260 research outputs found
Magnetic Properties of a-Si films doped with rare-earth elements
Amorphous silicon films doped with Y, La, Gd, Er, and Lu rare-earth elements
(a-Si:RE) have been prepared by co-sputtering and studied by means of electron
spin resonance (ESR), dc-magnetization, ion beam analysis, optical
transmission, and Raman spectroscopy. For comparison the magnetic properties of
laser-crystallized and hydrogenated a-Si:RE films were also studied. It was
found that the rare-earth species are incorporated in the a-Si:RE films in the
RE3+ form and that the RE-doping depletes the neutral dangling bonds (D0)
density. The reduction of D0 density is significantly larger for the magnetic
REs (Gd3+ and Er3+) than for the non-magnetic ones (Y3+, La3+, Lu3+). These
results are interpreted in terms of a strong exchange-like interaction, J RE-DB
SRE SDB, between the spin of the magnetic REs and that of the D0. All our
Gd-doped Si films showed basically the same broad ESR Gd3+ resonance (DHpp ~
850 Oe) at g ~ 2.01, suggesting the formation of a rather stable RE-Si complex
in these films.Comment: 15 pages, 7 figure
Effect of antiferromagnetic exchange interactions on the Glauber dynamics of one-dimensional Ising models
We study the effect of antiferromagnetic interactions on the single spin-flip
Glauber dynamics of two different one-dimensional (1D) Ising models with spin
. The first model is an Ising chain with antiferromagnetic exchange
interaction limited to nearest neighbors and subject to an oscillating magnetic
field. The system of master equations describing the time evolution of
sublattice magnetizations can easily be solved within a linear field
approximation and a long time limit. Resonant behavior of the magnetization as
a function of temperature (stochastic resonance) is found, at low frequency,
only when spins on opposite sublattices are uncompensated owing to different
gyromagnetic factors (i.e., in the presence of a ferrimagnetic short range
order). The second model is the axial next-nearest neighbor Ising (ANNNI)
chain, where an antiferromagnetic exchange between next-nearest neighbors (nnn)
is assumed to compete with a nearest-neighbor (nn) exchange interaction of
either sign. The long time response of the model to a weak, oscillating
magnetic field is investigated in the framework of a decoupling approximation
for three-spin correlation functions, which is required to close the system of
master equations. The calculation, within such an approximate theoretical
scheme, of the dynamic critical exponent z, defined as (where \tau is the longest relaxation time and \xi is the
correlation length of the chain), suggests that the T=0 single spin-flip
Glauber dynamics of the ANNNI chain is in a different universality class than
that of the unfrustrated Ising chain.Comment: 5 figures. Phys. Rev. B (accepted July 12, 2007
Finite-size effects on the dynamic susceptibility of CoPhOMe single-chain molecular magnets in presence of a static magnetic field
The static and dynamic properties of the single-chain molecular magnet
[Co(hfac)NITPhOMe] are investigated in the framework of the Ising model
with Glauber dynamics, in order to take into account both the effect of an
applied magnetic field and a finite size of the chains. For static fields of
moderate intensity and short chain lengths, the approximation of a
mono-exponential decay of the magnetization fluctuations is found to be valid
at low temperatures; for strong fields and long chains, a multi-exponential
decay should rather be assumed. The effect of an oscillating magnetic field,
with intensity much smaller than that of the static one, is included in the
theory in order to obtain the dynamic susceptibility . We find
that, for an open chain with spins, can be written as a
weighted sum of frequency contributions, with a sum rule relating the
frequency weights to the static susceptibility of the chain. Very good
agreement is found between the theoretical dynamic susceptibility and the ac
susceptibility measured in moderate static fields ( kOe),
where the approximation of a single dominating frequency turns out to be valid.
