenging efficiencies of >100% for the elements I, Br, and Cl relative to Na and of <25% for the elements Al, Mn, and V relative to Na. These different scavenging efficiencies are consistent with predictions based on existing cloud physics theory and are a reflection of the geochemical properties of the aerosol consisting partly of a hygroscopic sea salt component containing I, Br, Cl, and Na and partly of a soil dust component containing Al, Mn, and possibly V

    BORON IN COASTAL NORTH FLORIDA RAINFALL.

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    Dissolved boron and sodium concentrations were determined in rainfall collected on the Gulf Coast of northern Florida in order to investigate chemical and physical processes influencing natural concentration levels in the coastal marine atmosphere. Rainfall samples were collected during summer showers, during drizzle and heavy downpours associated with winter frontal activities, and sequentially during tropical storm Becky. Mean calculated B enrichments E//N//a(B) for summer and winter sample sets were 32 and 11, respectively. A surprisingly constant concentration of 'excess' B above that expected from direct seawater injection of approximately 6 mu g 1** minus **1 was observed in the sequential Becky samples. The lower winter B/Na ratios, and thus the calculated E//N//a(B) values, appear related to higher Na concentrations; however, several alternative hypotheses can be advanced to explain the results, including greater particulate sea-salt injection during winter months, incorporation of soil materials with a B/Na ratio above the seawater value, and possible influences of temperature variation on gaseous B incorporation in rain and evaporation from the sea surface

    Methane flux from the Central Amazonian Floodplain

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    A total of 186 methane measurements from the three primary Amazon floodplain environments of open water lakes, flood forests, and floating grass mats were made over the period 18 July through 2 September 1985. These data indicate that emissions were lowest over open water lakes. Flux from flooded forests and grass mats was significantly higher. At least three transport processes contribute to tropospheric emissions: ebullition from sediments, diffusion along the concentration gradient from sediment to overlaying water to air, and transport through the roots and stems of aquatic plants. Measurements indicate that the first two of these processes are most significant. It was estimated that on the average bubbling makes up 49% of the flux from open water, 54% of that from flooded forests, and 64% of that from floating mats. If the measurements were applied to the entire Amazonian floodplain, it is calculated that the region could supply up to 12% of the estimated global natural sources of methane

    Role of carbon cycle observations and knowledge in carbon management

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    Author Posting. © Annual Reviews, 2003. This article is posted here by permission of Annual Reviews for personal use, not for redistribution. The definitive version was published in Annual Review of Environment and Resources 28 (2003): 521-558, doi:10.1146/annurev.energy.28.011503.163443.Agriculture and industrial development have led to inadvertent changes in the natural carbon cycle. As a consequence, concentrations of carbon dioxide and other greenhouse gases have increased in the atmosphere and may lead to changes in climate. The current challenge facing society is to develop options for future management of the carbon cycle. A variety of approaches has been suggested: direct reduction of emissions, deliberate manipulation of the natural carbon cycle to enhance sequestration, and capture and isolation of carbon from fossil fuel use. Policy development to date has laid out some of the general principles to which carbon management should adhere. These are summarized as: how much carbon is stored, by what means, and for how long. To successfully manage carbon for climate purposes requires increased understanding of carbon cycle dynamics and improvement in the scientific capabilities available for measurement as well as for policy needs. The specific needs for scientific information to underpin carbon cycle management decisions are not yet broadly known. A stronger dialogue between decision makers and scientists must be developed to foster improved application of scientific knowledge to decisions. This review focuses on the current knowledge of the carbon cycle, carbon measurement capabilities (with an emphasis on the continental scale) and the relevance of carbon cycle science to carbon sequestration goals.The National Center for Atmospheric Research is supported by the National Science Foundation

    Development of Atmospheric Tracer Methods To Measure Methane Emissions from Natural Gas Facilities and Urban Areas

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    A new, integrated methodology to locate and measure methane emissions from natural gas systems has been developed. Atmospheric methane sources are identified by elevated ambient CH4 concentrations measured with a mobile laser-based methane analyzer. The total methane emission rate from a source is obtained by simulating the source with a sulfur hexafluoride (SF6) tracer gas release and by measuring methane and tracer concentrations along downwind sampling paths using mobile, real-time analyzers. Combustion sources of methane are distinguished from noncombustion sources by concurrent ambient carbon dioxide measurements. Three variations on the tracer ratio method are described for application to (1) small underground vaults, (2) aboveground natural gas facilities, and (3) diffuse methane emissions from an entire town. Results from controlled releases and from replicate tests demonstrate that the tracer ratio approach can yield total emission rates to within approximately ±15%. The estimated accuracy of emission estimates for urban areas with a variety of diffuse emissions is ±50%. © 1995, American Chemical Society. All rights reserved

    Multiple novel prostate cancer susceptibility signals identified by fine-mapping of known risk loci among Europeans

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    Genome-wide association studies (GWAS) have identified numerous common prostate cancer (PrCa) susceptibility loci. We have fine-mapped 64 GWAS regions known at the conclusion of the iCOGS study using large-scale genotyping and imputation in 25 723 PrCa cases and 26 274 controls of European ancestry. We detected evidence for multiple independent signals at 16 regions, 12 of which contained additional newly identified significant associations. A single signal comprising a spectrum of correlated variation was observed at 39 regions; 35 of which are now described by a novel more significantly associated lead SNP, while the originally reported variant remained as the lead SNP only in 4 regions. We also confirmed two association signals in Europeans that had been previously reported only in East-Asian GWAS. Based on statistical evidence and linkage disequilibrium (LD) structure, we have curated and narrowed down the list of the most likely candidate causal variants for each region. Functional annotation using data from ENCODE filtered for PrCa cell lines and eQTL analysis demonstrated significant enrichment for overlap with bio-features within this set. By incorporating the novel risk variants identified here alongside the refined data for existing association signals, we estimate that these loci now explain ∼38.9% of the familial relative risk of PrCa, an 8.9% improvement over the previously reported GWAS tag SNPs. This suggests that a significant fraction of the heritability of PrCa may have been hidden during the discovery phase of GWAS, in particular due to the presence of multiple independent signals within the same regio

    Future global warming from atmospheric trace gases

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    Human activity this century has increased the concentrations of atmospheric trace gases, which in turn has elevated global surface temperatures by blocking the escape of thermal infrared radiation. Natural climate variations are masking this temperature increase, but further additions of trace gases during the next 65 years could double or even quadruple the present effects, causing the global average temperature to rise by at least 1 °C and possibly by more than 5 °C. If the rise continues into the twenty-second century, the global average temperature may reach higher values than have occurred in the past 10 million years. © 1986 Nature Publishing Group

    Clay Minerals and Oceanic Evolution

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