For static fields in this range, new data for the relaxation time,
versus , of the magnetization of CoPhOMe at low temperature are
also well reproduced by theory, provided that finite-size effects are included.Comment: 16 pages, 9 figure
Diffusive-like effects and possible non trivial local topology on the half-Heusler YPdBi compound
FAPESP - FUNDAÇÃO DE AMPARO À PESQUISA DO ESTADO DE SÃO PAULOCNPQ - CONSELHO NACIONAL DE DESENVOLVIMENTO CIENTÍFICO E TECNOLÓGICOCAPES - COORDENAÇÃO DE APERFEIÇOAMENTO DE PESSOAL E NÍVEL SUPERIORFINEP - FINANCIADORA DE ESTUDOS E PROJETOSThe non-ambiguous experimental identification of topological states of matter is one of the main interesting problems regarding this new quantum state of matter. In particular, the half-Heusler family RMT (R = rare-earth, T = Pd, Pt or Au and T = Bi, Sb, Pb or Sn) could be a useful platform to explore these states due to their cubic symmetry and the topological properties tunable via their unit cell volume and/or the nuclear charges of the M and T atoms. In this work, we report electron spin resonance (ESR) and complementary macroscopic measurements in the Nd3+-doped putative topologically trivial semimetal YPdBi. Following the Nd3+ ESR lineshape as a function of microwave power, size of the particle and temperature, we have been able to observe an evolution from a Dysonian lineshape to a diffusive-like lineshape. Furthermore, the Nd3+ ESR intensity saturation is concentration dependent, which could be due to a phonon-bottleneck process. Comparing these results with the Nd3+-doped YPtBi, we discuss a possible scenario in which the Nd3+ ions could locally tune the topological properties of the system.8516FAPESP - FUNDAÇÃO DE AMPARO À PESQUISA DO ESTADO DE SÃO PAULOCNPQ - CONSELHO NACIONAL DE DESENVOLVIMENTO CIENTÍFICO E TECNOLÓGICOCAPES - COORDENAÇÃO DE APERFEIÇOAMENTO DE PESSOAL E NÍVEL SUPERIORFINEP - FINANCIADORA DE ESTUDOS E PROJETOSFAPESP - FUNDAÇÃO DE AMPARO À PESQUISA DO ESTADO DE SÃO PAULOCNPQ - CONSELHO NACIONAL DE DESENVOLVIMENTO CIENTÍFICO E TECNOLÓGICOCAPES - COORDENAÇÃO DE APERFEIÇOAMENTO DE PESSOAL E NÍVEL SUPERIORFINEP - FINANCIADORA DE ESTUDOS E PROJETOS2013/17427-72012/04870-72006/60440-02009/09247-32010/11949-32011/01564-02011/23650-52012/05903-6442230/2014-1304649/2013-9sem informaçãosem informação62. Annual Conference on Magnetism and Magnetic Materials (MMM)2017Pittsburgh, PAIEEE Magnetics SocietyAIP Publishin
Gradual transition from insulator to semimetal of CaEuB with increasing Eu concentration
The local environment of Eu (, ) in
CaEuB () is investigated by
means of electron spin resonance (ESR). For the spectra show
resolved \textit{fine} and \textit{hyperfine} structures due to the cubic
crystal \textit{electric} field and nuclear \textit{hyperfine} field,
respectively. The resonances have Lorentzian line shape, indicating an
\textit{insulating} environment for the Eu ions. For , as increases, the ESR lines broaden due to local
distortions caused by the Eu/Ca ions substitution. For , the lines broaden further and the spectra gradually change from
Lorentzian to Dysonian resonances, suggesting a coexistence of both
\textit{insulating} and \textit{metallic} environments for the Eu ions.
In contrast to CaGdB, the \textit{fine} structure is still
observable up to . For the \textit{fine} and
\textit{hyperfine} structures are no longer observed, the line width increases,
and the line shape is purely Dysonian anticipating the \textit{semimetallic}
character of EuB. This broadening is attributed to a spin-flip scattering
relaxation process due to the exchange interaction between conduction and
Eu electrons. High field ESR measurements for
reveal smaller and anisotropic line widths, which are attributed to magnetic
polarons and Fermi surface effects, respectively.Comment: Submitted to PR
Simultaneous existence of two spin-wave modes in ultrathin Fe/GaAs(001) films studied by Brillouin Light Scattering: experiment and theory
A double-peaked structure was observed in the {\it in-situ} Brillouin Light
Scattering (BLS) spectra of a 6 \AA thick epitaxial Fe/GaAs(001) film for
values of an external magnetic field , applied along the hard in plane
direction, lower than a critical value kOe. This experimental
finding is theoretically interpreted in terms of a model which assumes a
non-homogeneous magnetic ground state characterized by the presence of
perperpendicular up/down stripe domains. For such a ground state, two spin-wave
modes, namely an acoustic and an optic mode, can exist. Upon increasing the
field the magnetization tilts in the film plane, and for the
ground state is homogeneous, thus allowing the existence of just a single
spin-wave mode. The frequencies of the two spin-wave modes were calculated and
successfully compared with the experimental data. The field dependence of the
intensities of the corresponding two peaks that are present in the BLS spectra
was also estimated, providing further support to the above-mentioned
interpretation.Comment: Shortened version (7 pages). Accepted for publication in Physical
Review
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